Citation: Liu Xiaobang, Yue Ting, Qi Kai, Qiu Yubing, Xia Bao Yu, Guo Xingpeng. Metal-organic framework membranes: From synthesis to electrocatalytic applications[J]. Chinese Chemical Letters, ;2020, 31(9): 2189-2201. doi: 10.1016/j.cclet.2019.12.009 shu

Metal-organic framework membranes: From synthesis to electrocatalytic applications

Liu Xiaobang ^a ,
Yue Ting ^a ,
Qi Kai ^a,*, ,
Qiu Yubing ^a ,
Xia Bao Yu ^a,*, ,
Guo Xingpeng ^b

a.
Key Laboratory of Material Chemistry for Energy Conversion and Storage(Ministry of Education), Hubei Key Laboratory of Material Chemistry and Service Failure, School of Chemistry and Chemical Engineering, Huazhong University of Science and Technology(HUST), Wuhan 430074, China
b.
School of Chemistry and Chemical Engineering, Guangzhou University, Guangzhou 510006, China

qikai@hust.edu.cn

byxia@hust.edu.cn

Received Date: 30 September 2019
Revised Date: 31 October 2019
Accepted Date: 2 December 2019
Available Online: 5 December 2019

Figures(10)

Metal-organic frameworks (MOFs), as an emerging family of porous inorganic-organic crystal materials, exhibit widely applications in gas storage and separation, drug release, sensing, and catalysis, owing to easily adjustable pore sizes, uniformly distributed metal centers, high surface areas, and tunable functionalities. However, MOF crystal powders are usually difficult to be directly applied into specific devices because of their brittleness, insolubility and low compatibility. Therefore, to expand versatile MOF membranes with robustness and operational flexibility is urgent to satisfy practical applications. Although numerous reports have reviewed the synthesis and applications of MOF membranes, relatively few reports the electrocatalytic properties based on MOF membranes. Herein, this mini-review provides an overview of preparation of MOF membranes, including directed synthesis, secondary growth and electrochemical deposition method. Meanwhile, fabrication of ultrathin 2D MOF nanosheets those can be also defined as a kind of nanoscale MOF membranes is also mentioned. Electrocatalytic performance of oxygen reduction reaction (ORR), oxygen evolution reaction (OER), hydrogen evolution reaction (HER) and CO₂ reduction reaction (CO₂RR) for diverse MOF membranes/nanosheets and their derivatives are introduced.
- Metal-organic frameworks,
- Membranes,
- Nanosheets,
- Derivatives,
- Synthesis,
- Electrocatalysis
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