聚腺嘌呤保护的金纳米团簇与金属有机框架材料ZIF-8复合物的聚集诱导发光增强及用于抗坏血酸的高灵敏荧光检测

曹程程 林祥芳 任晨宇 苏磊

引用本文: 曹程程, 林祥芳, 任晨宇, 苏磊. 聚腺嘌呤保护的金纳米团簇与金属有机框架材料ZIF-8复合物的聚集诱导发光增强及用于抗坏血酸的高灵敏荧光检测[J]. 分析化学, 2022, 50(6): 932-939. doi: 10.19756/j.issn.0253-3820.210807 shu
Citation:  CAO Cheng-Cheng,  LIN Xiang-Fang,  REN Chen-Yu,  SU Lei. Polyadenine-capped Gold Nanoclusters Incorporated into Zeolitic Imidazolate Framework-8 with Aggregation-induced Fluorescence Emission Enhancement for High-Sensitivity Fluorescence Detection of Ascorbic Acid[J]. Chinese Journal of Analytical Chemistry, 2022, 50(6): 932-939. doi: 10.19756/j.issn.0253-3820.210807 shu

聚腺嘌呤保护的金纳米团簇与金属有机框架材料ZIF-8复合物的聚集诱导发光增强及用于抗坏血酸的高灵敏荧光检测

    通讯作者: 苏磊,E-mail:sulei@szu.edu.cn
摘要: 纳米金属有机框架材料(NMOFs)在生物诊断和治疗领域中具有良好的应用前景。本研究建立了一种基于聚腺嘌呤保护的金纳米团簇(PolyA-AuNC)和金属有机框架沸石咪唑酯骨架-8(ZIF-8)纳米复合材料的荧光分析方法,用于血清中抗坏血酸(AA)的高灵敏检测。所制备的纳米复合材料(Poly A-Au NCs@ZIF-8)通过MOF (即ZIF-8)的限制效应显示出聚集诱导的荧光发射增强现象。当AA与ZIF-8作用时,复合材料的骨架被破坏,PolyA-AuNCs从聚集态转变为分散态,导致荧光强度大大降低。将本方法用于AA的检测,线性范围为10~100μmol/L,检出限(LOD,S/N=3)为0.3μmol/L。本方法可在2 min内完成AA的检测,对AA的选择性高。将本方法用于检测人血清中的AA,回收率为95.7%~100.9%。

English


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  • 收稿日期:  2021-10-24
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