Citation: Xu Han, Jialin Tong, Guanyu Ding, Chunyi Sun, Xinlong Wang, Zhongmin Su, Jing Sun, Li-Li Wen, Guo-Gang Shan. Highly emissive coordination polymer derived from tetraphenylethylene-tetrazole chromophore: Synthesis, characterization and piezochromic luminescent behavior[J]. Chinese Chemical Letters, ;2023, 34(1): 107255. doi: 10.1016/j.cclet.2022.02.060 shu

Highly emissive coordination polymer derived from tetraphenylethylene-tetrazole chromophore: Synthesis, characterization and piezochromic luminescent behavior

Xu Han ^a ,
Jialin Tong ^b ,
Guanyu Ding ^a ,
Chunyi Sun ^b ,
Xinlong Wang ^b ,
Zhongmin Su ^{a, *,} ,
Jing Sun ^a ,
Li-Li Wen ^{a, *,} ,
Guo-Gang Shan ^{b, *,}

a.
School of Chemical and Environmental Engineering, Changchun University of Science and Technology, Changchun 130022, China
b.
National & Local United Engineering Laboratory for Power Batteries, Key Laboratory of Polyoxometalate Science of Ministry of Education, Department of Chemistry, Northeast Normal University, Changchun 130024, China

zmsu@nenu.edu.cn

wll@cust.edu.cn

hhzhoushangg187@nenu.edu.cn

Received Date: 9 January 2022
Revised Date: 9 February 2022
Accepted Date: 21 February 2022
Available Online: 24 February 2022

Figures(4)

Solid-state materials that exhibit pressure stimulus-response characteristics in a manner of emission signal, known as piezochromic luminescence (PCL), demonstrate great potential in photoelectric devices. The weakened luminescence and insignificant color change in the aggregation state, however, hampers their practical applications. Herein, a highly emissive coordination polymer, [Zn₂(H₄TTPE)(H₂O)₄]·H₂O (CUST-805), is successfully constructed by employing an AIE-active chromophore as the building block. The structural characterization and photophysical properties are systematically studied. Owing to intrinsic twisted conformation and AIE feature of tetraphenylethylene-tetrazole ligand, CUST-805 achieves the visible and reversible PCL from blue to green switched by different external stimuli. The transformation between crystalline and amorphous states is proved to be the origin of present PCL behavior. Moreover, on basis of electron and energy transfer quenching mechanism, the highly selective and sensitive sensor based on CUST-805 is realized, showing the low detection limit of 0.29 ppm towards 2, 4, 6-trinitrophenol.
- Coordination polymer,
- Piezochromic luminescence,
- Aggregation-induced emission,
- Stimulus-response,
- Sensing
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