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Citation: Zhenxing Zeng, Kexin Li, Kai Wei, Yuhua Dai, Liushui Yan, Huiqin Guo, Xubiao Luo. Fabrication of highly dispersed platinum-deposited porous g-C₃N₄ by a simple in situ photoreduction strategy and their excellent visible light photocatalytic activity toward aqueous 4-fluorophenol degradation[J]. Chinese Journal of Catalysis, ;2017, 38(1): 29-38. doi: 10.1016/S1872-2067(16)62589-5 shu

Fabrication of highly dispersed platinum-deposited porous g-C₃N₄ by a simple in situ photoreduction strategy and their excellent visible light photocatalytic activity toward aqueous 4-fluorophenol degradation

Key Laboratory of Jiangxi Province for Persistent Pollutants Control and Resources Recycle, Nanchang Hangkong University, Nanchang 330063, Jiangxi, China

Received Date: 17 September 2016
Revised Date: 6 November 2016

Fund Project: This work was supported by the National Natural Science Foundation of China (51568049, 51208248, 51468043, 21366024), the National Science Fund for Excellent Young Scholars (51422807), the Natural Science Foundation of Jiangxi Province, China (20161BAB206118, 20114BAB213015), and the Natural Science Foundation of Jiangxi Provincial Department of Education, China (GJJ14515, GJJ12456).

A series of highly dispersed platinum-deposited porous g-C₃N₄ (Pt/pg-C₃N₄) were successfully fab-ricated by a simple in situ photoreduction strategy using chloroplatinic acid and porous g-C₃N₄ as precursors. Porous g-C₃N₄ was fabricated by a pretreatment strategy using melamine as a raw ma-terial. The morphology, porosity, phase, chemical structure, and optical and electronic properties of as-prepared Pt/pg-C₃N₄ were characterized. The photocatalytic activity of as-prepared Pt/pg-C₃N₄ was preliminarily evaluated by the degradation of aqueous azo dyes methyl orange under visible light irradiation. The as-prepared Pt/pg-C₃N₄ were further applied to the degradation and mineral-ization of aqueous 4-fluorophenol. The recyclability of Pt/pg-C₃N₄ was evaluated under four con-secutive photocatalytic runs.
- Photocatalysis,
- Porous graphitic carbon nitride,
- Photoreduction,
- Platinum deposition,
- 4-Fluorophenol
1. [1]
2. [2]
3. [3]
4. [4]
5. [5]
6. [6]
7. [7]
8. [8]
9. [9]
10. [10]
11. [11]
12. [12]
13. [13]
14. [14]
15. [15]
16. [16]
17. [17]
18. [18]
19. [19]
20. [20]
21. [21]
22. [22]
23. [23]
24. [24]
25. [25]
26. [26]
27. [27]
28. [28]
29. [29]
30. [30]
31. [31]
1. [1]
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Fabrication of highly dispersed platinum-deposited porous g-C3N4 by a simple in situ photoreduction strategy and their excellent visible light photocatalytic activity toward aqueous 4-fluorophenol degradation

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通讯作者: 陈斌, bchen63@163.com

Fabrication of highly dispersed platinum-deposited porous g-C₃N₄ by a simple in situ photoreduction strategy and their excellent visible light photocatalytic activity toward aqueous 4-fluorophenol degradation