Citation: Nan Zhang, Jianyang Zang, Gang Wang, Taihong Liu. Nonlinear Characterization and Related Photophysics of Two-Photon Absorption[J]. University Chemistry, ;2023, 38(1): 88-96. doi: 10.3866/PKU.DXHX202201037 shu

Nonlinear Characterization and Related Photophysics of Two-Photon Absorption

Key Laboratory of Applied Surface and Colloid Chemistry of Ministry of Education, School of Chemistry and Chemical Engineering, Shaanxi Normal University, Xi'an 710119, China

Corresponding author: Taihong Liu, liuth121@snnu.edu.cn
Received Date: 19 January 2022

Two-photon absorption (2PA) and two-photon excited fluorescence (2PEF) have received extensive attention due to their potential applications in the fields of high-resolution bioimaging, photodynamic therapy, optical power limiting, three-dimensional microfabrication and high-capacity data storage, etc. Innovative preparation of novel 2PA materials involves nonlinear optical characterization, photophysical studies and the underlying structure-property relationships. 2PA and 2PEF feature the characteristics of interdisciplinary and cross-fields. Aiming to prompt the development of 2PA mechanics and guide for designing efficient 2PA materials, we identify several key questions related to the photophysical processes and characterization methods of 2PA. The effect of laser characteristics on the nonlinear results is illustrated based on our research contributions and the future perspective and challenges in this field are also pointed out.
- Two-photon absorption,
- Nonlinear optics,
- Photophysics,
- Fluorescence
1. [1]
  Göppert-Mayer, M. Ann. Phys. 1931, 401 (3), 273.
2. [2]
  Kaiser, W.; Garrett, C. Phys. Rev. Lett. 1961, 7 (6), 229.
3. [3]
  Wenk, W.; Strickler, J.; Webb, W. Science 1990, 248 (4951), 73.
4. [4]
  He, G. S.; Tan, L.-S.; Zheng, Q.; Prasad, P. N. Chem. Rev. 2008, 108 (4), 1245.
5. [5]
  Terenziani, F.; Kantan, C.; Badaeva, E.; Tretiak, S.; Blanchard-Desce, M. Adv. Mater. 2008, 20 (24), 4641.
6. [6]
  Pawlicki, M.; Collins, H. A.; Denning, R. G.; Anderson, H. L. Angew. Chem. Int. Ed. 2009, 48 (18), 3244.
7. [7]
  Pascal, S.; David, S.; Andraud, C.; Maury, O. Chem. Soc. Rev. 2021, 50 (22), 6613.
8. [8]
  Kim, H. M.; Cho, B. R. Chem. Rev. 2015, 115 (11), 5014.
9. [9]
  Price, R. S.; Dubinina, G.; Wicks, G.; Drobizhev, M.; Rebane, A.; Schanze, K. S. ACS Appl. Mater. Interfaces 2015, 7 (20), 10795.
10. [10]
  Olesiak-Banska, J.; Waszkielewicz, M.; Obstarczyk, P.; Samoc, M. Chem. Soc. Rev. 2019, 48, 4087.
11. [11]
  Quah, H. S.; Chen, W.; Schreyer, M. K.; Yang, H.; Wong, W. H.; Ji, W.; Vittal, J. J. Nat. Commun. 2015, 6, 7954.
12. [12]
13. [13]
  Liu, Q.; Liu, T.; Fang, Y. Langmuir 2020, 36 (9), 2155.
14. [14]
  Liu, T.; Liu, X.; Zhang, Y.; Bondar, M. V.; Fang, Y.; Belfield, K. D. Eur. J. Org. Chem. 2018, 2018 (30), 4095.
15. [15]
  Feng, W.; Liu, K.; Zang, J.; Wang, G.; Miao, R.; Ding, L.; Liu, T.; Kong, J.; Fang, Y. ACS Appl. Mater. Interfaces 2021, 13 (24), 28985.
16. [16]
  Allen, T. G.; Benis, S.; Munera, N.; Zhang, J.; Dai, S.; Li, T.; Jia, B.; Wang, W.; Barlow, S.; Hagan, D. J.; et al. J. Phys. Chem. A 2020, 124 (22), 4367.
17. [17]
  Arnoux, C.; Konishi, T.; Elslande, E. V.; Poutougnigni, E.-A.; Mulatier, J.-C.; Khrouz, L.; Bucher, C.; Dumont, E.; Kamada, K.; Andraud, C.; et al. Macromolecules 2020, 53 (21), 9264.
18. [18]
  Rumi, M.; Ehrlich, J. E.; Heikal, A. A.; Perry, J. W.; Barlow, S.; Hu, Z.; McCord-Maughon, D.; Parker, T. C.; Ro1ckel, H.; Thayumanavan, S.; et al. J. Am. Chem. Soc. 2000, 122 (39), 9500.
19. [19]
  Signorini, R.; Ferrante, C.; Pedron, D.; Zerbetto, M.; Cecchetto, E.; Slaviero, M.; Fortunati, I.; Collini, E.; Bozio, R.; Abbotto, A.; et al. J. Phys. Chem. A 2008, 112 (18), 4224.
20. [20]
  Albota, M. A.; Xu, C.; Webb, W. W. Appl. Opt. 1998, 37 (31), 7352.
21. [21]
  Makarov1, N. S.; Drobizhev1, M.; Rebane, A. Opt. Express 2008, 16 (6), 4029.
22. [22]
  Ajami, A.; Husinsky, W.; Ovsianikov, A.; Liska, R. Appl. Phys. B 2018, 124, 142.
23. [23]
  Xu, C.; Webb, W. W. J. Opt. Soc. Am. B 1996, 13 (3), 481.
24. [24]
  Yang, W. J.; Kim, D. Y.; Kim, C. H.; Jeong, M.-Y.; Lee, S. K.; Jeon, S.-J.; Cho, B. R. Org. Lett. 2004, 6 (9), 1389.
25. [25]
  Liu, T.; Bondar, M. V.; Belfield, K. D.; Anderson, D.; Masunov, A. E.; Hagan, D. J.; Van Stryland, E. W. J. Phys. Chem. C 2016, 120 (20), 11099.
26. [26]
  Zang, J.; Feng, W.; Chang, X.; Liu, K.; Peng, H.; Ding, L.; Liu, T.; Fang, Y. Dyes Pigm. 2021, 193, 109487.
27. [27]
  Liu, T.; Liu, X.; Wang, W.; Luo, Z.; Liu, M.; Zou, S.; Sissa, C.; Painelli, A.; Zhang, Y.; Vengris, M.; et al. J. Phys. Chem. C 2018, 122 (7), 3994.
28. [28]
  Feng, W.; Liu, K.; Zang, J.; Xu, J.; Peng, H.; Ding, L.; Liu, T.; Fang, Y. J. Phys. Chem. B 2021, 125 (41), 11540.
29. [29]
30. [30]
  Poo, M.-M.; Du, J.-L.; Ip, N. Y.; Xiong, Z.-Q.; Xu, B. T.; Tan, N. Neuron 2016, 92, 591.
31. [31]
  Amunts, K.; Amunts, K.; Ebell, C.; Muller, J.; Telefont, M.; Knoll, A.; Lippert, T. Neuron 2016, 92, 574.
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