Citation: Hui Hu, Dashuai Zhang, Huiling Liu, Yaoqiang Jin, Jun Gao, Yongzheng Zhang, Zhongmin Liu, Xiuling Zhang, Longlong Geng, Suijun Liu, Ranhui Zhang. Two isostructural Ni(Ⅱ)/Co(Ⅱ)-based metal-organic frameworks for selective dye adsorption and catalytic cycloaddition of CO₂ with epoxides[J]. Chinese Chemical Letters, ;2021, 32(1): 557-560. doi: 10.1016/j.cclet.2020.02.028 shu

Two isostructural Ni(Ⅱ)/Co(Ⅱ)-based metal-organic frameworks for selective dye adsorption and catalytic cycloaddition of CO₂ with epoxides

Hui Hu ^{a, 1} ,
Dashuai Zhang ^{a, 1} ,
Huiling Liu ^a ,
Yaoqiang Jin ^{a, c} ,
Jun Gao ^d ,
Yongzheng Zhang ^a ,
Zhongmin Liu ^a ,
Xiuling Zhang ^{a, c, **,} ,
Longlong Geng ^{a, **,} ,
Suijun Liu ^{b, *,} ,
Ranhui Zhang ^{a, c}

a.
College of Chemistry and Chemical Engineering, Dezhou University, Dezhou 253023, China
b.
School of Chemistry and Chemical Engineering, Jiangxi University of Science and Technology, Ganzhou 341000, China
c.
College of Chemical Engineering, Qingdao University of Science and Technology, Qingdao 266000, China
d.
College of Chemical and Environmental Engineering, Shandong University of Science and Technology, Qingdao 266590, China

^**

xlzhang99@126.com

llgeng@126.com

sjliu@jxust.edu.cn

Received Date: 10 February 2020
Revised Date: 12 February 2020
Accepted Date: 12 February 2020
Available Online: 14 February 2020

Figures(3)

Two isostructural Ni(Ⅱ)/Co(Ⅱ)-based metal-organic frameworks (MOFs), namely {[M₃(L)₂(bpb)₃(H₂O)₄]·2DMF·2H₂O}_n [M = Ni (HL-5, HL is short for Hui-Ling Liu); M = Co (HL-6); H₃L = 2', 6'-dimethyl-[1, 1'-biphenyl]-3, 4', 5-tricarboxylic acid; bpb = 1, 4-bis(pyrid-4-yl)benzene], have been hydrothermally syn-thesized and structurally characterized. Both HL-5 and HL-6, which have the same three-interpenetrated 3D pillared-layer framework with sqc306 type topology, present good selective methyl orange (MO) adsorption over rhodamine B (RhB). Moreover, the catalytic CO₂ cycloaddition properties with epoxides of the two MOFs have also been studied at ambient pressure and temperature.
- Metal-organic frameworks,
- Dye separation,
- Heterogeneous catalysis,
- CO₂ cycloaddition,
- Coordination polymers
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Two isostructural Ni(Ⅱ)/Co(Ⅱ)-based metal-organic frameworks for selective dye adsorption and catalytic cycloaddition of CO2 with epoxides

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通讯作者: 陈斌, bchen63@163.com

Two isostructural Ni(Ⅱ)/Co(Ⅱ)-based metal-organic frameworks for selective dye adsorption and catalytic cycloaddition of CO₂ with epoxides