Citation: Xinxing Sun, Shuangke Liu, Weiwei Sun, Chunman Zheng. Emerging multifunctional iron-based nanomaterials as polysulfides adsorbent and sulfur species catalyst for lithium-sulfur batteries—A mini-review[J]. Chinese Chemical Letters, ;2023, 34(1): 107501. doi: 10.1016/j.cclet.2022.05.015 shu

Emerging multifunctional iron-based nanomaterials as polysulfides adsorbent and sulfur species catalyst for lithium-sulfur batteries—A mini-review

College of Aerospace Science and Engineering, National University of Defense Technology, Changsha 410073, China

liu_sk@139.com

wwsun@nudt.edu.cn

zhengchunman@nudt.edu.cn

Received Date: 19 January 2022
Revised Date: 3 April 2022
Accepted Date: 7 May 2022
Available Online: 11 May 2022

Figures(9)

Lithium-sulfur (Li-S) battery has been considered as one of the most promising next generation energy storage technologies for its overwhelming merits of high theoretical specific capacity (1673 mAh/g), high energy density (2500 Wh/kg), low cost, and environmentally friendliness of sulfur. However, critical drawbacks, including inherent low conductivity of sulfur and Li₂S, large volume changes of sulfur cathodes, undesirable shuttling and sluggish redox kinetics of polysulfides, seriously deteriorate the energy density, cycle life and rate capability of Li-S battery, and thus limit its practical applications. Herein, we reviewed the recent developments addressing these problems through iron-based nanomaterials for effective synergistic immobilization as well as conversion reaction kinetics acceleration for polysulfides. The mechanist configurations between different iron-based nanomaterials and polysulfides for entrapment and conversion acceleration were summarized at first. Then we concluded the recent progresses on utilizing various iron-based nanomaterials in Li-S battery as sulfur hosts, separators and cathode interlayers. Finally, we discussed the challenges and perspectives for designing high sulfur loading cathode architectures along with outstanding chemisorption capability and catalytic activity.
- Iron-based nanomaterials,
- Polysulfides,
- Chemical anchoring,
- Electrocatalyst,
- Lithium-sulfur batteries
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沈阳化工大学材料科学与工程学院沈阳 110142