优化氮化碳纳米片/球形共轭聚合物S型异质结界面电场以促进析氢反应

引用本文: 孟凡鹏, 赵飞, 林靖恺, 赵金生, 张华阳, 王少彬. 优化氮化碳纳米片/球形共轭聚合物S型异质结界面电场以促进析氢反应[J]. 物理化学学报, 2025, 41(8): 100095. doi: 10.1016/j.actphy.2025.100095 shu

Citation: Fanpeng Meng, Fei Zhao, Jingkai Lin, Jinsheng Zhao, Huayang Zhang, Shaobin Wang. 优化氮化碳纳米片/球形共轭聚合物S型异质结界面电场以促进析氢反应[J]. Acta Physico-Chimica Sinica, 2025, 41(8): 100095. doi: 10.1016/j.actphy.2025.100095 shu

优化氮化碳纳米片/球形共轭聚合物S型异质结界面电场以促进析氢反应

孟凡鹏 ^1, ,
赵飞 ^2, ,
林靖恺 ^3, ,
赵金生 ^1, ,
张华阳 ^3, ,
王少彬 ^3,

1.
山东省化学储能与新型电池技术重点实验室, 聊城大学化学化工学院, 山东聊城 252059;
2.
泰山学院化学化工学院, 山东泰安 271000;
3.
School of Chemical Engineering, The University of Adelaide, Adelaide SA 5005, Australia
基金项目:
国家自然科学基金(22302085,22172069),山东省自然科学基金(ZR2024QB046,ZR2021ME071)及聊城大学科研项目(318052272)资助.张华阳与王少彬获澳大利亚研究委员会发现项目(DP230102406,DP240102787)及桂冠学者计划(FL230100178)支持

摘要: 基于氮化碳设计异质结是提升光催化效率的有效途径。本研究通过简便高效的球磨技术，构建了由氮化碳纳米片(GCNNS)与供体-受体共轭聚合物(聚对氨基亚苄基异苯胺，PASO)组成的全有机S型无金属异质结。该异质结展现出优异的光催化产氢性能，优化后的GCNNS/PASO-10样品的产氢速率达到10.12 mmol·g^-1·h^-1，分别是GCNNS和PASO的5.9倍和19.5倍。这种提升源于独特的界面结合作用、增强的可见光吸收能力以及S型异质结强内建电场促进的高效电荷分离。理论计算与表征结果表明，该异质结的S型机制实现了能带最优匹配并推动了空间电荷的有效分离，从而显著提升了光催化活性。本工作揭示了全有机材料在异质结构建中的独特优势，为设计先进S型体系以实现可持续能源转化提供了新思路。

关键词:

English

优化氮化碳纳米片/球形共轭聚合物S型异质结界面电场以促进析氢反应

1.
Shandong Key Laboratory of Chemical Energy Storage and Novel Cell Technology, College of Chemistry and Chemical Engineering, Liaocheng University, Liaocheng 252059, Shandong Province, China;
2.
College of Chemistry and Chemical Engineering, Taishan University, Taian 271000, Shandong Province, China;
3.
School of Chemical Engineering, The University of Adelaide, Adelaide SA 5005, Australia
Received Date: 18 March 2025
Accepted Date: 15 April 2025
Revised Date: 02 April 2025
Fund Project:
This work was funded by the National Natural Science Foundation of China (22302085, 22172069), the Natural Science Foundation of Shandong Province (ZR2024QB046, ZR2021ME071) and the Research Projects of Liaocheng University (318052272). H. Zhang and S. Wang acknowledges the support from Discovery Project (DP230102406, DP240102787), and Australian Laureate Fellowships (FL230100178) from the Australian Research Council.

Abstract: 基于氮化碳设计异质结是提升光催化效率的有效途径。本研究通过简便高效的球磨技术，构建了由氮化碳纳米片(GCNNS)与供体-受体共轭聚合物(聚对氨基亚苄基异苯胺，PASO)组成的全有机S型无金属异质结。该异质结展现出优异的光催化产氢性能，优化后的GCNNS/PASO-10样品的产氢速率达到10.12 mmol·g^-1·h^-1，分别是GCNNS和PASO的5.9倍和19.5倍。这种提升源于独特的界面结合作用、增强的可见光吸收能力以及S型异质结强内建电场促进的高效电荷分离。理论计算与表征结果表明，该异质结的S型机制实现了能带最优匹配并推动了空间电荷的有效分离，从而显著提升了光催化活性。本工作揭示了全有机材料在异质结构建中的独特优势，为设计先进S型体系以实现可持续能源转化提供了新思路。

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沈阳化工大学材料科学与工程学院沈阳 110142

优化氮化碳纳米片/球形共轭聚合物S型异质结界面电场以促进析氢反应

English

优化氮化碳纳米片/球形共轭聚合物S型异质结界面电场以促进析氢反应

CCS Chemistry：嵌段共聚物自组装成 “三明治”二维有机材料，实现纳米级压力传感功能

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通讯作者: 陈斌, bchen63@163.com

中国化学会秘书处

优化氮化碳纳米片/球形共轭聚合物S型异质结界面电场以促进析氢反应

English

优化氮化碳纳米片/球形共轭聚合物S型异质结界面电场以促进析氢反应

CCS Chemistry：嵌段共聚物自组装成 “三明治”二维有机材料，实现纳米级压力传感功能

CCS Chemistry：颜徐州、鲍哲南： 你的皮肤可能是一片SPMs

CCS Chemistry：工作高效不疲劳，只须让催化剂动起来

CCS Chemistry：静电组装导向聚合- 聚电解质纳米凝胶量化制备新策略

CCS Chemistry：金黄色葡萄球菌醛基脱氢酶是如何识别特异性底物的？

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