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新型Brönsted酸性离子液体催化二氧化碳与环氧化合物偶联反应

常涛 ,  高晓蕊 ,  边丽 ,  付西英 ,  袁明霞 ,  景欢旺

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引用本文: 常涛, 高晓蕊, 边丽, 付西英, 袁明霞, 景欢旺. 新型Brönsted酸性离子液体催化二氧化碳与环氧化合物偶联反应[J]. 催化学报, 2015, 36(3): 408-413. doi: 10.1016/S1872-2067(14)60227-8 shu
Citation:  Tao Chang, Xiaorui Gao, Li Bian, Xiying Fu, Mingxia Yuan, Huanwang Jing. Coupling of epoxides and carbon dioxide catalyzed by Brönsted acid ionic liquids[J]. Chinese Journal of Catalysis, 2015, 36(3): 408-413. doi: 10.1016/S1872-2067(14)60227-8 shu

新型Brönsted酸性离子液体催化二氧化碳与环氧化合物偶联反应

    通讯作者: 常 涛, 景欢旺
  • 基金项目:

    河北省自然科学基金(B2012402001) (B2012402001)

    国家自然科学基金(51202054, 21173106). (51202054, 21173106)

摘要: 设计合成了一系列由碳链长度可调节的Brönsted酸中心阳离子及Lewis碱中心阴离子构成的酸性离子液体, 并应用于二氧化碳与环氧化合物的偶联反应合成环碳酸酯.考察了离子液体结构以及温度、压力和催化剂用量等参数的影响.结果表明, 具有长碳链的离子液体表现出高催化活性及可重复使用性能.离子液体的酸性影响催化活性.

English

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  • 发布日期:  2015-03-20
  • 收稿日期:  2014-08-11
  • 网络出版日期:  2014-09-15
通讯作者: 陈斌, bchen63@163.com
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