Citation: JIANG Hong-Xing, LI Jun, TANG Jiao, MO Yang-Zhi, ZHANG Gan. Applications of High Resolution Mass Spectrometry in Studies of Brown Carbon[J]. Chinese Journal of Analytical Chemistry, ;2018, 46(10): 1528-1538. doi: 10.11895/j.issn.0253-3820.171264 shu

Applications of High Resolution Mass Spectrometry in Studies of Brown Carbon

JIANG Hong-Xing ^1,2, ,
LI Jun ¹ ,
TANG Jiao ^1,2 ,
MO Yang-Zhi ^1,2 ,
ZHANG Gan ¹

1.
State Key Laboratory of Organic Geochemistry, Guangzhou Institute of Geochemistry, Chinese Academy of Sciences, Guangzhou 510640, China;
2.
University of Chinese Academy of Sciences, Beijing 100049, China

Received Date: 21 September 2017
Revised Date: 27 June 2018

Fund Project: This work was supported by the National Natural Science Foundation of China (No.41773120) and the Guangzhou Bureau of Science and Technology and Information, China (No.201504010002).

Brown carbon is one of the hotspots in the field of atmospheric carbonaceous aerosol research. It has significant influence on regional radiative forcing and climatic effects due to its apparent absorbance in the near ultraviolet-visible region. Brown carbon mainly originates from biomass or coal incomplete combustion, and it also comes from some secondary sources, such as a series of atmospheric photochemical reactions from volatile organic compounds (VOCs). Though the composition of the brown carbon is very complex, high resolution mass spectrometry technology provides effective methods for revealing the characteristic of organic components at the molecular level with its ultra-high mass resolution and precision. This paper introduced the application of high resolution mass spectrometry combined with traditional analytical methods in the study of brown carbon:the development of high resolution mass spectrometry for brown carbon separation was reviewed, as well as the composition analysis, source apportionment and formation mechanism of brown carbon based on high resolution data. In addition, the present situation, existing issues and prospects about the application of high resolution mass spectrometry on brown carbon were also discussed.
- Brown carbon,
- High resolution mass spectrometry,
- Light absorption,
- Components,
- Biomass burning,
- Secondary organic aerosol,
- Review
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