Citation: Wang Zhe, Zhao Zhixi. Research Advances of the Adsorption-Desorption Mechanism in Arsenic Mobilization and Retention[J]. Chemistry, ;2020, 83(1): 23-29. shu

Research Advances of the Adsorption-Desorption Mechanism in Arsenic Mobilization and Retention

Wang Zhe ,
Zhao Zhixi ^,

College of Chemistry and Chemical Engineering, Xinjiang Normal University, Urumqi, 830054

Corresponding author: Zhao Zhixi, zhixizhao@qq.com
Received Date: 14 August 2019
Accepted Date: 6 November 2019

Figures(1)

High arsenic pollution in groundwater is a global environmental issue. Under specific geological, geomorphological, climatic and hydrological and hydrochemical conditions, arsenic-containing minerals undergo adsorption and desorption reactions. Therefore the arsenic was released into groundwater and caused the formation of high arsenic groundwater. Based on the previous researches, the mechanism of adsorption-desorption during arsenic migration and intention in groundwater was analyzed and summarized. Effects of competitive adsorption, redox, pH and organic matter on arsenic adsorption-desorption were discussed from the aspects of adsorbate and adsorbent. Three mechanisms on arsenic adsorption-desorption, i.e. electrostatic attraction mechanism, ion exchange mechanism and complexation species mechanism, were summarized. This paper can provide useful help for revealing the mechanism of high arsenic groundwater and conducting arsenic pollution control and treatment.
- Arsenic,
- Adsorption-desorption,
- Electrostatic attraction,
- Ion exchange,
- Complexation species
1. [1]
  Zhao H S, Stanforth R. Environ. Sci. Technol., 2001, 35(24):4753~4757.
2. [2]
  Acharyya S K, Chakraborty P, Lahiri S, et al. Nature, 1999, 401(6753):545~547.
3. [3]
  Appelo C A J, Tournassat C, Charlet L, et al. Environ. Sci. Technol., 2002, 36(14):3096~3103.
4. [4]
  Anawar H M, J Akai, H Sakugawa. Chemosphere, 2004, 54(6):753~762.
5. [5]
  Radu T, Subacz J L, Phillippi J M, et al. Environ. Sci. Technol., 2005, 39(20):7875~7882.
6. [6]
  Christl I, Brechbühl Y, Graf M, et al. Environ. Sci. Technol., 2012, 46(24):13235~13243.
7. [7]
  Xu H, Allard B, Grimvall A. Water Air Soil Pollut., 1988, 40(3-4):293~305.
8. [8]
  Myneni S C B, Traina S J, Logan T J, et al. Environ. Sci. Technol., 1997, 31(6):1761~1768.
9. [9]
  Horneman A, Geen A V, Kent D V, et al. Geochim. Cosmochim. Acta, 2004, 68(17):3459~3473.
10. [10]
  Handler R M, Beard B L, Johnson C M, et al. Environ. Sci. Technol., 2009, 43(4):1102~1107.
11. [11]
  Mohan D, Pittman C U. J. Hazard. Mater., 2007, 142(1):1~53.
12. [12]
  Tufano K J, Reyes C, Saltikov C W, et al. Environ. Sci. Technol., 2008, 42(22):8283~8289.
13. [13]
  Manning B A, Goldberg S. Environ. Sci. Technol., 1997, 31(7):2005~2011.
14. [14]
  Smedley P L, Kinniburgh D G A. Appl. Geochem., 2002, 17(5):517~568.
15. [15]
  Charlet L, Chakraborty S,Appelo C A J, et al. Appl. Geochem., 2007, 22(7):1273~1292.
16. [16]
  Stollenwerk K G. Arsenic in Ground Water, 2003, Springer, Boston, MA:67~100.
17. [17]
  Takahash Yi, Mina Yi, Ambe S, et al. Geochim. Cosmochim. Acta, 1999, 63(6):815~836.
18. [18]
  Grafe M. Virginia:Virginia Polytechnic Institute and State University, 2001.
19. [19]
  Grafe M, Eick M J, Grossl P R, et al. J. Environ. Qual., 2002, 31(4):1115~1123.
20. [20]
  Redman A D, Macalady D L, Ahmann D. Environ. Sci. Technol., 2002, 36(13):2889~2896.
21. [21]
  de Oliveira L K, de Almeida Melo C, Fraceto L F, et al. Environ. Sci. Pollut. Res., 2016, 23(7):6205~6216.
22. [22]
  Mukhopadhyay R, Manjaiah K M, Datta S C, et al. J. Hazard. Mater., 2019, 377:124~131.
23. [23]
  Deng Y X, Weng L P, Li Y T, et al. Water Res., 2019, 157:372~380.
24. [24]
  Ying S C, Kocar B D, Fendorf S. Geochim. Cosmochim. Acta, 2012, 96(11):294~303.
25. [25]
  Li F H, Geng D, Cao Q. Desalin. Water Treat., 2015, 56(7):1829~1838.
26. [26]
27. [27]
  Welch A H, Westjohn D B, Helsel D R, et al. Groundwater, 2000, 38(4):589~604.
28. [28]
  Corwin D L, David A, Goldberg S. J. Contam. Hydrol., 1999, 39(1-2):35~58.
29. [29]
  Chowdhury T R, Basu G K, Mandal B K, et al. Nature, 1999, 401(6753):545~546.
30. [30]
  Swartz C H, Blute N K, Badruzzman B, et al. Geochim. Cosmochim. Acta, 2004, 68(22):4539~4557.
31. [31]
  Harvey C F, Swartz C H, Badruzzaman A B M, et al. Science, 2002, 298(5598):1602~1606.
32. [32]
  Savage K S, Tingle T N, O'Day P A, et al. Appl. Geochem., 2000, 15(8):1219~1244.
33. [33]
34. [34]
35. [35]
36. [36]
37. [37]
  Mikutta R, Lorenz D, Guggenberger G, et al. Geochim. Cosmochim. Acta, 2014, 144:258~276.
38. [38]
39. [39]
  Chen Y, Huang W G, Zha D J, et al. Hearing Res., 2007, 226(1):178~182.
40. [40]
41. [41]
42. [42]
  Jain C K, Ali I. Water Res., 2000, 34(17):4304~4312.
43. [43]
44. [44]
  Yang M Q, He J H, Hu M Z, et al. Sens. Actuat. B, 2015, 213:59~64.
45. [45]
  Pena M E, Korfiatis G P, Patal M, et al. Water Res., 2005, 39(11):2327~2337.
46. [46]
47. [47]
  Jain A, Raven K P, Loeppert R H. Environ. Sci. Technol., 1999, 33(8):1179~1184.
48. [48]
49. [49]
50. [50]
  Pecini E M, Springer V, Brigante M, et al. J. Environ. Chem. Eng., 2017, 5(5):4917~4922.
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