Toward Practical Lithium-Air Batteries by Avoiding Negative Effects of CO2

Tianjie Wang Yaowei Wang Yuhui Chen Jianpeng Liu Huibing Shi Limin Guo Zhiwei Zhao Chuntai Liu Zhangquan Peng

Citation:  Tianjie Wang, Yaowei Wang, Yuhui Chen, Jianpeng Liu, Huibing Shi, Limin Guo, Zhiwei Zhao, Chuntai Liu, Zhangquan Peng. Toward Practical Lithium-Air Batteries by Avoiding Negative Effects of CO2[J]. Acta Physico-Chimica Sinica, 2022, 38(8): 2009071-0. doi: 10.3866/PKU.WHXB202009071 shu

锂-空气电池的实用化之路:规避二氧化碳负面效应

    作者简介:

    Yuhui Chen obtained his Bachelor degree in Fudan University in 2009, and received his Ph.D. degree from University of St Andrews (United Kingdom) in 2014. Later, he worked with Prof. Peter Bruce at the University of Oxford (United Kingdom) on the topic of metal-air batteries. Since 2017, he is the professor at Nanjing Tech University. His research interests include CO2 electrochemical catalysis and novel batteries such as metal-air batteries;


    Limin Guo obtained her MSc and Ph.D. degrees from Changchun Institute of Applied Chemistry (CIAC) in 2004 and 2016, respectively. In 2018 she worked as an assistant professor in Jilin Engineering Normal University and promoted to full professor in 2020. Currently she is a professor in the College of Environment & Chemical Engineering of Dalian Jiaotong University. Her research interests include non-aqueous lithium-ion and lithium-air batteries investigated by the in situ electrochemistry techniques;


    Zhangquan Peng obtained his Bachelor degree in Wuhan University in 1997, and received his MSc and Ph.D. degrees from Changchun Institute of Applied Chemistry (CIAC) in 2000 and 2003, respectively. He continued by working as a postdoctoral researcher at University of Dusseldorf (Germany), University of Aarhus (Denmark) and University of St Andrews (United Kingdom) from 2004 to 2012. From 2012 to 2020, he worked as a principle investigator on the topic of interfacial electrochemistry of various energy storage devices in CIAC. Currently, he is the supervisor of the Laboratory of Advanced Spectro-electrochemistry and Li-ion Batteries, Dalian Institute of Chemical Physics (DICP). His research interests include in situ electrochemistry coupled with theoretical calculation focusing on Li-ion and Li-O2 batteries;
    通讯作者: 陈宇辉, cheny@njtech.edu.cn
    郭丽敏, lmguo@ciac.ac.cn
    彭章泉, zqpeng@dicp.ac.cn
  • 基金项目:

    国家重点研发计划 2016YFB0100100

    国家重点研发计划 2018YFB0104400

    国家自然科学基金 21972055

    国家自然科学基金 21825202

    国家自然科学基金 21575135

    国家自然科学基金 21733012

    国家自然科学基金 51773092

    国家自然科学基金 21975124

    国家自然科学基金 21972133

    英国皇家学会牛顿基金 NAF/R2/180603

摘要: 与其他的锂电池体系相比,锂-空气电池具有最高的理论比能量,被认为有潜力成为终极能量转换和储存装置。目前的锂-空气电池常常使用气体钢瓶提供纯氧气,而非空气中的氧气,这种电池设计极大降低了锂-空气电池的能量密度和实用性。然而,当空气作为锂-空气电池的氧气供给源时,二氧化碳作为杂质会引起严重的副反应,从而降低锂-空气电池的性能。要解决二氧化碳引起的副反应,理解其反应机制至关重要。本文综述了锂-空气电池中有关二氧化碳诱发的化学/电化学反应的研究进展; 总结了可缓解二氧化碳负面效应的有效策略。此外,对二氧化碳选透膜材料和分离技术用于锂-空气电池进行了展望。

English

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  • 发布日期:  2022-08-15
  • 收稿日期:  2020-09-21
  • 接受日期:  2020-10-16
  • 修回日期:  2020-10-15
  • 网络出版日期:  2020-10-22
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