掺杂型碳量子点的制备及其在重金属离子检测中的应用

朱锋利 杨玲 王亚虎 谭海湖

引用本文: 朱锋利, 杨玲, 王亚虎, 谭海湖. 掺杂型碳量子点的制备及其在重金属离子检测中的应用[J]. 分析化学, 2023, 51(1): 22-33. doi: 10.19756/j.issn.0253-3820.221308 shu
Citation:  ZHU Feng-Li,  YANG Ling,  WANG Ya-Hu,  TAN Hai-Hu. Preparation of Doped Carbon Quantum Dots and Its Application in Detection of Heavy Metal Ions[J]. Chinese Journal of Analytical Chemistry, 2023, 51(1): 22-33. doi: 10.19756/j.issn.0253-3820.221308 shu

掺杂型碳量子点的制备及其在重金属离子检测中的应用

    通讯作者: 谭海湖,E-mail:haihutan@163.com
  • 基金项目:

    国家自然科学基金项目(No.51874129)、中国博士后科学基金项目(Nos.2021M693549)、湖南省自然科学基金项目(Nos.2021JJ40178,2021JJ40179,2022JJ50061)和湖南省教育厅科学研究项目(Nos.18A260,20B169,20B181,21C0405)资助。

摘要: 碳量子点(CQDs)具有独特的荧光性质、制备原料来源广泛、合成过程绿色简便、水溶性和生物相容性良好等优点,因而受到广泛关注。CQDs与特定的重金属离子结合后,荧光强度会出现不同程度的增强或减弱,基于此可实现重金属离子的荧光检测。然而,传统的CQDs受限于自身荧光强度不高以及在重金属离子检测中的灵敏度与选择性较差等不足,应用效果并不理想。对CQDs进行杂原子掺杂可调节CQDs中碳原子的电荷密度和自旋密度,提供更多的活性位点,丰富CQDs的能级结构,从而提升其荧光强度。此外,杂原子掺杂可为CQDs引入丰富的官能团,构建易与重金属离子结合的功能界面,从而提高荧光检测的灵敏度。本文综述了近年来氮、硫、磷、锌和铜等原子掺杂CQDs的制备及在重金属离子检测中的研究进展,分析了原子掺杂对CQDs荧光检测性能的影响、原子掺杂CQDs的检测机理、检测应用效果,并展望了其未来的发展方向。

English


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