Citation: An Zhen-Zhen, Li Zhuang, Guo Yong-Yang, Chen Xiao-Ling, Zhang Kang-Ning, Zhang Dong-Xia, Xue Zhong-Hua, Zhou Xi-Bin, Lu Xiao-Quan. Preparation of chitosan/N-doped graphene natively grown on hierarchical porous carbon nanocomposite as a sensor platform for determination of tartrazine[J]. Chinese Chemical Letters, ;2017, 28(7): 1492-1498. doi: 10.1016/j.cclet.2017.02.014 shu

Preparation of chitosan/N-doped graphene natively grown on hierarchical porous carbon nanocomposite as a sensor platform for determination of tartrazine

a.
Key Laboratory of Bioelectrochemistry & Environmental Analysis of Gansu Province, College of Geography and Environment Science, Northwest Normal University, Lanzhou 730070, China
b.
College of Chemistry and Chemical Engineering, Northwest Normal University, Lanzhou 730070, China

Corresponding author: Zhou Xi-Bin, zhouxb@nwnu.edu.cn; 290194053@qq.com Lu Xiao-Quan, Luxq@nwnu.edu.cn
Received Date: 7 December 2016
Revised Date: 3 January 2017
Accepted Date: 20 February 2017
Available Online: 22 July 2017

Figures(7)

In this work, the chitosan and N-doped graphene natively grown on hierarchical porous carbon (N-PC-G/CS) nanocomposite was obtained by ultrasonic method, as a novel sensor platform for determination of tartrazine (TT). The nanocomposite as prepared had well dispersivity in water and excellent conductivity. The N-PC-G/CS nanocomposite was characterized by scanning electron microscopy (SEM), transmission electron microscopy (TEM), nitrogen adsorption-desorption, fourier transform infrared (FTIR) and electrochemical impedance spectroscopy (EIS). The application of N-PC-G/CS for determination of tartrazine (TT) was investigated by chronocoulometry (CC), cyclic voltammetry (CV) and differential pulse voltammetry (DPV). Under optimized conditions, the sensor displayed a sensitive response to TT within a wide concentration range of 0.05-15.0μmol/L, the detection limits is 0.036 μmol/L (S/N=3). Furthermore, this nanocomposite could be efficiently applied for determination of TT in soft drink samples.
- Porous carbon,
- Graphene,
- Chitosan,
- Sensor,
- Tartrazine
1. [1]
  Nevado J.J.B., Cabanillas C.G., Salcedo A.M.C.. Simultaneous spectrophotometric determination of three food dyes by using the first derivative of ratio spectra[J]. Talanta, 1995,42:2043-2051. doi: 10.1016/0039-9140(95)01695-3
2. [2]
  Rowe K.S., Rowe K.J.. Synthetic food coloring and behavior: a dose response effect in a double-blind placebo-controlled, repeated-measures study[J]. J. Pediatr., 1994,125:691-698. doi: 10.1016/S0022-3476(06)80164-2
3. [3]
  Borzelleca J.F., Hallagan J.B.. Chronic toxicity/carcinogenicity studies of FD & C Yellow No. 5(tartrazine) in rats[J]. Food Chem. Toxicol., 1988,26:179-187. doi: 10.1016/0278-6915(88)90117-2
4. [4]
  Tanaka T.. Reproductive and neurobehavioural toxicity study of Ponceau 4R administered to mice in the diet[J]. Food Chem. Toxicol., 2006,44:1651-1658. doi: 10.1016/j.fct.2006.05.001
5. [5]
  European Parliament and Council Directive 94/36/EC . Council directive 94/43/EC of 27 July 1994 establishing annex VI to directive 91/414/EEC concerning the placing of plant protection products on the market[J]. Off. J. L, 1994,227:31-55.
6. [6]
  Minioti K.S., Sakellariou C.F., Thomaidis N.S.. Determination of 13 synthetic food colorants in water-soluble foods by reversed-phase high-performance liquid chromatography coupled with diode-array detector[J]. Anal. Chim. Acta, 2007,583:103-110. doi: 10.1016/j.aca.2006.10.002
7. [7]
  Berzas J.J., Flores J.R., Llerena M.J.V., Farinas N.R.. Spectrophotometric resolution of ternary mixtures of Tartrazine, Patent Blue V and Indigo Carmine in commercial products[J]. Anal. Chim. Acta, 1999,391:353-364. doi: 10.1016/S0003-2670(99)00215-9
8. [8]
  Din? E., Baydan E., Kanbur M., Onur F.. Spectrophotometric multicomponent determination of sunset yellow, tartrazine and allura red in soft drink powder by double divisor-ratio spectra derivative, inverse least-squares and principal component regression methods[J]. Talanta, 2002,58:579-594. doi: 10.1016/S0039-9140(02)00320-X
9. [9]
  Yamada M., Nakamura M., Yamada T., Maitani T., Goda Y.. Structural determination of unknown subsidiary colors in food yellowNO.5(Sunset Yellow FCF)[J]. Chem. Pharm. Bull., 1996,44:1624-1627. doi: 10.1248/cpb.44.1624
10. [10]
  Zou T.T., He P.L., Yasen A., Li Z.. Determination of seven synthetic dyes in animal feeds and meat by high performance liquid chromatography with diode array and tandem mass detectors[J]. Food Chem., 2013,138:1742-1748. doi: 10.1016/j.foodchem.2012.11.084
11. [11]
  Cheng Q., Xia S.H., Tong J.H., Wu K.B.. Highly-sensitive electrochemical sensing platforms for food colourants based on the property-tuning of porous carbon[J]. Anal. Chim. Acta, 2015,887:75-81. doi: 10.1016/j.aca.2015.06.013
12. [12]
  Qiu X.L., Lu L.M., Leng J.. An enhanced electrochemical platform based on graphene oxide and multi-walled carbon nanotubes nanocomposite for sensitive determination of Sunset Yellow and Tartrazine[J]. Food Chem., 2016,190:889-895. doi: 10.1016/j.foodchem.2015.06.045
13. [13]
  Wang M.L., Zhao J.W.. A facile method used for simultaneous determination of Ponceau 4R, allura red and Tartrazine in alcoholic beverages[J]. J. Electrochem. Soc., 2015,162:H321-H327. doi: 10.1149/2.0111506jes
14. [14]
  Song X.J., Shi Z., Tan X.. One-step solvent exfoliation of graphite to produce a highly-sensitive electrochemical sensor for tartrazine[J]. Sens. Actuators B Chem., 2014,197:104-108. doi: 10.1016/j.snb.2014.02.064
15. [15]
  Liang J., Du X., Gibson C., Du X.W., Qiao S.Z.. N-doped graphene natively grown on hierarchical ordered porous carbon for enhanced oxygen reduction[J]. Adv. Mater., 2013,25:6226-6231. doi: 10.1002/adma.201302569
16. [16]
  Li Z., An Z.Z., Guo Y.Y.. Au-Pt bimetallic nanoparticles supported on functionalized nitrogen-doped graphene for sensitive detection of nitrite[J]. Talanta, 2016,161:713-720. doi: 10.1016/j.talanta.2016.09.033
17. [17]
  Zhang Y., Su M., Ge L.. Synthesis and characterization of graphene nanosheets attached to spiky MnO₂ nanospheres and its application in ultrasensitive immunoassay[J]. Carbon, 2013,57:22-33. doi: 10.1016/j.carbon.2013.01.012
18. [18]
  Janegitz B.C., Marcolino-Junior L.H., Campana-Filho S.P., Faria R.C., FatibelloFilho O.. Anodic stripping voltammetric determination of copper(Ⅱ) using a functionalized carbon nanotubes paste electrode modified with crosslinked chitosan[J]. Sens. Actuators B Chem., 2009,142:260-266. doi: 10.1016/j.snb.2009.08.033
19. [19]
  Ling S.J., Yuan R., Chai Y.Q., Zhang T.T.. Study on immunosensor based on gold nanoparticles/chitosan and MnO₂ nanoparticles compositemembrane/Prussian blue modified gold electrode[J]. Bioprocess Biosyst. Eng., 2009,32:407-414. doi: 10.1007/s00449-008-0260-2
20. [20]
  Batra B., Pundir C.S.. An amperometric glutamate biosensor based on immobilization of glutamate oxidase onto carboxylated multiwalled carbon nanotubes/gold nanoparticles/chitosan composite film modified Au electrode[J]. Biosens. Bioelectron., 2013,47:496-501. doi: 10.1016/j.bios.2013.03.063
21. [21]
  Darmstadt H., Roy C., Kaliaguine S., Choi S.J., Ryoo R.. Surface chemistry of ordered mesoporous carbons[J]. Carbon, 2002,40:2673-2683. doi: 10.1016/S0008-6223(02)00187-2
22. [22]
  Thomas A., Fischer A., Goettmann F.. Graphitic carbon nitride materials: variation of structure and morphology and their use as metal-free catalysts[J]. J. Mater. Chem., 2008,18:4893-4908. doi: 10.1039/b800274f
23. [23]
  Zheng Y., Jiao Y., Chen J.. Nanoporous graphitic-C3N4@carbon metal-free electrocatalysts for highly efficient oxygen reduction[J]. J. Am. Chem. Soc., 2011,133:20116-20119. doi: 10.1021/ja209206c
24. [24]
  Liang J., Zheng Y., Chen J.. Facile oxygen reduction on a threedimensionally ordered macroporous graphitic C₃N₄/carbon composite electrocatalyst[J]. Angew. Chem., 2012,51:3892-3896. doi: 10.1002/anie.v51.16
25. [25]
  Thein-Han W.W., Misra R.D.K.. Biomimetic chitosan-nanohydroxyapatite composite scaffolds for bone tissue engineering[J]. Acta Biomater., 2009,5:1182-1197. doi: 10.1016/j.actbio.2008.11.025
26. [26]
  Venkatesan J., Qian Z.J., Ryu B., Kumar N.A., Kima S.K.. Preparation and characterization of carbon nanotube-grafted-chitosan-natural hydroxyapatite composite for bone tissue engineering[J]. Carbohyd. Polym., 2011,83:569-577. doi: 10.1016/j.carbpol.2010.08.019
27. [27]
  Anson F.C.. Application of potentiostatic current integration to the study of the adsorption of cobalt (Ⅲ)-(ethylenedinitrilo(tetraacetate) on mercury electrodes[J]. Anal. Chem., 1964,36:932-934. doi: 10.1021/ac60210a068
28. [28]
  R.N. Adams, Electrochemistry at Solid Electrodes, Marcel Dekker Inc., New York, 1969.
29. [29]
  Zhang J., Wang X., Zhang S.B.. An electrochemical sensor for simultaneous determination of ponceau 4R and tartrazine based on an ionic liquid modified expanded graphite paste electrode[J]. J. Electrochem. Soc., 2014,161:H453-H457. doi: 10.1149/2.0271409jes
30. [30]
  Meng Y., Gu D., Zhang F.Q., Shi Y.F.. Ordered mesoporous polymers and homologous carbon frameworks: amphiphilic surfactant templating and direct transformation[J]. Angew. Chem., 2005,117:7215-7221. doi: 10.1002/(ISSN)1521-3757
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1.
沈阳化工大学材料科学与工程学院沈阳 110142