Citation: Zeqiu Chen, Limiao Cai, Jie Guan, Zhanyang Li, Hao Wang, Yaoguang Guo, Xingtao Xu, Likun Pan. Advanced electrode materials in capacitive deionization for efficient lithium extraction[J]. Acta Physico-Chimica Sinica, ;2025, 41(8): 100089. doi: 10.1016/j.actphy.2025.100089 shu

Advanced electrode materials in capacitive deionization for efficient lithium extraction

Zeqiu Chen ^{1, †} ,
Limiao Cai ^{1, †} ,
Jie Guan ¹ ,
Zhanyang Li ¹ ,
Hao Wang ² ,
Yaoguang Guo ^1,, ,
Xingtao Xu ^3,, ,
Likun Pan ^{2, 4,,}

1.
Shanghai Collaborative Innovation Centre for WEEE Recycling, School of Resources and Environmental Engineering, Shanghai Polytechnic University, Shanghai 201209, China
2.
Shanghai Key Laboratory of Magnetic Resonance, School of Physics and Electronic Science, East China Normal University, Shanghai 200241, China
3.
Marine Science and Technology College, Zhejiang Ocean University, Zhoushan 316022, Zhejiang Province, China
4.
Institute of Magnetic Resonance and Molecular Imaging in Medicine, East China Normal University, Shanghai 200241, China

Corresponding author: Yaoguang Guo, ygguo@sspu.edu.cn Xingtao Xu, xingtao.xu@zjou.edu.cn Likun Pan, lkpan@phy.ecnu.edu.cn

^†

Received Date: 17 January 2025
Revised Date: 3 April 2025
Accepted Date: 7 April 2025

Fund Project: the National Natural Science Foundation of China 52400174the National Natural Science Foundation of China 52270129the National Natural Science Foundation of China 52370142Shanghai Sailing Program 24YF2714000Oriental Talent Youth Program, and Shanghai Shuguang Program 23SG52

Efficient technologies for lithium extraction are progressively pivotal in response to the growing requirement for lithium in new energy applications. However, due to its high energy consumption and possible secondary pollution problems, traditional lithium absorption and recovery technologies, are limited in practical application and development. Capacitive deionization (CDI) demonstrates significant potential for lithium extraction with regard to efficiency, cost-effectiveness, and energy consumption. This review commences with bibliometric analysis to dissect the key research topics of lithium extraction via CDI, and presents a complete synopsis of recent advances in electrode materials for lithium extraction using CDI technology, along with various types of CDI systems that utilize these materials. This study elucidates in detail the main electrode materials used in CDI systems for lithium resource recovery——aqueous lithium ion electrode materials (including LiFePO₄, LiMn₂O₄, LiNi_1/3Co_1/3Mn_1/3O₂) and their modification materials (including carbon nanotubes, graphene, MOFs). In addition, this paper discusses the improvement of lithium extraction efficiency through different CDI systems and evaluates the capability of various advanced electrode materials in these systems. The end of the paper emphasizes the application potential of machine learning in the domain of lithium extraction via CDI. The study is anticipated to deliver a strong theoretical basis and practical recommendations for advancing efficient lithium extraction systems that utilize CDI.
- Capacitive deionization,
- Lithium extraction,
- Electrochemical,
- Electrode material
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