Citation: Gongxun Yu, Fenghui Yang, Xu Han, Qiongyao Song, Jiangtao Zheng, Ying Qi, Tianming Chen, Qian Shen, Jingxia Qiu, Sheng Li. Oxygen functional groups modified amorphous hollow carbon bowls for pseudocapacitive Zn-ion storage[J]. Chinese Chemical Letters, ;2023, 34(12): 108288. doi: 10.1016/j.cclet.2023.108288 shu

Oxygen functional groups modified amorphous hollow carbon bowls for pseudocapacitive Zn-ion storage

Gongxun Yu ^{a, c} ,
Fenghui Yang ^a ,
Xu Han ^a ,
Qiongyao Song ^c ,
Jiangtao Zheng ^c ,
Ying Qi ^a ,
Tianming Chen ^a ,
Qian Shen ^a ,
Jingxia Qiu ^{b, c, *,} ,
Sheng Li ^{a, *,}

a.
Key Laboratory of Flexible Electronics (KLOFE) and Institute of Advanced Materials (IAM), Nanjing Tech University (NanjingTech), Nanjing 211816, China
b.
School of Physical and Mathematical Sciences, Nanjing Tech University (NanjingTech), Nanjing 211816, China
c.
Institute for Energy Research, Jiangsu University, Zhenjiang 212013, China

jxqiu@njtech.edu.cn

iamsli@njtech.edu.cn

Received Date: 24 January 2023
Revised Date: 16 February 2023
Accepted Date: 1 March 2023
Available Online: 5 March 2023

Figures(4)

Carbon is a promising capacitive electrode material for Zn-ion hybrid supercapacitors (ZHSCs), as it is low-cost, environmentally friendly, controllable and adjustable. By now, achieving both high energy and high power with carbon electrodes is still challenging, limited by their intrinsic properties. In this work, we have designed and presented an amorphous hollow carbon bowl material with surface chemical modifications of oxygen groups to figure out these concerns. The preparation of bowl-like structures and the storage behavior between Zn²⁺ and oxygen functional groups have also been discussed. With the contributions from its unique hollow structure and surface functional groups, it can significantly enhance the electrode pseudocapacitance and the entire electrochemical performance.
- Zn-ion hybrid supercapacitors,
- Hollow carbon bowls,
- Oxygen groups,
- Pseudocapacitance,
- Zn-ion storage
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