Citation: Fanpeng Meng, Fei Zhao, Jingkai Lin, Jinsheng Zhao, Huayang Zhang, Shaobin Wang. Optimizing interfacial electric fields in carbon nitride nanosheet/spherical conjugated polymer S-scheme heterojunction for hydrogen evolution[J]. Acta Physico-Chimica Sinica, ;2025, 41(8): 100095. doi: 10.1016/j.actphy.2025.100095 shu

Optimizing interfacial electric fields in carbon nitride nanosheet/spherical conjugated polymer S-scheme heterojunction for hydrogen evolution

Fanpeng Meng ^{1, †} ,
Fei Zhao ^{2, †} ,
Jingkai Lin ³ ,
Jinsheng Zhao ^1,, ,
Huayang Zhang ^3,, ,
Shaobin Wang ³

1.
Shandong Key Laboratory of Chemical Energy Storage and Novel Cell Technology, College of Chemistry and Chemical Engineering, Liaocheng University, Liaocheng 252059, Shandong Province, China
2.
College of Chemistry and Chemical Engineering, Taishan University, Taian 271000, Shandong Province, China
3.
School of Chemical Engineering, The University of Adelaide, Adelaide SA 5005, Australia

Corresponding author: Jinsheng Zhao, j.s.zhao@163.com Huayang Zhang, huayang.zhang@adelaide.edu.au

^†

Received Date: 18 March 2025
Revised Date: 2 April 2025
Accepted Date: 15 April 2025

Fund Project: the National Natural Science Foundation of China 22302085the National Natural Science Foundation of China 22172069the Natural Science Foundation of Shandong Province ZR2024QB046the Natural Science Foundation of Shandong Province ZR2021ME071the Research Projects of Liaocheng University 318052272H. Zhang and S. Wang acknowledges the support from Discovery Project DP230102406H. Zhang and S. Wang acknowledges the support from Discovery Project DP240102787Australian Laureate Fellowships from the Australian Research Council FL230100178

Designing heterojunctions based on carbon nitride offers a promising pathway for enhancing photocatalytic efficiency. This study develops an all-organic S-scheme metal-free heterojunction uniquely composed of carbon nitride nanosheets (GCNNS) and a donor-acceptor conjugated polymer, poly p-aminobenzylidene-so-aniline (PASO), synthesized through a simple yet effective ball-milling technique. This heterojunction demonstrates excellent photocatalytic efficiency for hydrogen (H₂) evolution. The optimized GCNNS/PASO-10 sample attains an H₂ evolution rate of 10.12 mmol·g⁻¹·h⁻¹, which is about 5.9 times and 19.5 times greater than those of pure GCNNS and PASO, respectively. This improvement is due to the unique interfacial bonding, increased visible-light absorption, and efficient charge carrier separation facilitated by a strong internal electric field within the S-scheme. Theoretical calculations and characterization reveal that this heterojunction's S-scheme mechanism optimally aligns energy bands and promotes spatial charge separation, driving superior photocatalytic activity. This work presents the unique advantage of all-organic materials for heterojunction construction and provides insights into designing advanced S-scheme systems for sustainable energy conversion.
- All-organic heterojunction,
- Carbon nitride nanosheets,
- S-scheme heterojunction,
- H₂ evolution,
- D-A conjugated polymers
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沈阳化工大学材料科学与工程学院沈阳 110142