Citation: Kexin Dong, Chuqi Shen, Ruyu Yan, Yanping Liu, Chunqiang Zhuang, Shijie Li. Integration of Plasmonic Effect and S-Scheme Heterojunction into Ag/Ag₃PO₄/C₃N₅ Photocatalyst for Boosted Photocatalytic Levofloxacin Degradation[J]. Acta Physico-Chimica Sinica, ;2024, 40(10): 231001. doi: 10.3866/PKU.WHXB202310013 shu

Integration of Plasmonic Effect and S-Scheme Heterojunction into Ag/Ag₃PO₄/C₃N₅ Photocatalyst for Boosted Photocatalytic Levofloxacin Degradation

1.
Key Laboratory of Health Risk Factors for Seafood of Zhejiang Province, National Engineering Research Center for Marine Aquaculture, Zhejiang Ocean University, Zhoushan 316022, Zhejiang Province, China;
2.
Institute of Microstructure and Property of Advanced Materials, Faculty of Materials and Manufacturing, Beijing University of Technology, Beijing 100124, China

Corresponding author: Shijie Li, lishijie@zjou.edu.cn
Received Date: 16 October 2023
Revised Date: 15 November 2023
Accepted Date: 15 November 2023

Fund Project: This work was supported by the National Natural Science Foundation of China (U1809214), Natural Science Foundation of Zhejiang Province of China (LY20E080014, LTGN23E080001), and Science and Technology Project of Zhoushan of China (2022C41011).

The escalating presence of pharmaceutical antibiotics in natural water poses an overwhelming threat to the sustainable development of society. Photocatalysis technology stands out as a promising and cutting-edge environmental purification alternative. C₃N₅, identified as a distinctive nonprecious nonmetal photocatalyst, holds potential for environmental protection. However, challenges persist originating from the sluggish photoreaction kinetics and severe photo-carrier reunion. Currently, the design of a special S-scheme photosystem proves to be a reliable strategy for obtaining outstanding photocatalysts. In this context, a plasmonic S-scheme photosystem involving Ag/Ag₃PO₄/C₃N₅ was developed through a feasible route. The compactly connected 0D/0D/2D Ag/Ag₃PO₄/C₃N₅ heterostructure, benefitting from the synergy between the plasmonic effect and the S-scheme junction, facilitates the efficient utilization of appreciably reinforced sunlight absorption, effective photo-carrier disassociation, and notable photoredox capacity. Consequently, this system generates ·OH and ·O₂^- effectively. Ag/Ag₃PO₄/C₃N₅ demonstrates a superb photocatalytic levofloxacin eradication rate of 0.0362 min^-1, marking a substantial advancement of 24.8, 1.1, and 0.7 folds compared to C₃N₅, Ag₃PO₄, and Ag₃PO₄/C₃N₅, respectively. Impressively, Ag/Ag₃PO₄/C₃N₅ delivers remarkable anti-interference performance and reusability. This achievement signifies a significant step toward developing potent C₃N₅-involved photosystems for environmental purification.
- Plasmonic effect,
- C₃N₅,
- S-scheme heterojunction,
- Synergistic effect,
- Antibiotic removal,
- Internal electric field
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通讯作者: 陈斌, bchen63@163.com

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沈阳化工大学材料科学与工程学院沈阳 110142

Integration of Plasmonic Effect and S-Scheme Heterojunction into Ag/Ag3PO4/C3N5 Photocatalyst for Boosted Photocatalytic Levofloxacin Degradation

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通讯作者: 陈斌, bchen63@163.com

Integration of Plasmonic Effect and S-Scheme Heterojunction into Ag/Ag₃PO₄/C₃N₅ Photocatalyst for Boosted Photocatalytic Levofloxacin Degradation