Citation: Li Ma, Xianang Gao, Xin Liu, Xiaojun Gu, Baoying Li, Beibei Mao, Zeyuan Sun, Wei Gao, Xiaofei Jia, Jianbin Chen. Recent advances in organic electrosynthesis using heterogeneous catalysts modified electrodes[J]. Chinese Chemical Letters, ;2023, 34(4): 107735. doi: 10.1016/j.cclet.2022.08.015 shu

Recent advances in organic electrosynthesis using heterogeneous catalysts modified electrodes

Li Ma ^{a, *,} ,
Xianang Gao ^a ,
Xin Liu ^a ,
Xiaojun Gu ^a ,
Baoying Li ^a ,
Beibei Mao ^b ,
Zeyuan Sun ^a ,
Wei Gao ^a ,
Xiaofei Jia ^c ,
Jianbin Chen ^{a, *,}

a.
Shandong Provincial Key Laboratory of Molecular Engineering, State Key Laboratory of Biobased Material and Green Papermaking, School of Chemistry and Chemical Engineering, Qilu University of Technology (Shandong Academy of Sciences), Ji'nan, 250353, China
b.
College of Pharmacy, Shandong University of Traditional Chinese Medicine, Ji'nan, 250355, China
c.
Key Laboratory of Optic-electric Sensing and Analytical Chemistry for Life Science, MOE, College of Chemistry and Molecular Engineering, Qingdao University of Science and Technology, Qingdao 266042, China

li_ma@qlu.edu.cn

jchen@qlu.edu.cn

Received Date: 25 April 2022
Revised Date: 27 July 2022
Accepted Date: 5 August 2022
Available Online: 10 August 2022

Figures(36)

Organic electrosynthesis as an emerging green and advantageous alternative to traditional synthetic methods has achieved remarkable progress in recent years because sustainable electricity can be employed as traceless redox agents. To surmount the over-oxidation/reduction issues of direct electrolysis, mediated or indirect electrochemical processes are attaining remarkable significance and promoting the selectivity of products. Molecular electrocatalysts, benefiting from the easily electronic and steric modulation, suffers from readily degradation issue in most cases. Remarkably, heterogeneous catalysts have drawn more attention due to their high activity, stability, and recyclability. Hence, in this review, the most recent growth of heterogeneous catalysts modified electrodes for organic electrosynthesis were summarized, highlighting structural optimization and electrochemical performance of these materials as well as reaction mechanism. Furthermore, key challenges and future directions in this area were also discussed.
- Organic electrosynthesis,
- Indirect electrosynthesis,
- Heterogeneous catalysis,
- Hybrid materials,
- Electrocatalysis
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