Citation: Minjun Liu, Ying Liu, Xinru Liu, Chengcheng Chu, Ducheng Yao, Shun Mao. Modification strategies on 2D Ni-Fe MOF-based catalysts in peroxydisulfate activation for efficient organic pollutant removal[J]. Chinese Chemical Letters, ;2023, 34(4): 107708. doi: 10.1016/j.cclet.2022.07.051 shu

Modification strategies on 2D Ni-Fe MOF-based catalysts in peroxydisulfate activation for efficient organic pollutant removal

Minjun Liu ^{a, b} ,
Ying Liu ^b, ,
Xinru Liu ^b ,
Chengcheng Chu ^b ,
Ducheng Yao ^b ,
Shun Mao ^{b, *,}

a.
College of Environmental and Chemical Engineering, Shanghai University of Electric Power, Shanghai 200090, China
b.
College of Environmental Science and Engineering, Biomedical Multidisciplinary Innovation Research Institute, Shanghai East Hospital, State Key Laboratory of Pollution Control and Resource Reuse, Tongji University, Shanghai 200092, China

yingliu@tongji.edu.cn

shunmao@tongji.edu.cn

Received Date: 22 April 2022
Revised Date: 2 July 2022
Accepted Date: 22 July 2022
Available Online: 25 July 2022

Figures(5)

This study reports several modification strategies to optimize and enhance the performance of two-dimensional (2D) metal organic frameworks (MOFs)-derived catalysts in peroxydisulfate (PDS) activation. The raw 2D Ni-MOF and 2D Ni-Fe-MOF without modification show poor catalytic activities for PDS activation and high metal ion leaching. The carbonization of 2D MOF can increase the activity of the catalyst but cannot solve the metal leaching problem. The further acid treatment of carbonization products can further improve the catalytic activity and decrease the metal ion leaching. The in-situ growth of 2D MOF on graphene oxide (GO) support with subsequent carbonization and acid treatment offers the best performance in PDS activation for organic pollutant removal with low metal ion leaching. Compared with other PDS systems, the Ni-Fe-C-acid/GO system displays much lower catalyst and PDS dosages for p-chloroaniline degradation. This study presents new insights in the modification strategies of 2D MOF-based catalysts in PDS activation.
- Peroxydisulfate oxidation,
- 2D MOF,
- Modification strategy,
- Synergistic effect,
- Organic pollutant removal
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