Citation: Chao Tan, Rui Tao, Zhihao Yang, Lei Yang, Xiaolei Huang, Yong Yang, Fei Qi, Zegao Wang. Tune the photoresponse of monolayer MoS₂ by decorating CsPbBr₃ perovskite nanoparticles[J]. Chinese Chemical Letters, ;2023, 34(7): 107979. doi: 10.1016/j.cclet.2022.107979 shu

Tune the photoresponse of monolayer MoS₂ by decorating CsPbBr₃ perovskite nanoparticles

Chao Tan ^a ,
Rui Tao ^a ,
Zhihao Yang ^a ,
Lei Yang ^a ,
Xiaolei Huang ^b ,
Yong Yang ^b ,
Fei Qi ^c ,
Zegao Wang ^{a, *,}

a.
College of Materials Science and Engineering, Sichuan University, Chengdu 610065, China
b.
State Key Laboratory of Solidification Processing, Center of Advanced Lubrication and Seal Materials, Northwestern Polytechnical University, Xi'an 710072, China
c.
College of Optoelectronic Engineering, Chongqing University of Posts and Telecommunications, Chongqing 400065, China

zegao@scu.edu.cn

Received Date: 17 September 2022
Revised Date: 29 October 2022
Accepted Date: 2 November 2022
Available Online: 5 November 2022

Figures(5)

Tuning the photoresponse of monolayer MoS₂ could extend its potential application in many fields, however, it is still a challenge. In this study, CsPbBr₃ nanoparticles were prepared and spin-coated on the surface of monolayer MoS₂ to fabricate hybrid CsPbBr₃/MoS₂ photodetectors. By combing the photoelectrical property of the CsPbBr₃, the synergistic effect has been systematically studied from its carrier mobility, photoresponse and detectivity. It was found that nanofilm-coating of CsPbBr₃ would impede the photoelectric performance due to the electron-hole recombination facilitated by the defects at the interface of CsPbBr₃ and MoS₂ films. While the nanoparticles decorating was observed to significantly improve the conductivity of the monolayer MoS₂, which also increased the on/off ratio of the MoS₂ transistor from 8.2 × 10³ to 4.4 × 10⁴, and enhanced the carrier mobility from 0.090 cm² V⁻¹ s⁻¹ to 0.202 cm² V⁻¹ s⁻¹, ascribing to a mixed electron recombination-injection process. Furthermore, the CsPbBr₃ nanofilm would decrease the responsivity to 136 and 178 A/W under the light wavelength of 400 and 500 nm, respectively, while decorating CsPbBr₃ nanoparticles improve the photoresponse to 948 and 883 A/W with the detectivity at the level of 10¹¹ Jones. This work may provide an easy and cost-efficient way to tune the photoresponse of MoS₂ photodetectors.
- MoS₂ photodetector,
- CsPbBr₃ NPs,
- Surface charge doping,
- Carrier mobility,
- Photoresponse
1. [1]
  X. Song, J. Xu, L. Liu, et al., Appl. Surf. Sci. 542 (2021) 148437. doi: 10.1016/j.apsusc.2020.148437
2. [2]
  J. Wang, X. Xu, T. Cheng, et al., Nat. Nanotechnol. 17 (2022) 33–38. doi: 10.1038/s41565-021-01004-0
3. [3]
  H. Huang, J. Zha, S. Li, et al., Chin. Chem. Lett. 33 (2022) 163–176. doi: 10.1016/j.cclet.2021.06.004
4. [4]
  X. Niu, Y. Yu, J. Yao, et al., Chem. Phys. Lett. 772 (2021) 138571. doi: 10.1016/j.cplett.2021.138571
5. [5]
  D.S. Schneider, A. Grundmann, A. Bablich, et al., ACS Photonics 7 (2020) 1388–1395. doi: 10.1021/acsphotonics.0c00361
6. [6]
  X. Luo, Z. Peng, Z. Wang, et al., ACS Appl. Mater. Interfaces 13 (2021) 59154–59163. doi: 10.1021/acsami.1c19906
7. [7]
  M. Liao, Z. Wei, L. Du, et al., Nat. Commun. 11 (2020) 2153. doi: 10.1038/s41467-020-16056-4
8. [8]
  L. Wang, X. Li, C. Pei, et al., Chin. Chem. Lett. 33 (2022) 2611–2616. doi: 10.1016/j.cclet.2021.09.094
9. [9]
  S. Luo, C.P. Cullen, G. Guo, et al., Appl. Surf. Sci. 508 (2020) 145126. doi: 10.1016/j.apsusc.2019.145126
10. [10]
  R. Muñoz, E. López-Elvira, C. Munuera, et al., Appl. Surf. Sci. 581 (2022) 151858. doi: 10.1016/j.apsusc.2021.151858
11. [11]
  J. Zha, M. Luo, M. Ye, et al., Adv. Funct. Mater. 32 (2022) 2111970. doi: 10.1002/adfm.202111970
12. [12]
  L. Bu, Y. Qiu, P. Wei, et al., Phys. Rev. Appl. 6 (2016) 054022. doi: 10.1103/PhysRevApplied.6.054022
13. [13]
  C. Zhu, I. Ahmed, A. Parsons, et al., Polym. Compos. 39 (2018) 140–151. doi: 10.1002/pc.24499
14. [14]
  S. Cho, Y. Jo, H. Woo, et al., Appl. Sci. Converg. Technol. 26 (2017) 47–49. doi: 10.5757/ASCT.2017.26.3.47
15. [15]
  W. Wang, X. Niu, H. Qian, et al., Nanotechnology 27 (2016) 505204. doi: 10.1088/0957-4484/27/50/505204
16. [16]
  X. Liu, Z. Liu, J. Li, et al., J. Mater. Chem. C 8 (2020) 3337–3350. doi: 10.1039/C9TC06630F
17. [17]
  H. Min, D.Y. Lee, J. Kim, et al., Nature 598 (2021) 444–450. doi: 10.1038/s41586-021-03964-8
18. [18]
  R. Lin, J. Xu, M. Wei, et al., Nature 603 (2022) 73–78. doi: 10.1038/s41586-021-04372-8
19. [19]
  W. Zhai, J. Lin, C. Li, et al., Nanoscale 10 (2018) 21451–21458. doi: 10.1039/c8nr05683h
20. [20]
  Y. Li, Z.F. Shi, S. Li, et al., J. Mater. Chem. C 5 (2017) 8355–8360. doi: 10.1039/C7TC02137B
21. [21]
  Y. Meng, C. Lan, F. Li, et al., ACS Nano 13 (2019) 6060–6070. doi: 10.1021/acsnano.9b02379
22. [22]
  J. Duan, Y. Zhao, B. He, et al., Angew. Chem. Int. Ed. 57 (2018) 3787–3791. doi: 10.1002/anie.201800019
23. [23]
  G. Tong, T. Chen, H. Li, et al., Nano Energy 65 (2019) 104015. doi: 10.1016/j.nanoen.2019.104015
24. [24]
  K. Du, L. He, S. Song, et al., Adv. Funct. Mater. 31 (2021) 2103275. doi: 10.1002/adfm.202103275
25. [25]
  K.C. Tang, P. YouF. Yan, Sol. RRL 2 (2018) 1800075. doi: 10.1002/solr.201800075
26. [26]
  F. Palazon, S. Dogan, S. Marras, et al., J. Phys. Chem. C 121 (2017) 11956–11961. doi: 10.1021/acs.jpcc.7b03389
27. [27]
  J. Choi, H. ZhangJ. H. Choi, ACS Nano 10 (2016) 1671–1680. doi: 10.1021/acsnano.5b07457
28. [28]
  H. Ahn, Y.C. Huang, C.W. Lin, et al., ACS Appl. Mater. Interfaces 10 (2018) 29145–29152. doi: 10.1021/acsami.8b09378
29. [29]
  T. Han, H. Liu, S. Wang, et al., Nanomaterials 9 (2019) 740. doi: 10.3390/nano9050740
30. [30]
  C. Tan, C.D. Rudd, A.J. Parsons, et al., J. Mech. Behav. Biomed. Mater. 136 (2022) 105480. doi: 10.1016/j.jmbbm.2022.105480
31. [31]
  A. Syari'ati, S. Kumar, A. Zahid, et al., Chem. Commun. 55 (2019) 10384–10387. doi: 10.1039/c9cc01577a
32. [32]
  C.K. Cheng, C.H. Lin, H.C. Wu, et al., Nanoscale Res. Lett. 11 (2016) 117. doi: 10.1186/s11671-016-1277-0
33. [33]
  X. Pan, M. Yan, C. Sun, et al., Adv. Funct. Mater. 31 (2020) 2007840.
34. [34]
  J. Liu, F. Liu, H. Liu, et al., Nano Today 36 (2021) 101055. doi: 10.1016/j.nantod.2020.101055
35. [35]
  T. Qin, Z. Wang, Y. Wang, et al., Nano-Micro Lett. 13 (2021) 183. doi: 10.1007/s40820-021-00710-7
36. [36]
  B. Cao, Z. Ye, L. Yang, et al., Nanotechnology 32 (2021) 412001. doi: 10.1088/1361-6528/ac0d7c
37. [37]
  F. Li, R. Tao, B. Cao, et al., Adv. Funct. Mater. 31 (2021) 2104367. doi: 10.1002/adfm.202104367
38. [38]
  G. Tong, H. Li, D. Li, et al., Small 14 (2018) 1702523. doi: 10.1002/smll.201702523
39. [39]
  D. Wang, Z. Wang, Z. Yang, et al., Mater. Today Phys. 24 (2022) 100678. doi: 10.1016/j.mtphys.2022.100678
40. [40]
  J.D. Wood, S.A. Wells, D. Jariwala, et al., Nano Lett. 14 (2014) 6964–6970. doi: 10.1021/nl5032293
41. [41]
  W. Chen, K. Li, Y. Wang, et al., J. Phys. Chem. Lett. 8 (2017) 591–598. doi: 10.1021/acs.jpclett.6b02843
42. [42]
  L. Hao, Y. Du, Z. Wang, et al., Nanoscale 12 (2020) 7358–7365. doi: 10.1039/d0nr00319k
43. [43]
  C. Chen, Y. Wu, L. Liu, et al., Adv. Sci. 6 (2019) 1802046. doi: 10.1002/advs.201802046
44. [44]
  X.F. Zhang, L. Wei, L. Wang, et al., Appl. Phys. Lett. 102 (2013) 113501. doi: 10.1063/1.4795609
45. [45]
  D.B. Farmer, R. Golizadeh-Mojarad, V. Perebeinos, et al., Nano Lett. 9 (2009) 388–392. doi: 10.1021/nl803214a
46. [46]
  R. Tao, Z. Hao, C. Tan, et al., J. Electron. Sci. Technol. 20 (2022) 100167. doi: 10.1016/j.jnlest.2022.100167
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Tune the photoresponse of monolayer MoS₂ by decorating CsPbBr₃ perovskite nanoparticles