Citation: Xuan Ding, Wanjun Yu, Xin Sheng, Hui Shi, Deng You, Mingming Peng, Penghui Shao, Liming Yang, Lingling Liu, Xubiao Luo. Feasible fabrication of o-phenanthroline-based polymer adsorbent for selective capture of aqueous Ag(Ⅰ)[J]. Chinese Chemical Letters, ;2023, 34(3): 107485. doi: 10.1016/j.cclet.2022.04.083 shu

Feasible fabrication of o-phenanthroline-based polymer adsorbent for selective capture of aqueous Ag(Ⅰ)

Xuan Ding ^{a, b} ,
Wanjun Yu ^{a, b} ,
Xin Sheng ^{a, b} ,
Hui Shi ^{a, b, *,} ,
Deng You ^{a, b} ,
Mingming Peng ^{a, b} ,
Penghui Shao ^{a, b} ,
Liming Yang ^{a, b} ,
Lingling Liu ^{a, b} ,
Xubiao Luo ^{a, b, *,}

a.
Key Laboratory of Jiangxi Province for Persistent Pollutants Control and Resources Recycle, Nanchang Hangkong University, Nanchang 330063, China
b.
National-Local Joint Engineering Research Center of Heavy Metals Pollutants Control and Resource Utilization, Nanchang Hangkong University, Nanchang 330063, China

shihui900501@126.com

luoxubiao@126.com

Received Date: 12 January 2022
Revised Date: 31 March 2022
Accepted Date: 29 April 2022
Available Online: 2 May 2022

Figures(6)

Devising a desirable adsorbent for efficiently selective capture of Ag(Ⅰ) from wastewater has attracted much attention but faced with huge challenges. Herein, a novel linear o-phenanthroline-based polymer l-PRL was prepared via chemical oxidative polymerization for the adsorption of Ag(Ⅰ). The maximum adsorption capacity for Ag(Ⅰ) by l-PRL is 325.8 mg/g at pH 0. In addition, l-PRL owes ascendant selectivity for Ag(Ⅰ) from aqueous solutions containing various interfering metal ions of Pb(Ⅱ), Co(Ⅱ), Ni(Ⅱ), Cd(Ⅱ) and Fe(Ⅲ). Multiple characterizations of FT-IR and XPS uncover that the N groups on l-PRL act as adsorption sites to coordinate with Ag(Ⅰ). Density functional theory (DFT) calculations further evidence the mechanism that l-PRL is provided with the admirable adsorptivity and selectivity for Ag(Ⅰ). It is mainly attributed to the most stable complexes of l-PRL with Ag(Ⅰ), which possesses shortest Ag-N bond length compared with other heavy metal ions. Furthermore, 93.5% of initial adsorption capacity is reserved after four continuous regeneration cycles, indicating that l-PRL is equipped with superior recyclability and durability, and l-PRL is capable of removing Ag(Ⅰ) in low-concentration actual Ag(Ⅰ)-containing wastewater completely. This study shed light on the rational design of polymer adsorbents and in-depth insight into selective removal of aqueous Ag(Ⅰ).
- Wastewater,
- o-Phenanthroline,
- Polymer,
- Adsorbent,
- Ag(Ⅰ),
- Selective capture
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