Citation: Liu Na, Shi Liangfeng, Han Xianghao, Qi Qiao-Yan, Wu Zong-Quan, Zhao Xin. A heteropore covalent organic framework for adsorptive removal of Cd(Ⅱ) from aqueous solutions with high efficiency[J]. Chinese Chemical Letters, ;2020, 31(2): 386-390. doi: 10.1016/j.cclet.2019.06.050 shu

A heteropore covalent organic framework for adsorptive removal of Cd(Ⅱ) from aqueous solutions with high efficiency

Liu Na ^a ,
Shi Liangfeng ^a,b,1 ,
Han Xianghao ^b,1 ,
Qi Qiao-Yan ^b ,
Wu Zong-Quan ^a,*, ,
Zhao Xin ^b,*,

a.
Department of Polymer Science and Engineering, School of Chemistry and Chemical Engineering, and Anhui Key Laboratory of Advanced Catalytic Materials and Reaction Engineering, Hefei University of Technology, Hefei 230009, China
b.
CAS Key Laboratory of Synthetic and Self-Assembly Chemistry for Organic Functional Molecules, Center for Excellence in Molecular Synthesis, Shanghai Institute of Organic Chemistry, Chinese Academy of Sciences, Shanghai 200032, China

zqwu@hfut.edu.cn

xzhao@sioc.ac.cn

Received Date: 7 May 2019
Revised Date: 18 June 2019
Accepted Date: 27 June 2019
Available Online: 27 June 2019

Figures(5)

A heteropore covalent organic framework (COF) integrating tetraphenylethene skeleton and catechol segment is designed and synthesized. It exhibits extremely high stability in water under different pH conditions, which makes it an excellent material for adsorptive removal of Cd(Ⅱ) from aqueous solutions with very fast adsorption kinetics, high uptake capacity, and good recyclability.
- Covalent organic frameworks,
- Heteropore,
- Hierarchical porosity,
- Cd(Ⅱ) removal,
- Water treatment
1. [1]
  (a) R.P. Schwarzenbach, B.I. Escher, K. Fenner, et al., Science 313 (2006) 1072-1077;
  (b) M.P. Waalkes, J. Inorg, Biochem. 79 (2000) 241-244;
  (c) M. Hua, S. Zhang, B. Pan, et al., J. Hazard. Mater. 211-212 (2012) 317-331;
  (d) P. Miretzky, A.F. Cirelli, J. Hazard. Mater. 167 (2009) 10-23;
  (e) M.T. Hayat, M. Nauman, N. Nazir, S.Ali N. Bangash, Environmental hazards of cadmium: past, present, and future, in: M. Hasanuzzaman, M.N.V. Prasad, M. Fujita (Eds.), Cadmium Toxicity and Tolerance in Plants, Academic Press, New York, 2019, pp. 163-183;
  (f) H. Liu, G. Liu, Z. Yuan, et al., Mar. Pollut. Bull. 140 (2019) 388-394;
  (g) P.K. Samantaray, S. Baloda, G. Madras, S. Bose, J. Mater. Chem. A 6 (2018) 16664-16679.
2. [2]
  (a) H. Yamada, T. Miyahara, Y. Sasaki, Mutat. Res. Lett. 302 (1993) 137-145;
  (b) I.A. Darwish, D.A. Blake, Anal. Chem. 73 (2001) 1889-1895;
  (c) K. Nogawa, E. Kobayashi, Y. Okubo, Y. Suwazono, Biometals 17 (2004) 581-587;
  (d) S. Khan, Q. Cao, Y.M. Zheng, Y.Z. Huang, Y.G. Zhu, Environ. Pollut. 152 (2008) 686-692;
  (e) R. Zha, R. Nadimicherla, X. Guo, J. Mater. Chem A 2 (2014) 13932-13941.
3. [3]
  (a) S. Rodrigues, N. Munichandraiah, A.K. Shukla, J. Power Sources 87 (2000) 12-20;
  (b) S. Ghatak, G. Chakraborty, M. Sinha, S.K. Pradhan, A.K. Meikap, Physica B 406 (2011) 3261-3266.
4. [4]
  (a) C. Zhu, Y. Guo, Y. Yang, et al., J. Environ. Eng. Technol. 8 (2018) 58-64;
  (b) Y. Lan, R. Liang, X. Zhao, et al., Acta Sci. Circumstantiae 37 (2017) 3602-3612.
5. [5]
  (a) A. Özverdi, M. Erdem, J. Hazard. Mater. B 137 (2006) 626-632;
  (b) J. Koelmel, M.N.V. Prasad, G. Velvizhi, S.K. Butti, S.V. Mohan, Metalliferous waste in India and knowledge explosion in metal recovery techniques and processes for the prevention of pollution, in: M.N.V. Prasad, K. Shih (Eds.), Environmental Materials and Waste, Academic Press, New York, 2016, pp. 339-390;
  (c) D. Purkayastha, U. Mishra, S. Biswas, J. Water Process. Eng. 2 (2014) 105-128;
  (d) F. Fu, Q. Wang, J. Environ. Manag. 92 (2011) 407-418.
6. [6]
  (a) J. Shao, J.D. Gu, L. Peng, et al., J. Hazard. Mater. 272 (2014) 83-88;
  (b) M.Q. Jiang, X.Y. Jin, X.Q. Lu, Z.L. Chen, Desalination 252 (2010) 33-39;
  (c) P. Pavasant, R. Apiratikul, V. Sungkhum, et al., Bioresour. Technol. 97 (2006) 2321-2329;
  (d) Z. Feng, S. Zhu, D.R. Martins de Godoi, A.C.S. Samia, D. Scherson, Anal. Chem. 84 (2012) 3764-3770.
7. [7]
  (a) E. Samper, M. Rodríguez, M.A. De la Rubia, D. Prats, Sep. Purif. Technol. 65 (2009) 337-342;
  (b)J.H. Huang, G.M. Zeng, C.F. Zhou, et al., J.Hazard.Mater.183 (2010) 287-293;
  (c) D.J. Ennigrou, L. Gzara, M.R. Ben Romdhane, M. Dhahbi, Desalination 246 (2009) 363-369.
8. [8]
  (a) L.E. Kanagy, B.M. Johnson, J.W. Castle, J.H. Rodgers Jr., Bioresour. Technol. 99 (2008) 1877-1885;
  (b) H.A. Qdais, H. Moussa, Desalination 164 (2004) 105-110.
9. [9]
  (a) A. Üçer, A. Uyanik, Ş.F. Aygün, Sep. Purif. Technol. 47 (2006) 113-118;
  (b) B.E.Reed, S.Arunachalam, B.Thomas, Environ.Prog.Sustain. 13 (1994)60-64;
  (c) B. Xiao, K.M. Thomas, Langmuir 21 (2005) 3892-3902.
10. [10]
  (a) J.L. Weidman, R.A. Mulvenna, B.W. Boudouris, W.A. Phillip, ACS Appl. Mater. Interfaces 9 (2017) 19152-19160;
  (b) M.X. Tan, Y.N. Sum, J.Y. Ying, Y. Zhang, EnergyEnviron. Sci. 6 (2013) 3254-3259;
  (c) H. Zhu, X. Tan, L. Tan, et al., ACS Sustain. Chem. Eng. 6 (2018) 5206-5213.
11. [11]
  (a) Y. Wang, G. Ye, H. Chen, et al., J. Mater. Chem. A 3 (2015) 15292-15298;
  (b) J. Zhang, Z. Xiong, C. Li, C. Wu, J. Mol. Liq. 221 (2016) 43-50;
  (c) C. Liu, P. Wang, X. Liu, et al., Chem. -Asian J. 14 (2019) 261-268;
  (d) J. Li, X. Wang, G. Zhao, et al., Chem. Soc. Rev. 47 (2018) 2322-2356.
12. [12]
  (a) A.P. Côté, A.I. Benin, N.W. Ockwig, M. O'Keeffe, A.J. Matzger, O.M. Yaghi, Science 310 (2005) 1166-1170;
  (b) S.Y. Ding, W. Wang, Chem. Soc. Rev. 42 (2013) 548-568;
  (c) P.J. Waller, F. Gándara, O.M. Yaghi, Acc. Chem. Res. 48 (2015) 3053-3063;
  (d) S.Kandambeth, K. Dey, R. Banerjee, J.Am. Chem. Soc.141 (2019) 1807-1822.
13. [13]
  (a) M.S. Lohse, T. Bein, Adv. Funct. Mater. 28 (2018) 1705553;
  (b) Y. Song, Q. Sun, B. Aguila, S. Ma, Adv. Sci. 6 (2019) 1801410;
  (c) N. Huang, P. Wang, D. Jiang, Nat. Rev. Mater. 1 (2016) 16068;
  (d) M.X. Wu, Y.W. Yang, Chin. Chem. Lett. 28 (2017) 1135-1143.
14. [14]
  (a) S.Y. Ding, M. Dong, Y.W. Wang, et al., J. Am. Chem. Soc. 138 (2016) 3031-3037;
  (b) N. Huang, L. Zhai, H. Xu, D. Jiang, J. Am. Chem. Soc. 139 (2017) 2428-2434;
  (c) Q. Sun, B. Aguila, J. Perman, et al., J. Am. Chem. Soc.139 (2017) 2786-2793;
  (d) K. Leus, K. Folens, N.R. Nicomel, et al., J. Hazard. Mater. 353 (2018) 312-319;
  (e) Q. Lu, Y. Ma, H. Li, et al., Angew. Chem. Int. Ed. 57 (2018) 6042-6048;
  (f) Z.A. Ghazi, A.M. Khattak, R. Iqbal, et al., New J. Chem. 42 (2018) 10234-10242;
  (g) F.Z. Cui, R.R. Liang, Q.Y. Qi, G.F. Jiang, X. Zhao, Adv. Sustain. Syst. (2019) 1800150.
15. [15]
  (a) X.Y. Yang, L.H. Chen, Y. Li, et al., Chem. Soc. Rev. 46 (2017) 481-558;
  (b) S. Lopez-Orozco, A. Inayat, A. Schwab, T. Selvam, W. Schwieger, Adv. Mater. 23 (2011) 2602-2615;
  (c) Y. Li, Z.Y. Fu, B.L. Su, Adv. Funct. Mater. 22 (2012) 4634-4667.
16. [16]
  R.R. Liang, X. Zhao, Org. Chem. Front. 5 (2018) 3341-3356. doi: 10.1039/C8QO00830B
17. [17]
  (a) D.B. Shinde, S. Kandambeth, P. Pachfule, R.R. Kumar, R. Banerjee, Chem. Commun. 51 (2015) 310-313;
  (b) A. Halder, S. Kandambeth, B.P. Biswal, et al., Angew. Chem. Int. Ed. 55 (2016) 7806-7810.
18. [18]
  Dassault Systèmes BIOVIA, Materials Studio 8.0, Dassault Systèmes San Diego, (2014).
19. [19]
  (a) T.Y. Zhou, S.Q. Xu, Q. Wen, Z.F. Pang, X. Zhao, J. Am. Chem. Soc. 136 (2014) 15885-15888;
  (b) Z.F. Pang, T.Y. Zhou, R.R. Liang, Q.Y. Qi, X. Zhao, Chem. Sci. 8 (2017) 3866-3870.
20. [20]
  X. Chen, M. Addicoat, E. Jin, et al., J. Am. Chem. Soc. 137 (2015) 3241-3247. doi: 10.1021/ja509602c
1. [1]
  Yuting Wu , Haifeng Lv , Xiaojun Wu . Design of two-dimensional porous covalent organic framework semiconductors for visible-light-driven overall water splitting: A theoretical perspective. Chinese Journal of Structural Chemistry, 2024, 43(11): 100375-100375. doi: 10.1016/j.cjsc.2024.100375
2. [2]
  Jiaqi Ma , Lan Li , Yiming Zhang , Jinjie Qian , Xusheng Wang . Covalent organic frameworks: Synthesis, structures, characterizations and progress of photocatalytic reduction of CO2. Chinese Journal of Structural Chemistry, 2024, 43(12): 100466-100466. doi: 10.1016/j.cjsc.2024.100466
3. [3]
  Weixu Li , Yuexin Wang , Lin Li , Xinyi Huang , Mengdi Liu , Bo Gui , Xianjun Lang , Cheng Wang . Promoting energy transfer pathway in porphyrin-based sp2 carbon-conjugated covalent organic frameworks for selective photocatalytic oxidation of sulfide. Chinese Journal of Structural Chemistry, 2024, 43(7): 100299-100299. doi: 10.1016/j.cjsc.2024.100299
4. [4]
  Deshuai Zhen , Chunlin Liu , Qiuhui Deng , Shaoqi Zhang , Ningman Yuan , Le Li , Yu Liu . A review of covalent organic frameworks for metal ion fluorescence sensing. Chinese Chemical Letters, 2024, 35(8): 109249-. doi: 10.1016/j.cclet.2023.109249
5. [5]
  Guorong Li , Yijing Wu , Chao Zhong , Yixin Yang , Zian Lin . Predesigned covalent organic framework with sulfur coordination: Anchoring Au nanoparticles for sensitive colorimetric detection of Hg(Ⅱ). Chinese Chemical Letters, 2024, 35(5): 108904-. doi: 10.1016/j.cclet.2023.108904
6. [6]
  Yue Qian , Zhoujia Liu , Haixin Song , Ruize Yin , Hanni Yang , Siyang Li , Weiwei Xiong , Saisai Yuan , Junhao Zhang , Huan Pang . Imide-based covalent organic framework with excellent cyclability as an anode material for lithium-ion battery. Chinese Chemical Letters, 2024, 35(6): 108785-. doi: 10.1016/j.cclet.2023.108785
7. [7]
  Xiaotao Jin , Yanlan Wang , Yingping Huang , Di Huang , Xiang Liu . Percarbonate activation catalyzed by nanoblocks of basic copper molybdate for antibiotics degradation: High performance, degradation pathways and mechanism. Chinese Chemical Letters, 2024, 35(10): 109499-. doi: 10.1016/j.cclet.2024.109499
8. [8]
  Gaofeng Zeng , Shuyu Liu , Manle Jiang , Yu Wang , Ping Xu , Lei Wang . Micro/Nanorobots for Pollution Detection and Toxic Removal. University Chemistry, 2024, 39(9): 229-234. doi: 10.12461/PKU.DXHX202311055
9. [9]
  Chao Liu , Chao Jia , Shi-Xian Gan , Qiao-Yan Qi , Guo-Fang Jiang , Xin Zhao . A luminescent one-dimensional covalent organic framework for organic arsenic sensing in water. Chinese Chemical Letters, 2024, 35(11): 109750-. doi: 10.1016/j.cclet.2024.109750
10. [10]
  Fan Wu , Wenchang Tian , Jin Liu , Qiuting Zhang , YanHui Zhong , Zian Lin . Core-Shell Structured Covalent Organic Framework-Coated Silica Microspheres as Mixed-Mode Stationary Phase for High Performance Liquid Chromatography. University Chemistry, 2024, 39(11): 319-326. doi: 10.12461/PKU.DXHX202403031
11. [11]
  Qiuting Zhang , Fan Wu , Jin Liu , Zian Lin . Chromatographic Stationary Phase and Chiral Separation Using Frame Materials. University Chemistry, 2025, 40(4): 291-298. doi: 10.12461/PKU.DXHX202405174
12. [12]
  Yunyu Zhao , Chuntao Yang , Yingjian Yu . A review on covalent organic frameworks for rechargeable zinc-ion batteries. Chinese Chemical Letters, 2024, 35(7): 108865-. doi: 10.1016/j.cclet.2023.108865
13. [13]
  Hong Dong , Feng-Ming Zhang . Covalent organic frameworks for artificial photosynthetic diluted CO2 reduction. Chinese Journal of Structural Chemistry, 2024, 43(7): 100307-100307. doi: 10.1016/j.cjsc.2024.100307
14. [14]
  Zhiqiang Liu , Qiang Gao , Wei Shen , Meifeng Xu , Yunxin Li , Weilin Hou , Hai-Wei Shi , Yaozuo Yuan , Erwin Adams , Hian Kee Lee , Sheng Tang . Removal and fluorescence detection of antibiotics from wastewater by layered double oxides/metal-organic frameworks with different topological configurations. Chinese Chemical Letters, 2024, 35(8): 109338-. doi: 10.1016/j.cclet.2023.109338
15. [15]
  Di An , Mingdong She , Ziyang Zhang , Ting Zhang , Miaomiao Xu , Jinjun Shao , Qian Shen , Xuna Tang . Light-responsive nanomaterials for biofilm removal in root canal treatment. Chinese Chemical Letters, 2025, 36(2): 109841-. doi: 10.1016/j.cclet.2024.109841
16. [16]
  Yinyin Xu , Yuanyuan Li , Jingbo Feng , Chen Wang , Yan Zhang , Yukun Wang , Xiuwen Cheng . Covalent organic frameworks doped with manganese-metal organic framework for peroxymonosulfate activation. Chinese Chemical Letters, 2024, 35(4): 108838-. doi: 10.1016/j.cclet.2023.108838
17. [17]
  Xinyi Cao , Yucheng Jin , Hailong Wang , Xu Ding , Xiaolin Liu , Baoqiu Yu , Xiaoning Zhan , Jianzhuang Jiang . A tetraaldehyde-derived porous organic cage and covalent organic frameworks: Syntheses, structures, and iodine vapor capture. Chinese Chemical Letters, 2024, 35(9): 109201-. doi: 10.1016/j.cclet.2023.109201
18. [18]
  Rongxin Zhu , Shengsheng Yu , Xuanzong Yang , Ruyu Zhu , Hui Liu , Kaikai Niu , Lingbao Xing . Construction of pyrene-based hydrogen-bonded organic frameworks as photocatalysts for photooxidation of styrene in water. Chinese Chemical Letters, 2024, 35(10): 109539-. doi: 10.1016/j.cclet.2024.109539
19. [19]
  Tao Long , Peng Chen , Bin Feng , Caili Yang , Kairong Wang , Yulei Wang , Can Chen , Yaping Wang , Ruotong Li , Meng Wu , Minhuan Lan , Wei Kong Pang , Jian-Fang Wu , Yuan-Li Ding . Reinforced concrete-like Na_3.5V_1.5Mn_0.5(PO₄)₃@graphene hybrids with hierarchical porosity as durable and high-rate sodium-ion battery cathode. Chinese Chemical Letters, 2024, 35(4): 109267-. doi: 10.1016/j.cclet.2023.109267
20. [20]
  Junhua Wang , Xin Lian , Xichuan Cao , Qiao Zhao , Baiyan Li , Xian-He Bu . Dual polarization strategy to enhance CH₄ uptake in covalent organic frameworks for coal-bed methane purification. Chinese Chemical Letters, 2024, 35(8): 109180-. doi: 10.1016/j.cclet.2023.109180

Get Citation

PDF

XML

Metrics

PDF Downloads(9)
Abstract views(1629)
HTML views(297)

通讯作者: 陈斌, bchen63@163.com

1.
沈阳化工大学材料科学与工程学院沈阳 110142