CdS柱撑钛铌酸介孔复合材料的制备与光解水制氢活性

蒋少锋 姚倩茹 高碧芬 陈亦琳 林碧洲

引用本文: 蒋少锋, 姚倩茹, 高碧芬, 陈亦琳, 林碧洲. CdS柱撑钛铌酸介孔复合材料的制备与光解水制氢活性[J]. 无机化学学报, 2015, (3): 514-520. doi: 10.11862/CJIC.2015.077 shu
Citation:  JIANG Shao-Feng, YAO Qian-Ru, GAO Bi-Fen, CHEN Yi-Lin, LIN Bi-Zhou. Preparation of Mesoporous CdS-Pillared Titanoniobate Nanohybrids and Their Photocatalytic Water-Splitting Activity for Hydrogen Generation[J]. Chinese Journal of Inorganic Chemistry, 2015, (3): 514-520. doi: 10.11862/CJIC.2015.077 shu

CdS柱撑钛铌酸介孔复合材料的制备与光解水制氢活性

    通讯作者: 林碧洲 bzlinhqu@126.com, bzlin@hqu.edu.cn
  • 基金项目:

    国家自然科学基金(No.50872037) (No.50872037)

    福建省自然科学基金(No.2014J01187)资助项目。 (No.2014J01187)

摘要: 以钛铌酸纳米片层为主体, CdS纳米颗粒为客体, 通过剥离-重堆积法合成了不同投料比的CdS-TiNbO5介孔复合材料, 材料的层间距为1.19 nm, 比表面积约为93 m2·g-1。CdS-TiNbO5复合材料表现出良好的光解水制氢活性, 当投料比nCdS :nHTiNbO5=1:2时, 复合材料在模拟太阳光和可见光下的产氢速率分别为231和184 μmol·h-1·g-1, 是CdS的8.6和9.7倍。复合材料光催化活性的提高归因于比表面积的增加和光生载流子的有效分离。

English

  • 
    1. [1] Fujishima A. Nature, 1972,238:37-38[1] Fujishima A. Nature, 1972,238:37-38

    2. [2] Chen X B, Shen S H, Guo L J, et al. Chem. Rev., 2010,110: 6503-6570[2] Chen X B, Shen S H, Guo L J, et al. Chem. Rev., 2010,110: 6503-6570

    3. [3] Maeda K, Domen K. J. Phys. Chem. Lett., 2010,1:2655-2661[3] Maeda K, Domen K. J. Phys. Chem. Lett., 2010,1:2655-2661

    4. [4] Teets T S, Nocera D G. Chem. Commun., 2011,47:9268-9274[4] Teets T S, Nocera D G. Chem. Commun., 2011,47:9268-9274

    5. [5] Fan W Q, Zhang Q H, Wang Y. Phys. Chem. Chem. Phys., 2013,15:2632-2649[5] Fan W Q, Zhang Q H, Wang Y. Phys. Chem. Chem. Phys., 2013,15:2632-2649

    6. [6] Kudo A, Miseki Y. Chem. Soc. Rev., 2009,38:253-278[6] Kudo A, Miseki Y. Chem. Soc. Rev., 2009,38:253-278

    7. [7] Takagaki A, Tagusagawa C, Hayashi S, et al. Energy Environ. Sci., 2010,3:82-93[7] Takagaki A, Tagusagawa C, Hayashi S, et al. Energy Environ. Sci., 2010,3:82-93

    8. [8] Inoue K, Suzuki S, Nagai M. J. Electroceram, 2008,24:110-114[8] Inoue K, Suzuki S, Nagai M. J. Electroceram, 2008,24:110-114

    9. [9] Fan X R, Lin B Zh, Liu H, et al. Int. J. Hydrogen Energy, 2013,38:832-839[9] Fan X R, Lin B Zh, Liu H, et al. Int. J. Hydrogen Energy, 2013,38:832-839

    10. [10] Zhang L H, Hu C H, Zhang J F, et al. Chem. Commun., 2013,49:7507-7509[10] Zhang L H, Hu C H, Zhang J F, et al. Chem. Commun., 2013,49:7507-7509

    11. [11] Zhai Z, Huang Y C, Xu L, et al. Nano Res., 2011,4:635-647[11] Zhai Z, Huang Y C, Xu L, et al. Nano Res., 2011,4:635-647

    12. [12] Lin H Y, Chang Y S. Int. J. Hydrogen Energy, 2014,39: 3118-3126[12] Lin H Y, Chang Y S. Int. J. Hydrogen Energy, 2014,39: 3118-3126

    13. [13] Pergentino O, de Brito M M, Andrade H M C, et al. J. Catal., 2014,2014:1-8[13] Pergentino O, de Brito M M, Andrade H M C, et al. J. Catal., 2014,2014:1-8

    14. [14] Fu J, Chang B B, Tian Y L, et al. J. Mater. Chem. A, 2013, 1:3083-3090[14] Fu J, Chang B B, Tian Y L, et al. J. Mater. Chem. A, 2013, 1:3083-3090

    15. [15] Kar A, Kundu S, Patra A. RSC Adv., 2012,2:10222-10230[15] Kar A, Kundu S, Patra A. RSC Adv., 2012,2:10222-10230

    16. [16] ZHANG Yu(张宇), ZHANG Jun-Xiang(张俊祥), FU De-Gang(付德刚), et al. Chin. J. Inorg. Mater.(无机材料学报), 1999,15(5):595-600[16] ZHANG Yu(张宇), ZHANG Jun-Xiang(张俊祥), FU De-Gang(付德刚), et al. Chin. J. Inorg. Mater.(无机材料学报), 1999,15(5):595-600

    17. [17] Zirak M, Akhavan O, Moradlou O, et al. J. Alloys Compd., 2014,590:507-513[17] Zirak M, Akhavan O, Moradlou O, et al. J. Alloys Compd., 2014,590:507-513

    18. [18] Zhai Z, Hu C H, Yang X Y, et al. J. Mater. Chem., 2012, 22:19122-19131[18] Zhai Z, Hu C H, Yang X Y, et al. J. Mater. Chem., 2012, 22:19122-19131

    19. [19] Zhai Z, Yang X Y, Xu L, et al. Nanoscale, 2012,4:547-556[19] Zhai Z, Yang X Y, Xu L, et al. Nanoscale, 2012,4:547-556

    20. [20] Zhu B L, Lin B Z, Zhou Y, et al. J. Mater. Chem. A, 2014, 2:3819-3827[20] Zhu B L, Lin B Z, Zhou Y, et al. J. Mater. Chem. A, 2014, 2:3819-3827

    21. [21] Nan Z, Zhang Y H, Pan X Y, et al. J. Phys. Chem. C, 2011, 115:23501-23511[21] Nan Z, Zhang Y H, Pan X Y, et al. J. Phys. Chem. C, 2011, 115:23501-23511

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  • 收稿日期:  2014-09-29
  • 网络出版日期:  2014-12-03
通讯作者: 陈斌, bchen63@163.com
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