Citation: WANG Bin, WANG Xiao-Hong, LIU Zhe-Lin, DONG Zhe, WANG Xiao-Hui, UAN Li-Mei, XU Liang, LIU Zong-Rui. Photocatalytic Degradation Activity of Methyl Orange by Composite Catalysts of Surfantant@Polyoxoanions Weakley Type[J]. Chinese Journal of Inorganic Chemistry, ;2020, 36(10): 1865-1872. doi: 10.11862/CJIC.2020.220 shu

Photocatalytic Degradation Activity of Methyl Orange by Composite Catalysts of Surfantant@Polyoxoanions Weakley Type

WANG Bin ^1,2,, ,
WANG Xiao-Hong ¹ ,
LIU Zhe-Lin ³ ,
DONG Zhe ¹ ,
WANG Xiao-Hui ¹ ,
UAN Li-Mei ¹ ,
XU Liang ^1,2 ,
LIU Zong-Rui ^1,,

1.
College of Chemistry and Materials Science, Inner Mongolia University for the Nationalities, Tongliao, Inner Mongolia 028043, China
2.
Key Laboratory of the Natural Products Chemistry and Functional Molecular Synthesis of Autonomous Region, Tongliao, Inner Mongolia 028000, China
3.
School of Chemistry & Environment Engineering, Changchun University of Science and Technology, Changchun 130022, China

Corresponding author: WANG Bin, jluwangbin09@163.com LIU Zong-Rui, liuzr716@163.com
Received Date: 14 March 2020
Revised Date: 22 July 2020

Figures(11)

A series of complexes of surfactant@polyoxoanions were prepared by water/chloroform two-phase electrostatic encapsulating technology, employing polyoxoanion CeW₁₀O₃₆^9- with high photocatalytic activity and cationic surfactants in different structure as building blocks. The composition and structure of the complexes were analyzed by Fourier infrared spectroscopy (FTIR) and thermogravimetric analysis (TGA). The effects of various surfactants, catalyst dosage, concentration of methyl orange, and organic dyes on the photocatalytic degradation rate were investigated, in which methyl orange and surfactant@polyoxoanions complexes were used as photodegradation substrate molecule and photocatalyst, respectively. The photodegradation activities for different composite catalysts of surfac-tant@polyoxoanions are in the order of DTAB (dodecyltrimethylammonium bromide)@CeW₁₀ > TTAB (tetradecyltrimethylammonium bromide)@CeW₁₀ > CTAB (cetyltrimethylammonium bromide)@CeW₁₀ > OTAB (octadecyl trimethyl ammonium bromide)@CeW₁₀ > DODA (dioctadecyl dimethyl ammonium bromide)@CeW₁₀.
- polyoxometalates,
- composite catalyst,
- photocatalytic degradation,
- organic dye
1. [1]
  Chen C C, Ma W H, Zhao J C. Chem. Soc. Rev., 2010, 39(11): 4206-4219 doi: 10.1039/b921692h
2. [2]
  GU Yi-Tong, CHEN Li, LI Jian-Ping, et al. Chinese J. Inorg. Chem., 2019, 35(11):1905-1920 doi: 10.3321/j.issn:1001-4861.1999.03.001
3. [3]
  Wang S S, Yang G Y. Chem. Rev., 2015, 115(11):4893-4962 doi: 10.1021/cr500390v
4. [4]
  Dolbecq A, Mialane P, Keita B, et al. J. Mater. Chem., 2012, 22(47):24509-24521 doi: 10.1039/c2jm33246a
5. [5]
  Troupis A, Gkika E, Hiskia A, et al. J. Adv. Oxid. Technol., 2007, 10(1):79-84 doi: 10.1515/jaots-1996-0209
6. [6]
  WANG Bin, WU Ying-Ga, LIU Zhe-Lin, et al. Chem. J. Chinese Universities, 2018, 39(5):1003-1008 doi: 10.3321/j.issn:0251-0790.2001.04.047
7. [7]
  Liu C G, Zheng T, Liu S, et al. J. Mol. Struct., 2016, 1110:4452 doi: 10.1016/j.molstruc.2004.07.045
8. [8]
  Yan G, Feng X J, Xiao L G, et al. Dalton Trans., 2017, 46(46): 16019-16024 doi: 10.1039/C7DT03372A
9. [9]
  Li Y S, Liu M X, Chen L. J. Mater. Chem. A, 2017, 5(26): 13757-13762 doi: 10.1039/C7TA03776G
10. [10]
  Gao S Y, Cao R, Lv J, et al. J. Mater. Chem., 2009, 19(24): 4157-4163 doi: 10.1039/b903065d
11. [11]
  Liu Y W, Luo F, Liu S M, et al. Small, 2017, 13(14):1603174 doi: 10.1002/smll.201603174
12. [12]
  Liu M, Yang X F, Zhu H B, et al. Dalton Trans., 2018, 47(15):5245-5251 doi: 10.1039/C8DT00366A
13. [13]
  Tao S Y, Wang Y C, Yu Y X, et al. J. Environ. Chem. Eng., 2013, 1(4):719-727 doi: 10.1016/j.jece.2013.07.014
14. [14]
  Zhao L, Chi Y, Yuan Q, et al. J. Colloid Interface Sci., 2013, 390(1):70-77 doi: 10.1016/j.jcis.2008.06.031
15. [15]
  Khoshnavazi R, Fereydouni S, Bahrami L. Water Sci. Technol., 2016, 73(7):1746-1755 doi: 10.2166/wst.2016.008
16. [16]
  Peacock R D, Weakley T J R. J. Chem. Soc. A, 1971:18361839
17. [17]
  AlDamen M A, Cardona-Serra S, Clemente-Juan J M, et al. Inorg. Chem., 2009, 48(8):3467-3479
18. [18]
  Wang Z L, Zhang R L, Ma Y, et al. J. Mater. Chem., 2010, 20(2):271-277
19. [19]
  Yamase T. Chem. Rev., 1998, 98(1):307-326 doi: 10.1039/b712170a
20. [20]
  Yi X Y, Sung H H, Williams L D, et al. Chem. Commun., 2008, 44(28):3269-3271
21. [21]
  Keita B, Lu Y W, Nadjo L, et al. Electrochem. Commun., 2000, 2(10):720-726 doi: 10.1016/S1388-2481(00)00104-1
22. [22]
  Zhang J, Li W, Wu C, et al. Chem. Eur. J., 2013, 19(25):8129 -8135 doi: 10.1002/chem.201300309
23. [23]
  Hiskia A, Mylonasa A, Papaconstantinou E. Chem. Soc.Rev., 2001, 30(1):62-69 doi: 10.1039/A905675K
1. [1]
  Guangming YIN , Huaiyao WANG , Jianhua ZHENG , Xinyue DONG , Jian LI , Yi'nan SUN , Yiming GAO , Bingbing WANG . Preparation and photocatalytic degradation performance of Ag/protonated g-C₃N₄ nanorod materials. Chinese Journal of Inorganic Chemistry, 2024, 40(8): 1491-1500. doi: 10.11862/CJIC.20240086
2. [2]
  Hongbo Zhang , Yihong Tang , Suxia Zhang , Yuanting Li . Electrochemical Monitoring of Photocatalytic Degradation of Phenol Pollutants: A Recommended Comprehensive Analytical Chemistry Experiment. University Chemistry, 2024, 39(6): 326-333. doi: 10.3866/PKU.DXHX202310013
3. [3]
  Xinzhe HUANG , Lihui XU , Yue YANG , Liming WANG , Zhangyong LIU , Zhongjian WANG . Preparation and visible light responsive photocatalytic properties of BiSbO₄/BiOBr. Chinese Journal of Inorganic Chemistry, 2025, 41(2): 284-292. doi: 10.11862/CJIC.20240212
4. [4]
  Xinyu Miao , Hao Yang , Jie He , Jing Wang , Zhiliang Jin . 调整Keggin型多金属氧酸盐电子结构构建S型异质结用于光催化析氢. Acta Physico-Chimica Sinica, 2025, 41(6): 100051-. doi: 10.1016/j.actphy.2025.100051
5. [5]
  Zelong LIANG , Shijia QIN , Pengfei GUO , Hang XU , Bin ZHAO . Synthesis and electrocatalytic CO₂ reduction performance of metal-organic framework catalysts loaded with silver particles. Chinese Journal of Inorganic Chemistry, 2025, 41(1): 165-173. doi: 10.11862/CJIC.20240409
6. [6]
  Xuejie Wang , Guoqing Cui , Congkai Wang , Yang Yang , Guiyuan Jiang , Chunming Xu . 碳基催化剂催化有机液体氢载体脱氢研究进展. Acta Physico-Chimica Sinica, 2025, 41(5): 100044-. doi: 10.1016/j.actphy.2024.100044
7. [7]
  Wenxiu Yang , Jinfeng Zhang , Quanlong Xu , Yun Yang , Lijie Zhang . Bimetallic AuCu Alloy Decorated Covalent Organic Frameworks for Efficient Photocatalytic Hydrogen Production. Acta Physico-Chimica Sinica, 2024, 40(10): 2312014-. doi: 10.3866/PKU.WHXB202312014
8. [8]
  Ke Li , Chuang Liu , Jingping Li , Guohong Wang , Kai Wang . 钛酸铋/氮化碳无机有机复合S型异质结纯水光催化产过氧化氢. Acta Physico-Chimica Sinica, 2024, 40(11): 2403009-. doi: 10.3866/PKU.WHXB202403009
9. [9]
  Ruolin CHENG , Haoran WANG , Jing REN , Yingying MA , Huagen LIANG . Efficient photocatalytic CO₂ cycloaddition over W₁₈O₄₉/NH₂-UiO-66 composite catalyst. Chinese Journal of Inorganic Chemistry, 2024, 40(3): 523-532. doi: 10.11862/CJIC.20230349
10. [10]
  Yaping ZHANG , Tongchen WU , Yun ZHENG , Bizhou LIN . Z-scheme heterojunction β-Bi₂O₃ pillared CoAl layered double hydroxide nanohybrid: Fabrication and photocatalytic degradation property. Chinese Journal of Inorganic Chemistry, 2025, 41(3): 531-539. doi: 10.11862/CJIC.20240256
11. [11]
  Jiahui YU , Jixian DONG , Yutong ZHAO , Fuping ZHAO , Bo GE , Xipeng PU , Dafeng ZHANG . The morphology control and full-spectrum photodegradation tetracycline performance of microwave-hydrothermal synthesized BiVO₄:Yb³⁺,Er³⁺ photocatalyst. Journal of Fuel Chemistry and Technology, 2025, 53(3): 348-359. doi: 10.1016/S1872-5813(24)60514-1
12. [12]
  Qingqing SHEN , Xiangbowen DU , Kaicheng QIAN , Zhikang JIN , Zheng FANG , Tong WEI , Renhong LI . Self-supporting Cu/α-FeOOH/foam nickel composite catalyst for efficient hydrogen production by coupling methanol oxidation and water electrolysis. Chinese Journal of Inorganic Chemistry, 2024, 40(10): 1953-1964. doi: 10.11862/CJIC.20240028
13. [13]
  Kun WANG , Wenrui LIU , Peng JIANG , Yuhang SONG , Lihua CHEN , Zhao DENG . Hierarchical hollow structured BiOBr-Pt catalysts for photocatalytic CO₂ reduction. Chinese Journal of Inorganic Chemistry, 2024, 40(7): 1270-1278. doi: 10.11862/CJIC.20240037
14. [14]
  Jiajie Li , Xiaocong Ma , Jufang Zheng , Qiang Wan , Xiaoshun Zhou , Yahao Wang . Recent Advances in In-Situ Raman Spectroscopy for Investigating Electrocatalytic Organic Reaction Mechanisms. University Chemistry, 2025, 40(4): 261-276. doi: 10.12461/PKU.DXHX202406117
15. [15]
  Jiapei Zou , Junyang Zhang , Xuming Wu , Cong Wei , Simin Fang , Yuxi Wang . A Comprehensive Experiment Based on Electrocatalytic Nitrate Reduction into Ammonia: Synthesis, Characterization, Performance Exploration, and Applicable Design of Copper-based Catalysts. University Chemistry, 2024, 39(6): 373-382. doi: 10.3866/PKU.DXHX202312081
16. [16]
  Juntao Yan , Liang Wei . 2D S-Scheme Heterojunction Photocatalyst. Acta Physico-Chimica Sinica, 2024, 40(10): 2312024-. doi: 10.3866/PKU.WHXB202312024
17. [17]
  Yuanyin Cui , Jinfeng Zhang , Hailiang Chu , Lixian Sun , Kai Dai . Rational Design of Bismuth Based Photocatalysts for Solar Energy Conversion. Acta Physico-Chimica Sinica, 2024, 40(12): 2405016-. doi: 10.3866/PKU.WHXB202405016
18. [18]
  Juan WANG , Zhongqiu WANG , Qin SHANG , Guohong WANG , Jinmao LI . NiS and Pt as dual co-catalysts for the enhanced photocatalytic H₂ production activity of BaTiO₃ nanofibers. Chinese Journal of Inorganic Chemistry, 2024, 40(9): 1719-1730. doi: 10.11862/CJIC.20240102
19. [19]
  Yuchen Zhou , Huanmin Liu , Hongxing Li , Xinyu Song , Yonghua Tang , Peng Zhou . 设计热力学稳定的贵金属单原子光催化剂用于乙醇的高效非氧化转化形成高纯氢和增值产物乙醛. Acta Physico-Chimica Sinica, 2025, 41(6): 100067-. doi: 10.1016/j.actphy.2025.100067
20. [20]
  Bing WEI , Jianfan ZHANG , Zhe CHEN . Research progress in fine tuning of bimetallic nanocatalysts for electrocatalytic carbon dioxide reduction. Chinese Journal of Inorganic Chemistry, 2025, 41(3): 425-439. doi: 10.11862/CJIC.20240201

Get Citation

PDF

XML

Metrics

PDF Downloads(5)
Abstract views(781)
HTML views(131)

通讯作者: 陈斌, bchen63@163.com

1.
沈阳化工大学材料科学与工程学院沈阳 110142