高效金属-有机框架的工程设计用于光催化CO<sub>2</sub>还原

引用本文: 彭国强, 李秀艳, 李敏, 苏志博, 胡发露, 周国伟. 高效金属-有机框架的工程设计用于光催化CO₂还原[J]. 物理化学学报, 2026, 42(2): 100164. doi: 10.1016/j.actphy.2025.100164 shu

Citation: Guoqiang Peng, Xiuyan Li, Min Li, Zhibo Su, Falu Hu, Guowei Zhou. Engineering efficient metal-organic frameworks for photocatalytic CO₂ reduction[J]. Acta Physico-Chimica Sinica, 2026, 42(2): 100164. doi: 10.1016/j.actphy.2025.100164 shu

高效金属-有机框架的工程设计用于光催化CO₂还原

彭国强 ^1, ,
李秀艳 ^2, ,
李敏 ^1, ,
苏志博 ^1, ,
胡发露 ^{1,
,} ,
周国伟 ^{1,
,}

1.
齐鲁工业大学(山东省科学院)化学与化工学院, 山东省高校轻工精细化学品重点实验室, 济南市多尺度功能材料工程实验室, 山东济南 250353
2.
潍坊科技学院, 化工与环境学院, 山东省海洋精细化工绿色化高值化工程技术研究中心, 山东潍坊 262700

通讯作者: Email: faluhu@qlu.edu.cn (胡发露); gwzhou@qlu.edu.cn (周国伟)

摘要: 过去几十年间，过量CO₂排放引发了诸多环境问题。太阳能驱动的光催化CO₂转化为高附加值化学品，为能源与环境问题提供了极具前景的解决方案。近年来，一种由有机配体与金属离子/簇自组装形成的多孔配位聚合物——金属有机框架(MOFs)，因其优异的CO₂捕获能力和可调控结构，在光催化转化CO₂领域获得广泛探索。然而，开发具有高效CO₂转化性能的MOFs仍面临重大挑战。本综述系统阐述了构建高效光催化CO₂还原MOFs的四大关键工程策略：配体工程、次级构筑单元(SBU)工程、缺陷工程和形貌工程。这些策略聚焦于优化MOFs的关键结构特性，这些特性对其光催化CO₂还原性能(特别是光吸收能力、CO₂吸附能力及电荷分离传输效率)具有决定性影响。所建立的设计原则与调控策略展现出广泛适用性，可拓展用于指导多种MOF基功能体系的理性设计。此外，我们批判性评估了各策略的优缺点，着重阐明其特定贡献与固有局限性。最后，我们展望了MOF基光催化CO₂还原的发展前景，并指明了未来具有潜力的研究方向。

关键词:

English

Engineering efficient metal-organic frameworks for photocatalytic CO₂ reduction

Guoqiang Peng ^1, ,
Xiuyan Li ^2, ,
Min Li ^1, ,
Zhibo Su ^1, ,
Falu Hu ^{1,
,} ,
Guowei Zhou ^{1,
,}

1.
Key Laboratory of Fine Chemicals in Universities of Shandong, Jinan Engineering Laboratory for Multi-scale Functional Materials, School of Chemistry and Chemical Engineering, Qilu University of Technology (Shandong Academy of Sciences), Jinan 250353, Shandong Province, China
2.
School of Chemical Engineering and Environment, Shandong Engineering Research Center of Green and High-Value Marine Fine Chemical, Weifang University of Science and Technology, Weifang 262700, Shandong Province, China

Corresponding author: Email: faluhu@qlu.edu.cn (Falu Hu); gwzhou@qlu.edu.cn (Guowei Zhou)

Received Date: 12 July 2025
Accepted Date: 17 August 2025
Revised Date: 14 August 2025
Available Online: 15 February 2026

Abstract: Over the past decades, excessive CO₂ emissions have led to various environmental issues. Solar-driven photocatalytic conversion of CO₂ into valuable chemicals offers a promising solution for energy and environmental problems. Recently, a class of porous coordination polymers that self-assemble from organic linkers and metal ions or clusters, metal-organic frameworks (MOFs), have been widely explored for photoinduced CO₂ conversion because of their great CO₂ capture ability and adjustable structures. However, the development of MOFs with high efficiency for CO₂ conversion remains a significant challenge. In this review, we elaborate on four key engineering strategies for constructing efficient MOFs toward photocatalytic CO₂ reduction: ligand engineering, secondary building unit (SBU) engineering, defect engineering, and morphology engineering. These strategies focus on optimizing key structural properties of MOFs that critically influence their catalytic performance in CO₂ photoreduction, notably light absorption, CO₂ adsorption capacity, and charge separation and transport. The established design principles and modulation strategies demonstrate broad applicability and can be extended to guide the rational design of diverse MOF-based functional systems. Furthermore, we critically evaluate the advantages and disadvantages of each strategy, highlighting their specific contributions and inherent limitations. Finally, we outline the development prospects and identify promising future research directions for MOF-based photocatalytic CO₂ reduction.

Key words:

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通讯作者: 陈斌, bchen63@163.com

1.
沈阳化工大学材料科学与工程学院沈阳 110142

高效金属-有机框架的工程设计用于光催化CO₂还原

通讯作者: Email: faluhu@qlu.edu.cn (胡发露); gwzhou@qlu.edu.cn (周国伟)

English

Engineering efficient metal-organic frameworks for photocatalytic CO₂ reduction

Corresponding author: Email: faluhu@qlu.edu.cn (Falu Hu); gwzhou@qlu.edu.cn (Guowei Zhou)

CCS Chemistry：嵌段共聚物自组装成 “三明治”二维有机材料，实现纳米级压力传感功能

CCS Chemistry：颜徐州、鲍哲南：你的皮肤可能是一片SPMs

CCS Chemistry：工作高效不疲劳，只须让催化剂动起来

CCS Chemistry：静电组装导向聚合- 聚电解质纳米凝胶量化制备新策略

CCS Chemistry：金黄色葡萄球菌醛基脱氢酶是如何识别特异性底物的？

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通讯作者: 陈斌, bchen63@163.com

中国化学会秘书处

高效金属-有机框架的工程设计用于光催化CO2还原

通讯作者: Email: faluhu@qlu.edu.cn (胡发露); gwzhou@qlu.edu.cn (周国伟)

English

Engineering efficient metal-organic frameworks for photocatalytic CO2 reduction

Corresponding author: Email: faluhu@qlu.edu.cn (Falu Hu); gwzhou@qlu.edu.cn (Guowei Zhou)

CCS Chemistry：嵌段共聚物自组装成 “三明治”二维有机材料，实现纳米级压力传感功能

CCS Chemistry：颜徐州、鲍哲南： 你的皮肤可能是一片SPMs

CCS Chemistry：工作高效不疲劳，只须让催化剂动起来

CCS Chemistry：静电组装导向聚合- 聚电解质纳米凝胶量化制备新策略

CCS Chemistry：金黄色葡萄球菌醛基脱氢酶是如何识别特异性底物的？

计量

文章相关

通讯作者: 陈斌, bchen63@163.com

中国化学会秘书处

高效金属-有机框架的工程设计用于光催化CO₂还原

Engineering efficient metal-organic frameworks for photocatalytic CO₂ reduction

CCS Chemistry：颜徐州、鲍哲南：你的皮肤可能是一片SPMs