Citation: Xu Zi-Yue, Luo Yi, Wang Hui, Zhang Dan-Wei, Li Zhan-Ting. Porous Organic Polymers as Heterogeneous Catalysts for Visible Light-Induced Organic Transformations[J]. Chinese Journal of Organic Chemistry, ;2020, 40(11): 3777-3793. doi: 10.6023/cjoc202003070 shu

Porous Organic Polymers as Heterogeneous Catalysts for Visible Light-Induced Organic Transformations

Department of Chemistry, Fudan University, Shanghai 200438

Corresponding author: Zhang Dan-Wei, zhangdw@fudan.edu.cn Li Zhan-Ting, ztli@fudan.edu.cn
Received Date: 31 March 2020
Revised Date: 22 April 2020
Available Online: 30 April 2020
Fund Project: the National Natural Science Foundation of China 21890732the National Natural Science Foundation of China 21921003Project supported by the National Natural Science Foundation of China (Nos. 21890732, 21890730, 21921003)the National Natural Science Foundation of China 21890730

Figures(19)

The recent applications of porous organic polymers (POPs) as heterogeneous catalysts for visible light-induced organic transformations are summarized. POPs are constructed from conjugated organic monomers, having the features of convenient synthesis and characterization, high stability for quick recovery and reuse, structural diversity as well as high modifiability. POPs possess rigid conjugated frameworks, relatively large surface areas, tunable porosity and typically insoluble in water or organic solvents, and thus ideal platforms for the development of heterogeneous catalysts. Through incorporating conjugated sensitizer units into the backbones or attaching the sensitizers to the backbone linkers, POPs can be developed as efficient heterogeneous photocatalysts for visible light-induced organic transformations. Due to their high stability and insolubility, POP catalysts can be easily recovered through filtration or centrifugation and recycled. POP-based photocatalysis combines visible light utility and catalyst recycling and thus represents a green and sustainable technique.
- porous organic polymer,
- photocatalysis,
- heterogeneous catalysis,
- organic transformation,
- sustainability,
- green chemistry
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沈阳化工大学材料科学与工程学院沈阳 110142