Citation: Liu Lifen, Zhang Xiao, Xie Xin, Li Ruihan, Gao Congjie. Modification of Polyimide-Urethane Reverse Osimosis Composite Membrane Based on NaA Zeolite[J]. Chinese Journal of Organic Chemistry, ;2018, 38(11): 3127-3136. doi: 10.6023/cjoc201806027 shu

Modification of Polyimide-Urethane Reverse Osimosis Composite Membrane Based on NaA Zeolite

Liu Lifen ^a,b,, ,
Zhang Xiao ^a ,
Xie Xin ^a ,
Li Ruihan ^a ,
Gao Congjie ^a,b

a.
Center for Membrane and Water Science and Technology, Ocean College, Zhejiang University of Technology, Hangzhou 310014
b.
Collaborative Innovation Center of Membrane Separation and Water Treatment of Zhejiang Province, Hangzhou 310014

Corresponding author: Liu Lifen, lifenliu@zjut.edu.cn
Received Date: 19 June 2018
Revised Date: 26 June 2018
Available Online: 29 November 2018
Fund Project: the National Key Research and Development Program of China 2016YFC0401508the Open Research Fund Program of Collaborative Innovation Center of Membrane Separation and Water Treatment of Zhejiang Province 2015the National Basic Research Program of China 2015CB655303Project supported by the National Natural Science Foundation of China (No. 21776253 & 21774077), the National Key Research and Development Program of China (No. 2016YFC0401508), the National Basic Research Program of China (No. 2015CB655303) and the Open Research Fund Program of Collaborative Innovation Center of Membrane Separation and Water Treatment of Zhejiang Province (No. 2015)the National Natural Science Foundation of China 21774077the National Natural Science Foundation of China 21776253

Figures(9)

A polyimide-urethane reverse osmosis (RO) composite membrane (MMPD-CFIC@CFIC-DMMPD) was prepared through the reaction of N, N'-dimethyl-m-phenylenediamine (DMMPD) and 4-methyl-phenylenediamine (MMPD) with 5-choroformyloxyisophaloyl chloride (CFIC) via two-step interfacial polymerization method, and this membrane exhibits good oxidation resistance. Then, this MMPD-CFIC@CFIC-DMMPD membrane was further modified with NaA zeolite by doping in the CFIC organic phase. The chemical structure of membrane active layer was examined by the attenuated total reflectance infrared (ATR-IR) and X-ray photoelectronic spectroscopy (XPS). The membrane surface and cross-section morphologies were observed with scanning electronic microscopy (SEM), atomic force microscope (AFM) and transmission electron microscopy (TEM), and the hydrophicity of membrane surface was evaluated by contact angle. Moreover, the separation performance, chlorine resistance and organic foulant resistance properties of the two membranes were systematically investigated. The results showed that the modified polyimide-urethane RO membrane (MMPD-CFIC/NaA@CFIC-DMMPD) presented higher water flux, better organic foulant resistance performance as well as favourite chlorine resistance property than the origin MMPD-CFIC@CFIC-DMMPD membrane due to the incorporating of NaA nanoparticles into the membrane.
- polyimide-urethane,
- reverse osmosis composite membrane,
- NaA zeolite,
- high water flux,
- foulant resistance,
- chlorine resistance
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