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高效金属-有机框架的工程设计用于光催化CO2还原

彭国强 ,  李秀艳 ,  李敏 ,  苏志博 ,  胡发露 ,  周国伟

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引用本文: 彭国强, 李秀艳, 李敏, 苏志博, 胡发露, 周国伟. 高效金属-有机框架的工程设计用于光催化CO2还原[J]. 物理化学学报, 2026, 42(2): 100164. doi: 10.1016/j.actphy.2025.100164 shu
Citation:  Guoqiang Peng, Xiuyan Li, Min Li, Zhibo Su, Falu Hu, Guowei Zhou. Engineering efficient metal-organic frameworks for photocatalytic CO2 reduction[J]. Acta Physico-Chimica Sinica, 2026, 42(2): 100164. doi: 10.1016/j.actphy.2025.100164 shu

高效金属-有机框架的工程设计用于光催化CO2还原

  • 1.

    齐鲁工业大学(山东省科学院)化学与化工学院, 山东省高校轻工精细化学品重点实验室, 济南市多尺度功能材料工程实验室, 山东 济南 250353

  • 2.

    潍坊科技学院, 化工与环境学院, 山东省海洋精细化工绿色化高值化工程技术研究中心, 山东 潍坊 262700

    • 通讯作者: Email: faluhu@qlu.edu.cn (胡发露); gwzhou@qlu.edu.cn (周国伟)
摘要: 过去几十年间，过量CO2排放引发了诸多环境问题。太阳能驱动的光催化CO2转化为高附加值化学品，为能源与环境问题提供了极具前景的解决方案。近年来，一种由有机配体与金属离子/簇自组装形成的多孔配位聚合物——金属有机框架(MOFs)，因其优异的CO2捕获能力和可调控结构，在光催化转化CO2领域获得广泛探索。然而，开发具有高效CO2转化性能的MOFs仍面临重大挑战。本综述系统阐述了构建高效光催化CO2还原MOFs的四大关键工程策略：配体工程、次级构筑单元(SBU)工程、缺陷工程和形貌工程。这些策略聚焦于优化MOFs的关键结构特性，这些特性对其光催化CO2还原性能(特别是光吸收能力、CO2吸附能力及电荷分离传输效率)具有决定性影响。所建立的设计原则与调控策略展现出广泛适用性，可拓展用于指导多种MOF基功能体系的理性设计。此外，我们批判性评估了各策略的优缺点，着重阐明其特定贡献与固有局限性。最后，我们展望了MOF基光催化CO2还原的发展前景，并指明了未来具有潜力的研究方向。

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