Citation: Zhou Cong, Li Miao, Yu Jintao, Sun Song, Cheng Jiang. Recent Progress in the Carboxylation/Cyclization Reactions Using Carbon Dioxide as the C1 Source[J]. Chinese Journal of Organic Chemistry, ;2020, 40(8): 2221-2231. doi: 10.6023/cjoc202003039 shu

Recent Progress in the Carboxylation/Cyclization Reactions Using Carbon Dioxide as the C1 Source

School of Petrochemical Engineering, Changzhou University, Changzhou, Jiangsu 213164

Corresponding author: Sun Song, sunsong@cczu.edu.cn Cheng Jiang, chengjiang@cczu.edu.cn
Received Date: 15 March 2020
Revised Date: 13 May 2020
Available Online: 15 May 2020
Fund Project: the National Natural Science Foundation of China 21602019the Jiangsu Key Laboratory of Advanced Catalytic Materials & Technology BM2012110the National Natural Science Foundation of China 21971025Project supported by the National Natural Science Foundation of China (Nos. 21602019, 21971025), the Jiangsu Key Laboratory of Advanced Catalytic Materials & Technology (No. BM2012110) and the Advanced Catalysis and Green Manufacturing Collaborative Innovation Center

Figures(24)

Carbon dioxide is a readily available, low-cost, abundant, non-toxic C1 source, which can potentially serve as an ideal building block in synthetic chemistry. Recently, much progress, expecially multi-component reactions (MCRs) has been achieved in construction of carbonyl-containing heterocycles through annulation by using carbon dioxide as carbonyl/carboxyl source. Herein, the advances on the annulation reaction of atmospheric CO₂ with N-, and O-nucleophiles for the constructioin of various carbonyl-containing heterocycles, including benzoxazin, cyclic carbamates, lactams, oxazolidine-2, 4-diones are reviewed. In addition, the carboxylation of C-nucleophiles with CO₂ toward carboxylic acids is also summarized.
- carbon dioxide,
- multicomponent reaction,
- annulation,
- carboxylic acid,
- heterocycle
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