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Citation: Xiangyu CAO, Jiaying ZHANG, Yun FENG, Linkun SHEN, Xiuling ZHANG, Juanzhi YAN. Synthesis and electrochemical properties of bimetallic-doped porous carbon cathode material[J]. Chinese Journal of Inorganic Chemistry, ;2025, 41(3): 509-520. doi: 10.11862/CJIC.20240270 shu

Synthesis and electrochemical properties of bimetallic-doped porous carbon cathode material

  • Department of Materials and Chemical Engineering, Taiyuan University, Taiyuan 030032, China

  • Corresponding author: Juanzhi YAN, yanjuanzhi@tyu.edu.cn
  • Received Date: 16 July 2024
    Revised Date: 14 January 2025

Figures(11)

  • A bimetallic (Co, Fe) and nitrogen-doped porous carbon/sulfur composite material (e-CF@NPC/S, CF represents CoFe alloy, NPC represents nitrogen-doped porous carbon) was prepared by hydro-thermal reaction, carbonization, acid etching, and S loading. Then a series of composite materials with different nuclear shell ratios were obtained by changing the ratio of raw materials. The structural analysis and electrochemical properties test results of these composite materials show that core-shell structure porous carbon composite had a rich surface area and space to serve active substance loading and volume changes. The spatial domain restriction of the shell can be helpful to anchor sulfur and polysulfide (LiPSs) inside the structure, however, the shell can also block ion diffusion. The catalytic and absorptive capability of Co-Fe alloy depends on the quantities of active sites. Cathodes of e-CF@NPC-3/S show the best electrochemistry performance with a capacity retention rate of 92.35% at 0.2C after 100 cycles (initial capacity was 996.9 mAh·g-1). After 300 cycles at 1C, it can achieve a capacity decay rate of 0.049% per cycle (initial capacity was 684.5 mAh·g-1).
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