Citation: Liu Zengjie, Wu Jiarui, Wang Chunyu, Yang Jie, Wang Yan, Yang Ying-Wei. Stimuli-responsive fluorescent supramolecular polymer network based on a monofunctionalized leaning tower[6]arene[J]. Chinese Chemical Letters, ;2019, 30(12): 2299-2303. doi: 10.1016/j.cclet.2019.10.023 shu

Stimuli-responsive fluorescent supramolecular polymer network based on a monofunctionalized leaning tower[6]arene

Liu Zengjie ^a ,
Wu Jiarui ^a ,
Wang Chunyu ³ ,
Yang Jie ^a ,
Wang Yan ^a,*, ,
Yang Ying-Wei ^a,b,d,*,

a.
State Key Laboratory of Inorganic Synthesis and Preparative Chemistry, International Joint Research Laboratory of Nano-Micro Architecture Chemistry, NMAC, College of Chemistry, Jilin University, Changchun, China
b.
The State Key Laboratory of Refractories and Metallurgy, School of Chemistry and Chemical Engineering, Wuhan University of Science and Technology, Wuhan, China
c.
State Key Laboratory of Supramolecular Structure and Materials, Institute of Theoretical Chemistry, Jilin University, Changchun, China
d.
California NanoSystems Institute and Department of Chemistry, Biochemistry, University of California, Los Angeles, CA, United States

wangy2011@jlu.edu.cn

ywyang@jlu.edu

Received Date: 26 September 2019
Revised Date: 14 October 2019
Accepted Date: 18 October 2019
Available Online: 24 December 2019

Figures(6)

A fluorescent supramolecular polymer network with an excellent triple-stimuli responsive property based on metal-ligand coordination and host-guest interactions has been constructed from a terpyridine-monofunctionalized leaning tower[6]arene, a tetraphenylethylene AIEgen, and a bridging coordination ion (Zn²⁺). Addition of competitive binding agents, trifluoroacetic acid, and/or pillar[5]arene can break the metal coordination and/or host-guest inclusion complexation, and thermal heating can weaken the non-covalent interactions in the supramolecular polymer gel, all leading to the gel-to-sol transition.
- Aggregation-induced emission,
- Coordination,
- Leaning tower[n]arene,
- Stimuli-responsive materials,
- Supramolecular polymer
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