Citation: MA Miao-Miao, LI Mei, KE Fu-Sheng. Fabrication and Properties of Metal-Organic Framework@Mesoporous Composites[J]. Chinese Journal of Inorganic Chemistry, ;2018, 34(9): 1663-1669. doi: 10.11862/CJIC.2018.176 shu

Fabrication and Properties of Metal-Organic Framework@Mesoporous Composites

College of Chemistry and Molecular Sciences, Wuhan University, Wuhan 430072, China

Corresponding author: KE Fu-Sheng, kefs@whu.edu.cn
Received Date: 30 April 2018
Revised Date: 22 May 2018

Figures(6)

Metal-organic framework@mesoporous composites were obtained via introducing H₂BDC into the composite materials Al₂O₃@SBA-15, which was synthesized through vapor-induced internal hydrolysis (VIH) method. The structure of MIL-53@SBA-15 composites was confirmed by combination of different characterization techniques, such as powder X-ray diffraction (PXRD), N₂ adsorption-desorption isotherm test, scanning electron microscopy (SEM) and transmission electron microscopy (TEM). Through dye adsorption experiment, MIL-53@SBA-15 compound demonstrated the best adsorptivity performance of butyl rhodamine B dye compared to SBA-15, MIL-53, and physical mixed samples.
- Al₂O₃@SBA-15 composite,
- MIL-53@SBA-15 composite,
- dye adsorption
1. [1]
  Rosi N L, Eckert J, Eddaoudi M, et al. Science, 2003, 300:1127-1129 doi: 10.1126/science.1083440
2. [2]
  Li J R, Kuppler R J, Zhou H C. Chem. Soc. Rev., 2009, 38:1477-1504 doi: 10.1039/b802426j
3. [3]
  Dong Z Y, Sun Y Z S, Chu J, et al. J. Am. Chem. Soc., 2017, 139:14209-14216 doi: 10.1021/jacs.7b07392
4. [4]
  Zhu Q L, Li J, Xu Q. J. Am. Chem. Soc., 2013, 135:10210-10213 doi: 10.1021/ja403330m
5. [5]
  ZHAO Nan, DENG Hong-Ping, SHU Mou-Hai. Chinese J. Inorg. Chem., 2010, 26:1213-1217
6. [6]
  Jiang H Q, Liu X C, Wu Y, et al. Angew. Chem. Int. Ed., 2018, 57:3916-3921 doi: 10.1002/anie.201712872
7. [7]
  Czaja A U, Trukhan N, Müller U. Chem. Soc. Rev., 2009, 38:1284-1293 doi: 10.1039/b804680h
8. [8]
  Zhao D Y, Feng J L, Huo Q S, et al. Science, 1998, 279:548-552 doi: 10.1126/science.279.5350.548
9. [9]
  Zhao D Y, Huo Q S, Feng J L, et al. J. Am. Chem. Soc., 1998, 120:6024-6036 doi: 10.1021/ja974025i
10. [10]
  Kruk M, Jaroniec M, Ko C H, et al. Chem. Mater., 2000, 12:1961-1968 doi: 10.1021/cm000164e
11. [11]
  HAO Shi-You, XIAO Qiang, ZHU Wei-Dong, et al. Chinese J. Inorg. Chem., 2010, 26:982-988
12. [12]
  WEI Qi, ZHONG Zhen-Xing, NIE Zuo-Ren, et al. Chinese J. Inorg. Chem., 2008, 24:130-137 doi: 10.3321/j.issn:1001-4861.2008.01.023
13. [13]
  Li Z, Zeng H C. J. Am. Chem. Soc., 2014, 136:5631-5639 doi: 10.1021/ja409675j
14. [14]
  Wu C M, Rathi M, Ahrenkiel S P, et al. Chem. Commun., 2013, 49:1223-1225 doi: 10.1039/c2cc38366g
15. [15]
  Doherty C M, Buso D, Hill A J, et al. Acc. Chem. Res., 2013, 47:396-405
16. [16]
  Ulker Z, Erucar I, Keskin S, et al. Microporous Mesoporous Mater., 2013, 170:352-358 doi: 10.1016/j.micromeso.2012.11.040
17. [17]
  Zhan G W, Zeng H C. Coord. Chem. Rev., 2016, 320:181-192
18. [18]
  Chakraborty A, Maji T K. APL Mater., 2014, 2:124107(7 Pages) doi: 10.1063/1.4902816
19. [19]
  Cirujano F G, Luz I, Soukri M, et al. Angew. Chem. Int. Ed., 2017, 129:13302-13306 doi: 10.1002/ange.201706893
20. [20]
  Luz I, Soukri M, Lail M. Chem. Mater., 2017, 29:9628-9638 doi: 10.1021/acs.chemmater.7b02042
21. [21]
  Krishnan C K, Hayashi T, Ogura M. Adv. Mater., 2008, 20:2131-2136 doi: 10.1002/(ISSN)1521-4095
22. [22]
  Han Y, Ying J Y. Angew. Chem. Int. Ed., 2005, 117:292-296 doi: 10.1002/(ISSN)1521-3757
23. [23]
  MA Li-Qun, ZHAI Shang-Ru, LIU Na, et al. Prog. Chem., 2012, 24:471-482
24. [24]
  Landau M V, Vradman L, Wang X, et al. Microporous Mesoporous Mater., 2005, 78:117-129 doi: 10.1016/j.micromeso.2004.09.023
25. [25]
  Sauer J, Marlow F, Schüth F. Phys. Chem. Chem. Phys., 2001, 3:5579-5584
26. [26]
  Sauer J, Marlow F, Spliethoff B, et al. Chem. Mater., 2002, 14:217-224 doi: 10.1021/cm0111377
27. [27]
  Li C G, Wang Y Q, Guo Y L, et al. Chem. Mater., 2007, 19:173-178 doi: 10.1021/cm0619151
28. [28]
  Loiseau T, Serre C, Huguenard C, et al. Chem. Eur. J., 2004, 10:1373-1382 doi: 10.1002/(ISSN)1521-3765
29. [29]
  He Y C, Yang J, Kan W Q, et al. J. Mater. Chem. A, 2015, 3:1675-1681 doi: 10.1039/C4TA05391E
1. [1]
  Ping ZHANG , Chenchen ZHAO , Xiaoyun CUI , Bing XIE , Yihan LIU , Haiyu LIN , Jiale ZHANG , Yu'nan CHEN . Preparation and adsorption-photocatalytic performance of ZnAl@layered double oxides. Chinese Journal of Inorganic Chemistry, 2024, 40(10): 1965-1974. doi: 10.11862/CJIC.20240014
2. [2]
  Yaping ZHANG , Tongchen WU , Yun ZHENG , Bizhou LIN . Z-scheme heterojunction β-Bi₂O₃ pillared CoAl layered double hydroxide nanohybrid: Fabrication and photocatalytic degradation property. Chinese Journal of Inorganic Chemistry, 2025, 41(3): 531-539. doi: 10.11862/CJIC.20240256
3. [3]
  Lina Guo , Ruizhe Li , Chuang Sun , Xiaoli Luo , Yiqiu Shi , Hong Yuan , Shuxin Ouyang , Tierui Zhang . 层状双金属氢氧化物的层间阴离子对衍生的Ni-Al₂O₃催化剂光热催化CO₂甲烷化反应的影响. Acta Physico-Chimica Sinica, 2025, 41(1): 2309002-. doi: 10.3866/PKU.WHXB202309002
4. [4]
  Chuanming GUO , Kaiyang ZHANG , Yun WU , Rui YAO , Qiang ZHAO , Jinping LI , Guang LIU . Performance of MnO₂-0.39IrO_x composite oxides for water oxidation reaction in acidic media. Chinese Journal of Inorganic Chemistry, 2024, 40(6): 1135-1142. doi: 10.11862/CJIC.20230459
5. [5]
  Xinyu Yin , Haiyang Shi , Yu Wang , Xuefei Wang , Ping Wang , Huogen Yu . Spontaneously Improved Adsorption of H₂O and Its Intermediates on Electron-Deficient Mn^(3+δ)+ for Efficient Photocatalytic H₂O₂ Production. Acta Physico-Chimica Sinica, 2024, 40(10): 2312007-. doi: 10.3866/PKU.WHXB202312007
6. [6]
  Fei Xie , Chengcheng Yuan , Haiyan Tan , Alireza Z. Moshfegh , Bicheng Zhu , Jiaguo Yu . d带中心调控过渡金属单原子负载COF吸附O₂的理论计算研究. Acta Physico-Chimica Sinica, 2024, 40(11): 2407013-. doi: 10.3866/PKU.WHXB202407013
7. [7]
  Shiyi WANG , Chaolong CHEN , Xiangjian KONG , Lansun ZHENG , Lasheng LONG . Polynuclear lanthanide compound [Ce₄^ⅢCe₆^Ⅳ(μ₃-O)₄(μ₄-O)₄(acac)₁₄(CH₃O)₆]·2CH₃OH for the hydroboration of amides to amine. Chinese Journal of Inorganic Chemistry, 2025, 41(1): 88-96. doi: 10.11862/CJIC.20240342
8. [8]
  Ruolin CHENG , Haoran WANG , Jing REN , Yingying MA , Huagen LIANG . Efficient photocatalytic CO₂ cycloaddition over W₁₈O₄₉/NH₂-UiO-66 composite catalyst. Chinese Journal of Inorganic Chemistry, 2024, 40(3): 523-532. doi: 10.11862/CJIC.20230349
9. [9]
  Youlin SI , Shuquan SUN , Junsong YANG , Zijun BIE , Yan CHEN , Li LUO . Synthesis and adsorption properties of Zn(Ⅱ) metal-organic framework based on 3, 3', 5, 5'-tetraimidazolyl biphenyl ligands. Chinese Journal of Inorganic Chemistry, 2024, 40(9): 1755-1762. doi: 10.11862/CJIC.20240061
10. [10]
  Shasha Ma , Zujin Yang , Jianyong Zhang . Facile Synthesis of FeBTC Metal-Organic Gel and Its Adsorption of Cr₂O₇²⁻: A Physical Chemistry Innovation Experiment. University Chemistry, 2024, 39(8): 314-323. doi: 10.3866/PKU.DXHX202401008
11. [11]
  Jie ZHAO , Sen LIU , Qikang YIN , Xiaoqing LU , Zhaojie WANG . Theoretical calculation of selective adsorption and separation of CO₂ by alkali metal modified naphthalene/naphthalenediyne. Chinese Journal of Inorganic Chemistry, 2024, 40(3): 515-522. doi: 10.11862/CJIC.20230385
12. [12]
  Zhiyuan TONG , Ziyuan LI , Ke ZHANG . Three-dimensional porous collector based on Cu-Li_6.4La₃Zr_1.4Ta_0.6O₁₂ composite layer for the construction of stable lithium metal anode. Chinese Journal of Inorganic Chemistry, 2025, 41(3): 499-508. doi: 10.11862/CJIC.20240238
13. [13]
  Peng XU , Shasha WANG , Nannan CHEN , Ao WANG , Dongmei YU . Preparation of three-layer magnetic composite Fe₃O₄@polyacrylic acid@ZiF-8 for efficient removal of malachite green in water. Chinese Journal of Inorganic Chemistry, 2024, 40(3): 544-554. doi: 10.11862/CJIC.20230239
14. [14]
  Hui Wang , Abdelkader Labidi , Menghan Ren , Feroz Shaik , Chuanyi Wang . 微观结构调控的g-C₃N₄在光催化NO转化中的最新进展：吸附/活化位点的关键作用. Acta Physico-Chimica Sinica, 2025, 41(5): 100039-. doi: 10.1016/j.actphy.2024.100039
15. [15]
  Simin Fang , Wei Huang , Guanghua Yu , Cong Wei , Mingli Gao , Guangshui Li , Hongjun Tian , Wan Li . Integrating Science and Education in a Comprehensive Chemistry Design Experiment: The Preparation of Copper(I) Oxide Nanoparticles and Its Application in Dye Water Remediation. University Chemistry, 2024, 39(8): 282-289. doi: 10.3866/PKU.DXHX202401023
16. [16]
  Liuyun Chen , Wenju Wang , Tairong Lu , Xuan Luo , Xinling Xie , Kelin Huang , Shanli Qin , Tongming Su , Zuzeng Qin , Hongbing Ji . 软模板法诱导Cu/Al₂O₃深孔道结构促进等离子催化CO₂加氢制二甲醚. Acta Physico-Chimica Sinica, 2025, 41(6): 100054-. doi: 10.1016/j.actphy.2025.100054
17. [17]
  Ziliang KANG , Jiamin ZHANG , Hong AN , Xiaohua LIU , Yang CHEN , Jinping LI , Libo LI . Preparation and water adsorption properties of CaCl₂@MOF-808 in-situ composite moulded particles. Chinese Journal of Inorganic Chemistry, 2024, 40(11): 2133-2140. doi: 10.11862/CJIC.20240282
18. [18]
  Endong YANG , Haoze TIAN , Ke ZHANG , Yongbing LOU . Efficient oxygen evolution reaction of CuCo₂O₄/NiFe-layered bimetallic hydroxide core-shell nanoflower sphere arrays. Chinese Journal of Inorganic Chemistry, 2024, 40(5): 930-940. doi: 10.11862/CJIC.20230369
19. [19]
  Xun Zhu , Chenchen Zhang , Yingying Li , Yin Lu , Na Huang , Dawei Wang . Degradation of perfluorooctanoic acid by inductively heated Fenton-like process over the Fe₃O₄/MIL-101 composite. Chinese Chemical Letters, 2024, 35(12): 109753-. doi: 10.1016/j.cclet.2024.109753
20. [20]
  Bowen Yang , Rui Wang , Benjian Xin , Lili Liu , Zhiqiang Niu . C-SnO₂/MWCNTs Composite with Stable Conductive Network for Lithium-based Semi-Solid Flow Batteries. Acta Physico-Chimica Sinica, 2025, 41(2): 100015-. doi: 10.3866/PKU.WHXB202310024

Get Citation

PDF

XML

Metrics

PDF Downloads(84)
Abstract views(3075)
HTML views(737)

通讯作者: 陈斌, bchen63@163.com

1.
沈阳化工大学材料科学与工程学院沈阳 110142