Citation: Kaiyue Song, Panke Zhou, Lulu Zong, Zhencong Yang, Haohong Li, Zhirong Chen. The visible light-triggered nonvolatile memory performances in melamine-decorated <110> -oriented lead halide perovskites: A photo-responsive structural evolution insight[J]. Chinese Chemical Letters, ;2023, 34(3): 107464. doi: 10.1016/j.cclet.2022.04.062 shu

The visible light-triggered nonvolatile memory performances in melamine-decorated <110> -oriented lead halide perovskites: A photo-responsive structural evolution insight

Kaiyue Song ^a ,
Panke Zhou ^a ,
Lulu Zong ^a ,
Zhencong Yang ^a ,
Haohong Li ^{a, b, c, *,} ,
Zhirong Chen ^{a, c, *,}

a.
College of Chemistry, Fuzhou University, Fuzhou 350108, China
b.
Fujian Engineering Research Center of Advanced Manufacturing Technology for Fine Chemicals, Fuzhou University, Fuzhou 350108, China
c.
Fujian Science and Technology Innovation Laboratory for Optoelectronic Information of China, Fuzhou 350108, China

lihh@fzu.edu.cn

zrchen@fzu.edu.cn

Received Date: 24 March 2022
Revised Date: 22 April 2022
Accepted Date: 25 April 2022
Available Online: 28 April 2022

Figures(7)

The exploration of novel photo/thermal-responsive nonvolatile memorizers will be beneficial for energy-saving memories. Herein, new <110> -oriented perovskites using single template melamine, i.e., [(MLAI-H₂)(PbX₄)] (X = Br (α-1), Cl (α-2), MLAI = melamine) have been prepared and their structures upon irradiation of visible light have been investigated. They have been fabricated as nonvolatile memory devices with structures of ITO/[(MLAI-H₂)(PbX₄)]/PMMA/Ag (device-1: X = Br, device-2: X = Cl), which can exhibit unique visible light-triggered binary nonvolatile memory performances. Interestingly, the silent or working status can be monitored by visible chromisms. Furthermore, the light-triggered binary resistive switching mechanisms of these ITO/[(MLAI-H₂)(PbX₄)]/PMMA/Ag memory devices have been clarified in terms of EPR, fluorescence, and single-crystal structural analysis. The presence of light-activated traps in <110> -oriented [(MLAI-H₂)(PbX₄)] perovskites are dominated in the appearance of light-triggered resistive switching behaviors, based on which the inverted internal electrical fields can be established. According to the structural analysis, the more distorted PbX₆ octahedra, higher corrugated <110> -oriented perovskite sheets, and more condensed organic-inorganic packing in Br-containing perovskite are beneficial for the stabilization of light-activated traps, which lead to the better resistive switching behavior of device-1. This work can pave a new avenue for the establishment of novel energy-saving nonvolatile memorizers used in aerospace or military industries.
- Nonvolatile memorizer,
- Light-triggered memory,
- <110> -Oriented lead halide perovskite,
- Photo-responsive structural evolution,
- Photochromisms
1. [1]
  J.P. Randall, M.A.B. Meador, S.C. Jana, ACS Appl. Mater. Interfaces 3 (2011) 613–626. doi: 10.1021/am200007n
2. [2]
  K. Fayazbakhsh, A. Abedian, Adv. Space Res. 45 (2010) 741–749. doi: 10.1016/j.asr.2009.11.017
3. [3]
  B.J. Choi, A.C. Torrezan, J.P. Strachan, et al., Adv. Funct. Mater. 26 (2016) 5290–5296. doi: 10.1002/adfm.201600680
4. [4]
  X. Wu, H. Yu, J. Cao, AIP Adv. 10 (2020) 085202. doi: 10.1063/1.5130914
5. [5]
  B. Chen, Y.R. Huang, K.Y. Song, et al., Chem. Mater. 33 (2021) 2178–2186. doi: 10.1021/acs.chemmater.1c00090
6. [6]
  Y.R. Huang, X.L. Lin, B. Chen, et al., Angew. Chem. Int. Ed. 60 (2021) 16911–16916. doi: 10.1002/anie.202104333
7. [7]
  J.J. Yang, D.B. Strukov, D.R. Stewart, Nat. Nanotechnol. 8 (2013) 13–24. doi: 10.1038/nnano.2012.240
8. [8]
  C. Gu, J.S. Lee, ACS Nano 10 (2016) 5413–5418. doi: 10.1021/acsnano.6b01643
9. [9]
  B. Hwang, J.S. Lee, Adv. Mater. 29 (2017) 1701048. doi: 10.1002/adma.201701048
10. [10]
  A. Younis, C.H. Lin, X. Guan, et al., Adv. Mater. 33 (2021) 2005000. doi: 10.1002/adma.202005000
11. [11]
  J.Y. Chen, Y.C. Chiu, Y.T. Li, et al., Adv. Mater. 29 (2017) 1702217. doi: 10.1002/adma.201702217
12. [12]
  Y. Wang, Z. Lv, Q. Liao, et al., Adv. Mater. 30 (2018) 1800327. doi: 10.1002/adma.201800327
13. [13]
  T. Paul, P.K. Sarkar, S. Maiti, et al., ACS Appl. Electron. Mater. 2 (2020) 3667–3677. doi: 10.1021/acsaelm.0c00719
14. [14]
  C.H. Chen, Y. Wang, H. Tatsumi, et al., Adv. Funct. Mater. 29 (2019) 1902991. doi: 10.1002/adfm.201902991
15. [15]
  Y.J. Jeong, D.J. Yun, S.H. Kim, et al., ACS Appl. Mater. Interfaces 9 (2017) 11759–11769. doi: 10.1021/acsami.7b02365
16. [16]
  Y.J. Jeong, D.J. Yun, S.H. Noh, et al., ACS Nano 12 (2018) 7701–7709. doi: 10.1021/acsnano.8b01413
17. [17]
  Y.H. Chang, C.W. Ku, Y.H. Zhang, et al., Adv. Funct. Mater. 30 (2020) 2000764. doi: 10.1002/adfm.202000764
18. [18]
  M.Y. Liao, Y.C. Chiang, C.H. Chen, et al., ACS Appl. Mater. Interfaces 12 (2020) 36398–36408. doi: 10.1021/acsami.0c10587
19. [19]
  S.J. Chang, S.Y. Chen, P.W. Chen, et al., ACS Appl. Mater. Interfaces 11 (2019) 33803–33810. doi: 10.1021/acsami.9b08766
20. [20]
  C. Ríos, M. Stegmaier, P. Hosseini, et al., Nat. Photonics 9 (2015) 725–732. doi: 10.1038/nphoton.2015.182
21. [21]
  L. Pedesseau, D. Sapori, B. Traore, et al., ACS Nano 10 (2016) 9776–9786. doi: 10.1021/acsnano.6b05944
22. [22]
  M. Yuan, L.N. Quan, R. Comin, et al., Nat. Nanotechnol. 11 (2016) 872–877. doi: 10.1038/nnano.2016.110
23. [23]
  J. Yin, D. Cortecchia, A. Krishna, et al., J. Phys. Chem. Lett. 6 (2015) 1396–1402. doi: 10.1021/acs.jpclett.5b00431
24. [24]
  Y.C. Shih, Y.B. Lan, C.S. Li, et al., Small 13 (2017) 1604305. doi: 10.1002/smll.201604305
25. [25]
  D.B. Mitzi, S. Wang, C.A. Feild, et al., Science 267 (1995) 1473–1476. doi: 10.1126/science.267.5203.1473
26. [26]
  S. Wang, D.B. Mitzi, C.A. Feild, et al., J. Am. Chem. Soc. 117 (1995) 5297–5302. doi: 10.1021/ja00124a012
27. [27]
  Y. Wang, W. Li, T. Zhang, et al., Small Methods 4 (2020) 1900511. doi: 10.1002/smtd.201900511
28. [28]
  Y. Li, G. Zheng, J. Lin, Eur. J. Inorg. Chem. 2008 (2008) 1689–1692.
29. [29]
  Y.Y. Li, C.K. Lin, G.L. Zheng, et al., Chem. Mater. 18 (2006) 3463–3469. doi: 10.1021/cm060714u
30. [30]
  Q. Liu, L. Zhao, W. Wu, et al., J. Mater. Chem. C 8 (2020) 3258–3267. doi: 10.1039/C9TC05843E
31. [31]
  S.G. Kim, J. Chen, J.Y. Seo, et al., ACS Appl. Mater. Interfaces 10 (2018) 25372–25383. doi: 10.1021/acsami.8b06616
32. [32]
  F. Yang, M.A. Kamarudin, D. Hirotani, et al., Sol. RRL 3 (2019) 1800275. doi: 10.1002/solr.201800275
33. [33]
  J.A. Alonso, M.J. Martínez-Lope, M.T. Casais, et al., Inorg. Chem. 39 (2000) 917–923. doi: 10.1021/ic990921e
34. [34]
  B. Hamdi, R. Zouari, A. Ben Salah, Superlattices Microstruct 123 (2018) 97–110. doi: 10.1016/j.spmi.2018.04.025
35. [35]
  T. Ishihara, J. Takahashi, T. Goto, Phys. Rev. B 42 (1990) 11099–11107. doi: 10.1103/PhysRevB.42.11099
36. [36]
  W. Nie, J.C. Blancon, A.J. Neukirch, et al., Nat. Commun. 7 (2016) 11574. doi: 10.1038/ncomms11574
37. [37]
  G. Ding, Y. Wang, G. Zhang, et al., Adv. Funct. Mater. 29 (2019) 1806637. doi: 10.1002/adfm.201806637
38. [38]
  Y. He, Y.R. Huang, Y.L. Li, et al., Inorg. Chem. 58 (2019) 13862–13880. doi: 10.1021/acs.inorgchem.9b01740
39. [39]
  W. Wu, X.L. Lin, Q. Liu, et al., Inorg. Chem. Front. 7 (2020) 1451–1466. doi: 10.1039/C9QI01672D
40. [40]
  X. Chen, P. Huang, X. Zhu, et al., Nanoscale Horiz. 4 (2019) 697–704. doi: 10.1039/C8NH00366A
41. [41]
  C. Muthu, S. Agarwal, A. Vijayan, et al., Adv. Mater. Interfaces 3 (2016) 1600092. doi: 10.1002/admi.201600092
42. [42]
  L. Liang, K. Li, C. Xiao, et al., J. Am. Chem. Soc. 137 (2015) 3102–3108. doi: 10.1021/jacs.5b00021
43. [43]
  X. Zhang, J. Xu, X. Zhang, et al., Mater. Sci. Semicond. Process 57 (2017) 105–109. doi: 10.1016/j.mssp.2016.09.031
44. [44]
  H.T. Wu, Y.F. Chen, C.F. Shih, et al., Thin Solid Films 660 (2018) 320–327. doi: 10.1016/j.tsf.2018.06.032
45. [45]
  J. Lian, Q. Wang, Y. Yuan, et al., J. Mater. Chem. A 3 (2015) 9146–9151. doi: 10.1039/C5TA01595B
46. [46]
  V.M. Le Corre, E.A. Duijnstee, O. El Tambouli, et al., ACS Energy Lett. 6 (2021) 1087–1094. doi: 10.1021/acsenergylett.0c02599
47. [47]
  S. Sourisseau, N. Louvain, W. Bi, et al., Chem. Mater. 19 (2007) 600–607. doi: 10.1021/cm062380e
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