Citation: Ye Zhu, Yongheng Zhu, Jiaqiang Xu. Fabrication of high sensitivity 2-PEA sensor based on Aldehyde-functionalized mesoporous carbon[J]. Chinese Chemical Letters, ;2023, 34(1): 107391. doi: 10.1016/j.cclet.2022.03.114 shu

Fabrication of high sensitivity 2-PEA sensor based on Aldehyde-functionalized mesoporous carbon

Ye Zhu ^a ,
Yongheng Zhu ^{c, *,} ,
Jiaqiang Xu ^{b, *,}

a.
Department of Stomatology, Huashan Hospital Affiliated to Fudan University, Shanghai 200040, China
b.
Department of Physics & Department of Chemistry, College of Science, Shanghai University, Shanghai 200444, China
c.
College of Food Science & Technology, Shanghai Ocean University, Shanghai 213064, China

yh-zhu@shou.edu.cn

xujiaqiang@shu.edu.cn

Received Date: 18 November 2021
Revised Date: 21 February 2022
Accepted Date: 30 March 2022
Available Online: 2 April 2022

Figures(4)

2-Phenylethylamine (2-PEA) is one of the main ingredients for stimulants. Therefore, it is necessary to limit its use and illegal trade by conveniently detecting 2-PEA vapour. Here, a QCM based 2-PEA gas sensor was constructed by using aldehyde functionalized mesoporous carbon (FDU-15-CHO) as sensing materials designed according to Schiff base adsorption role. The 2D hexagonal mesoporous structures of the sensing material have been confirmed by small-angle X-ray diffraction (SXRD), transmission electron microscopy (TEM), and N₂ adsorption-desorption isotherms. The covalent grafting of aldehyde group onto the FDU-15 was confirmed by Fourier transform infrared spectroscopy (FT-IR). FDU-15-CHO based Quartz Crystal Microbalance (QCM) sensor shows better sensitivity to 2-PEA than its parent FDU-15. Besides, the detection limit of FDU-15-CHO based sensor can reach down to 1 ppm, and its selectivity and reproducibility are satisfactory. The high concentrations of active sites in the mesopores of FDU-15 are believed to facilitate 2-PEA adsorption, and thus the presence of the -CHO group leading to sensitive and selective response, which is verified by Gaussian simulation
- Quartz crystal microbalance (QCM),
- 2-Phenylethylamine,
- FDU-15-CHO,
- Gas sensor,
- Gaussian software
1. [1]
  T.A. Branchek, T.P. Blackburn, Curr. Opin. Pharmacol. 3 (2003) 90–97. doi: 10.1016/S1471-4892(02)00028-0
2. [2]
  A. Bouchet, M. Schütz, B. Chiavarino, et al., Phys. Chem. Chem. Phys. 17 (2015) 25742–25754. doi: 10.1039/C5CP00221D
3. [3]
  D.W. Arrigan, M. Ghita, V. Beni, Chem. Commun. (2004) 732–733.
4. [4]
  W. Fischer, R.H. Neubert, M. Brandsch, Eur. J. Pharm. Biopharm. 74 (2010) 281–289. doi: 10.1016/j.ejpb.2009.11.014
5. [5]
  V. Beni, M. Ghita, D.W. Arrigan, Biosens. Bioelectron. 20 (2005) 2097–2103. doi: 10.1016/j.bios.2004.08.004
6. [6]
  A. Berduque, R. Zazpe, D.W. Arrigan, Anal. Chim. Acta 611 (2008) 156–162. doi: 10.1016/j.aca.2008.01.077
7. [7]
  O. Dvorák, V. Mareček, Z. Samec, et al., J. Electroanal. Chem. 300 (1991) 407–413. doi: 10.1016/0022-0728(91)85407-G
8. [8]
  G. Herzog, B. McMahon, M. Lefoix, et al., J. Electroanal. Chem. 622 (2008) 109–114. doi: 10.1016/j.jelechem.2008.05.006
9. [9]
  B.A. Davis, A.A. Boulton, Prog. Neuro. Psychoph. 18 (1994) 17–45. doi: 10.1016/0278-5846(94)90022-1
10. [10]
  A.H. Lewin, Aaps J. 8 (2006) E138–E145. doi: 10.1208/aapsj080116
11. [11]
  N.E. Andén, H. Corrodi, K. Fuxe, et al., Eur. J. Pharmacol. 25 (1974) 176–184. doi: 10.1016/0014-2999(74)90047-8
12. [12]
  S. Amrehn, X. Wu, T. Wagner, ACS Sensor 3 (2018) 191–199. doi: 10.1021/acssensors.7b00845
13. [13]
  H. Tian, H. Fan, M. Li, et al., ACS Sensor 1 (2016) 243–250. doi: 10.1021/acssensors.5b00236
14. [14]
  J. Yu, X. Qin, X. Xian, et al., ACS Sensor 3 (2018) 160–166. doi: 10.1021/acssensors.7b00790
15. [15]
  H. Peng, C. Liang, A. Zhou, et al., Anal. Chim. Acta 423 (2000) 221–228. doi: 10.1016/S0003-2670(00)01104-1
16. [16]
  M. Rapp, J. Reibel, A. Voigt, et al., Sensor. Actuat. B: Chem. 65 (2000) 169–172. doi: 10.1016/S0925-4005(99)00321-4
17. [17]
  F.S. Coulibaly, B.B. C. Youan, Biosens. Bioelectron. 59 (2014) 404–411. doi: 10.1016/j.bios.2014.03.040
18. [18]
  H. Li, Q. Zheng, J. Luo, et al., Sensor. Actuat. B: Chem. 187 (2013) 604–610. doi: 10.1016/j.snb.2013.04.122
19. [19]
  Y. Zhu L. Wang, Q. Xiang, et al., Sensor. Actuat. B: Chem. 251 (2017) 590–600. doi: 10.1016/j.snb.2017.05.074
20. [20]
  S.N. Faisal, C.M. Pereira, S. Rho, et al., Phys. Chem. Chem. Phys. 12 (2010) 15184–15189. doi: 10.1039/c0cp00750a
21. [21]
  S. Cui, H. Pu, G. Lu, et al., ACS Appl. Mater. Inter. 4 (2012) 4898–4904. doi: 10.1021/am301229w
22. [22]
  J. Lee, S. Yoon, T. Hyeon, et al., Chem. Commun. 13 (1999) 2177–2178.
23. [23]
  C. Liang, Z. Li, S. Dai, Chem. Int. 47 (2008) 3696–3717. doi: 10.1002/anie.200702046
24. [24]
  J.C. Ndamanisha, J. Bai, B. Qi, et al., Anal. Biochem. 386 (2009) 79–84. doi: 10.1016/j.ab.2008.11.041
25. [25]
  X. Bo, J. Bai, L. Yang, et al., Sensor. Actuat. B: Chem. 157 (2011) 662–668. doi: 10.1016/j.snb.2011.05.050
26. [26]
  A. Molina, E. Torralba, C. Serna, et al., Electrochim. Acta 106 (2013) 244–257. doi: 10.1016/j.electacta.2013.05.080
27. [27]
  Z. Wu, Y. Yang, B. Tu, et al., Adsorption 15 (2009) 123–132. doi: 10.1007/s10450-009-9159-8
28. [28]
  D.H. Lin, Y.X. Jiang, S.R. Chen, et al., Electrochim. Acta 67 (2012) 127–132. doi: 10.1016/j.electacta.2012.02.007
29. [29]
  H. Li, S. Zhu, Z. Wen, et al., Micropor. Mesopor. Mat. 96 (2006) 357–362. doi: 10.1016/j.micromeso.2006.07.021
30. [30]
  P. Xu, H. Yu, S. Guo, et al., Anal. Chem. 86 (2014) 4178–4187. doi: 10.1021/ac403498x
1. [1]
  Yu Deng , Yan Liu , Yonghui Deng , Jinsheng Cheng , Yidong Zou , Wei Luo . In situ sulfur-doped mesoporous tungsten oxides for gas sensing toward benzene series. Chinese Chemical Letters, 2024, 35(7): 108898-. doi: 10.1016/j.cclet.2023.108898
2. [2]
  Ling Fan , Meili Pang , Yeyun Zhang , Yanmei Wang , Zhenfeng Shang . Quantum Chemistry Calculation Research on the Diels-Alder Reaction of Anthracene and Maleic Anhydride: Introduction to a Computational Chemistry Experiment. University Chemistry, 2024, 39(4): 133-139. doi: 10.3866/PKU.DXHX202309024
3. [3]
  Tingbo Wang , Yao Luo , Bingyan Hu , Ruiyuan Liu , Jing Miao , Huizhe Lu . Quantitative Computational Study on the Claisen Rearrangement Reaction of Allyl Phenyl Ethers: An Introduction to a Computational Chemistry Experiment. University Chemistry, 2024, 39(11): 278-285. doi: 10.12461/PKU.DXHX202403082
4. [4]
  Shuanglin TIAN , Tinghong GAO , Yutao LIU , Qian CHEN , Quan XIE , Qingquan XIAO , Yongchao LIANG . First-principles study of adsorption of Cl₂ and CO gas molecules by transition metal-doped g-GaN. Chinese Journal of Inorganic Chemistry, 2024, 40(6): 1189-1200. doi: 10.11862/CJIC.20230482
5. [5]
  Xueling Yu , Lixing Fu , Tong Wang , Zhixin Liu , Na Niu , Ligang Chen . Multivariate chemical analysis: From sensors to sensor arrays. Chinese Chemical Letters, 2024, 35(7): 109167-. doi: 10.1016/j.cclet.2023.109167
6. [6]
  Xiaoyan Peng , Xuanhao Wu , Fan Yang , Yefei Tian , Mingming Zhang , Hongye Yuan . Gas sensors based on metal-organic frameworks: challenges and opportunities. Chinese Journal of Structural Chemistry, 2024, 43(3): 100251-100251. doi: 10.1016/j.cjsc.2024.100251
7. [7]
  Hongxia Li , Xiyang Wang , Du Qiao , Jiahao Li , Weiping Zhu , Honglin Li . Mechanism of nanoparticle aggregation in gas-liquid microfluidic mixing. Chinese Chemical Letters, 2024, 35(4): 108747-. doi: 10.1016/j.cclet.2023.108747
8. [8]
  Jie Ma , Jianxiang Wang , Jianhua Yuan , Xiao Liu , Yun Yang , Fei Yu . The regulating strategy of hierarchical structure and acidity in zeolites and application of gas adsorption: A review. Chinese Chemical Letters, 2024, 35(11): 109693-. doi: 10.1016/j.cclet.2024.109693
9. [9]
  Tian Cao , Xuyin Ding , Qiwen Peng , Min Zhang , Guoyue Shi . Intelligent laser-induced graphene sensor for multiplex probing catechol isomers. Chinese Chemical Letters, 2024, 35(7): 109238-. doi: 10.1016/j.cclet.2023.109238
10. [10]
  Neng Shi , Haonan Jia , Jixiang Zhang , Pengyu Lu , Chenglong Cai , Yixin Zhang , Liqiang Zhang , Nongyue He , Weiran Zhu , Yan Cai , Zhangqi Feng , Ting Wang . Accurate expression of neck motion signal by piezoelectric sensor data analysis. Chinese Chemical Letters, 2024, 35(9): 109302-. doi: 10.1016/j.cclet.2023.109302
11. [11]
  Chenlu Huang , Xinyu Yang , Qingyu Yu , Linhua Zhang , Dunwan Zhu . Gas-generating polymersomes-based amplified photoimmunotherapy for abscopal effect and tumor metastasis inhibition. Chinese Chemical Letters, 2024, 35(6): 109680-. doi: 10.1016/j.cclet.2024.109680
12. [12]
  Haoyang Wang , Ronghao Zhang , Yanlun Ren , Li Zhang . A convenient method for measuring gas-liquid volumetric mass transfer coefficient in micro reactors. Chinese Chemical Letters, 2024, 35(4): 108833-. doi: 10.1016/j.cclet.2023.108833
13. [13]
  Jichun Li , Zhengren Wang , Yu Deng , Hongxiu Yu , Yonghui Deng , Xiaowei Cheng , Kaiping Yuan . Construction of mesoporous silica-implanted tungsten oxides for selective acetone gas sensing. Chinese Chemical Letters, 2024, 35(11): 110111-. doi: 10.1016/j.cclet.2024.110111
14. [14]
  Zhijia Zhang , Shihao Sun , Yuefang Chen , Yanhao Wei , Mengmeng Zhang , Chunsheng Li , Yan Sun , Shaofei Zhang , Yong Jiang . Epitaxial growth of Cu_2-xSe on Cu (220) crystal plane as high property anode for sodium storage. Chinese Chemical Letters, 2024, 35(7): 108922-. doi: 10.1016/j.cclet.2023.108922
15. [15]
  Weiping Guo , Ying Zhu , Hong-Hua Cui , Lingyun Li , Yan Yu , Zhong-Zhen Luo , Zhigang Zou . β-Pb₃P₂S₈: A new optical crystal with exceptional birefringence effect. Chinese Chemical Letters, 2025, 36(2): 110256-. doi: 10.1016/j.cclet.2024.110256
16. [16]
  Zhenghua ZHAO , Qin ZHANG , Yufeng LIU , Zifa SHI , Jinzhong GU . Syntheses, crystal structures, catalytic and anti-wear properties of nickel(Ⅱ) and zinc(Ⅱ) coordination polymers based on 5-(2-carboxyphenyl)nicotinic acid. Chinese Journal of Inorganic Chemistry, 2024, 40(3): 621-628. doi: 10.11862/CJIC.20230342
17. [17]
  Lu LIU , Huijie WANG , Haitong WANG , Ying LI . Crystal structure of a two-dimensional Cd(Ⅱ) complex and its fluorescence recognition of p-nitrophenol, tetracycline, 2, 6-dichloro-4-nitroaniline. Chinese Journal of Inorganic Chemistry, 2024, 40(6): 1180-1188. doi: 10.11862/CJIC.20230489
18. [18]
  Ying Chen , Li Li , Junyao Zhang , Tongrui Sun , Xuan Zhang , Shiqi Zhang , Jia Huang , Yidong Zou . Tailored ionically conductive graphene oxide-encased metal ions for ultrasensitive cadaverine sensor. Chinese Chemical Letters, 2024, 35(8): 109102-. doi: 10.1016/j.cclet.2023.109102
19. [19]
  Ting WANG , Peipei ZHANG , Shuqin LIU , Ruihong WANG , Jianjun ZHANG . A Bi-CP-based solid-state thin-film sensor: Preparation and luminescence sensing for bioamine vapors. Chinese Journal of Inorganic Chemistry, 2024, 40(8): 1615-1621. doi: 10.11862/CJIC.20240134
20. [20]
  Xiangshuai Li , Jian Zhao , Li Luo , Zhuohao Jiao , Ying Shi , Shengli Hou , Bin Zhao . Visual and portable detection of metronidazole realized by metal-organic framework flexible sensor and smartphone scanning. Chinese Chemical Letters, 2024, 35(10): 109407-. doi: 10.1016/j.cclet.2023.109407

Get Citation

PDF

XML

Metrics

PDF Downloads(3)
Abstract views(954)
HTML views(70)

通讯作者: 陈斌, bchen63@163.com

1.
沈阳化工大学材料科学与工程学院沈阳 110142