Citation: Xue Liu, Lipeng Wang, Luling Li, Kai Wang, Wenju Liu, Biao Hu, Daofan Cao, Fenghao Jiang, Junguo Li, Ke Liu. Research on Cu-Based and Pt-Based Catalysts for Hydrogen Production through Methanol Steam Reforming[J]. Acta Physico-Chimica Sinica, ;2025, 41(5): 100049. doi: 10.1016/j.actphy.2025.100049 shu

Research on Cu-Based and Pt-Based Catalysts for Hydrogen Production through Methanol Steam Reforming

Xue Liu ¹ ,
Lipeng Wang ¹ ,
Luling Li ² ,
Kai Wang ³ ,
Wenju Liu ¹ ,
Biao Hu ¹ ,
Daofan Cao ² ,
Fenghao Jiang ¹ ,
Junguo Li ¹ ,
Ke Liu ^{1, 4,,}

1.
Department of Chemistry, College of Science, Southern University of Science and Technology, Shenzhen 518055, Guangdong Province, China
2.
Shenzhen Gas Group Co Ltd. Shenzhen 518000, Guangdong Province, China
3.
Anyang Institute of Technology, Anyang 455099, Henan Province, China
4.
College of Innovation and Entrepreneurship, Southern University of Science and Technology, Shenzhen 518055, Guangdong Province, China

Corresponding author: Ke Liu, liuk@sustech.edu.cn
Received Date: 18 November 2024
Revised Date: 13 December 2024
Accepted Date: 20 December 2024

Fund Project: Shenzhen Science and Technology Innovation Committee KQTD20180411143418361Southern University of Science and Technology, Guangdong Provincial Key Laboratory of Catalysis 2020B121201002Key Scientific Research Project of Colleges and Universities in Henan Province 24B530001National Natural Science Foundation of China U22B20149

Methanol steam reforming (MSR) is a critical pathway for on-board hydrogen production from methanol, playing a significant role in clean energy applications. The catalytic performance in MSR reactions directly influences hydrogen yield and byproduct composition, with Cu-based and Pt-based catalysts extensively studied for their high efficiency. The catalytic mechanism primarily involves the cleavage of C―H and O―H bonds in methanol and water molecules. The activity of Cu-based catalysts depends on the ratio and synergistic interaction of Cu⁰ and Cu⁺ active sites, while Pt-based catalysts operate through Pt⁰, Pt^δ+ or Pt²⁺ active sites, in conjunction with oxygen vacancies. However, the electron transfer and interaction mechanisms between active metals and supports remain contentious, impacting the metal oxidation states, adsorption sites, and reaction pathway selectivity. This is particularly evident in the pathways for methanol dehydrogenation and intermediate product formation (e.g., formaldehyde, formic acid, and methyl formate), which lack a unified understanding. This review systematically examines the unitary and synergistic roles of Cu⁰ and Cu⁺ sites, explores the direct and synergistic pathways of Pt-based catalysts, and analyzes the effects of additives such as In₂O₃ on Pt site modulation and oxygen vacancy generation. By integrating catalytic performance evaluations with mechanistic insights, strategies are proposed to enhance catalyst activity and stability. This comprehensive review not only advances the understanding of MSR mechanisms but also provides a theoretical foundation and research direction for the development of high-performance catalysts for on-board hydrogen production.
- Hydrogen production of methanol steam reforming,
- Cu-based and Pt-Based catalysts,
- Active sites,
- Synergies,
- Reaction pathways
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沈阳化工大学材料科学与工程学院沈阳 110142