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中空结构光催化剂

刘方璇 ,  刘子妍 ,  周国伟 ,  高婷婷 ,  刘文宇 ,  孙彬

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引用本文: 刘方璇, 刘子妍, 周国伟, 高婷婷, 刘文宇, 孙彬. 中空结构光催化剂[J]. 物理化学学报, 2025, 41(7): 100071. doi: 10.1016/j.actphy.2025.100071 shu
Citation:  Fangxuan Liu, Ziyan Liu, Guowei Zhou, Tingting Gao, Wenyu Liu, Bin Sun. Hollow structured photocatalysts[J]. Acta Physico-Chimica Sinica, 2025, 41(7): 100071. doi: 10.1016/j.actphy.2025.100071 shu

中空结构光催化剂

  • 1.

    齐鲁工业大学(山东省科学院)化学与化工学院, 山东省高校轻工精细化学品重点实验室, 济南市多尺度功能材料工程实验室, 山东 济南 250353

  • 2.

    烟台先进材料与绿色制造山东省实验室, 山东 烟台 264006

  • 3.

    齐鲁工业大学(山东省科学院)机械工程学院, 山东 济南 250353

    • 通讯作者: 周国伟, gwzhou@qlu.edu.cn; 孙彬, binsun@qlu.edu.cn
  • 基金项目:

    国家自然科学基金 52202102

    国家自然科学基金 52472215

    国家自然科学基金 52202007

    国家自然科学基金 51972180

    山东省自然科学基金 ZR2019BB030

    山东省自然科学基金 ZR2021QE282

    山东省重点研发计划 2024TSGC0222

    山东省高等学校青年创新团队发展计划 2021KJ056

    烟台先进材料与绿色制造山东省实验室开放基金 AMGM2023F13

    烟台先进材料与绿色制造山东省实验室开放基金 AMGM2021F05

    齐鲁工业大学(山东省科学院)科教产融合试点工程重大创新类项目 2024ZDZX13

摘要: 利用太阳能驱动的光催化技术，有望成为缓解环境和能源压力的可行策略。因此，光催化性能的优异与否取决于光催化剂的合理设计。通过考虑形貌调控、带隙工程、助催化剂修饰以及异质结构建等因素，可以开发出性能优异的光催化剂。基于中空结构光催化剂独特特性的启发，具有中空结构的光催化剂在光催化剂设计中赋予了诸多优势，包括增强光的多重折射和反射、缩短光生载流子的传输距离以及提供丰富的表面反应位点。在此，我们系统地回顾了中空结构光催化剂的最新研究进展，并总结了其几何形貌、内部结构和化学成分的多样性。具体而言，我们重点介绍了中空结构光催化剂的合成策略，包括硬模板法、软模板法和无模板法。此外，还详细总结了一系列中空结构光催化剂，如金属氧化物、金属硫化物、金属有机框架和共价有机框架等。随后，我们概述了中空结构光催化剂在光催化污染物降解、H2生成、H2O2生成、CO2还原和N2固定等领域的潜在应用。同时，深入探讨了中空结构与光催化性能之间的内在关系。最后，我们分析了中空结构光催化剂未来发展方向中的挑战和前景。该综述为更好地设计中空结构光催化剂以满足环境修复和能源转换需求提供了启示。

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