Citation: SHI Mei, YU Min, LIU Guang-Xiang. Syntheses, Crystal Structures and Photoluminescent Properties of Three Zinc(Ⅱ) Coordination Polymers Constructed from 9, 10-Di(1H-imidazol-1-yl)anthracene[J]. Chinese Journal of Inorganic Chemistry, ;2020, 36(12): 2367-2376. doi: 10.11862/CJIC.2020.257 shu

Syntheses, Crystal Structures and Photoluminescent Properties of Three Zinc(Ⅱ) Coordination Polymers Constructed from 9, 10-Di(1H-imidazol-1-yl)anthracene

Nanjing Key Laboratory of Advanced Functional Materials, School of Environmental Science, Nanjing Xiaozhuang University, Nanjing 211171, China

Corresponding author: LIU Guang-Xiang, njuliugx@126.com
Received Date: 3 June 2020
Revised Date: 6 September 2020

Figures(5)

Three zinc(Ⅱ) coordination polymers, [Zn₂(DIA)(bdc)₂]_n (1), {[Zn(DIA)(cdc)]·H₂O}_n (2) and [Zn(DIA)(chdc)]_n (3) (DIA=9, 10-di(1H-imidazol-1-yl)anthracene, H₂bdc=1, 4-benzenedicarboxylic acid, H₂cdc=4, 4'-carbonyldibenzoic acid, H₂chdc=trans-1, 4-cyclohexanedicarboxylic acid), have been synthesized and characterized by IR spectroscopy, elemental analyses, thermogravimetric analyses and single-crystal X-ray diffraction. Structural analyses reveal that complex 1 displays an unprecedented three-dimensional (3D) (4, 7)-connected framework featuring {3².4.5².6} {3².4⁸.5⁴.6⁵.7²}₂ topology. Complex 2 has a two-dimensional (2D) structure, which is further packed into a 3D supramolecular architecture by intermolecular weak interactions, whereas complex 3 features a 2D two-fold interpenetrating layer structure. The results show that the length and the flexibility of the carboxylates exert obvious influence on the resulting architectures. Meanwhile, the photoluminescent properties of three complexes at room temperature were also investigated. CCDC: 1814085, 1; 1814086, 2; 1986966, 3.
- zinc (Ⅱ) coordination polymer,
- bis (imidazole) ligand,
- dicarboxylate,
- crystal structure,
- photoluminescence
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