Citation: Mamitiana Roger Razanajatovo, Wenyan Gao, Yaran Song, Xuan Zhao, Qina Sun, Qingrui Zhang. Selective adsorption of phosphate in water using lanthanum-based nanomaterials: A critical review[J]. Chinese Chemical Letters, ;2021, 32(9): 2637-2647. doi: 10.1016/j.cclet.2021.01.046 shu

Selective adsorption of phosphate in water using lanthanum-based nanomaterials: A critical review

Mamitiana Roger Razanajatovo ^a ,
Wenyan Gao ^a ,
Yaran Song ^{a, *,} ,
Xuan Zhao ^a ,
Qina Sun ^a ,
Qingrui Zhang ^{a, b, *,}

a.
Hebei Key Laboratory of Heavy Metal Deep-Remediation in Water and Resource Reuse, and the Laboratory of Applied Chemistry, Yanshan University, Qinhuangdao 066004, China
b.
State Key Laboratory of Metastable Materials Science and Technology, Yanshan University, Qinhuangdao 066004, China

songyr@ysu.edu.cn

zhangqr@ysu.edu.cn

Received Date: 17 November 2020
Revised Date: 16 December 2020
Accepted Date: 12 January 2021
Available Online: 2 February 2021

Figures(8)

In recent years, lanthanum-based nanomaterials (La-NMs) are selected as an efficient nano-adsorbent for phosphate removal because La³⁺ has a strong affinity with oxygen-donor atoms from phosphate. Additionally, there are a broad interest and literature base for the effect of different synthesis optimization and environmental parameters on the adsorption performance of La-NMs. A considerable amount of research has also investigated the regeneration and application of La-NMs to real wastewater in a laboratory scale. Based on the literature survey, it was found that La-NMs are often produced via co-precipitation and hydrothermal methods. Moreover, phosphate's adsorption process and behavior onto La-NMs are described well with the pseudo-second-order model and Langmuir model. The interaction mechanism between phosphate and La-NMs are dominated by ligand exchange, surface complexation and electrostatic attraction. Furthermore, phosphate could easily desorb from La-NMs due to the weak H-bonding interaction between phosphate and the H-bond acceptor groups on the surface of La-NMs. Despite the wealth of literature available in this area, there is a lack of systematic review to evaluate the gaps in the use of La-NMs to eliminate phosphate in water. In this review, we mainly summarize and discuss the role and the effect of the synthesis techniques on the physicochemical properties and the adsorption behavior of La-NMs. The possible adsorption mechanism, regeneration efficiency, and the application of La-NMs to the real environmental samples are also presented and highlighted.
- Lanthanum-nanomaterials,
- Synthesis,
- Phosphate,
- Adsorption mechanism,
- Regeneration,
- Application
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沈阳化工大学材料科学与工程学院沈阳 110142