MOF封装磷/氮离子液体作为高安全性锂离子电池的多功能阻燃添加剂

引用本文: 俞华, 陈鼎都, 王璇, 杨丽君, 王戈明, 胡朴. MOF封装磷/氮离子液体作为高安全性锂离子电池的多功能阻燃添加剂[J]. 物理化学学报, 2026, 42(7): 100201. doi: 10.1016/j.actphy.2025.100201 shu

Citation: Hua Yu, Dingdu Chen, Xuan Wang, Lijun Yang, Geming Wang, Pu Hu. MOF-encapsulated phosphorus/nitrogen ionic liquid as a multifunctional flame-retardant additive for high-safety lithium-ion batteries[J]. Acta Physico-Chimica Sinica, 2026, 42(7): 100201. doi: 10.1016/j.actphy.2025.100201 shu

MOF封装磷/氮离子液体作为高安全性锂离子电池的多功能阻燃添加剂

俞华 ^{1, 2, †,} ,
陈鼎都 ^{3, †,} ,
王璇 ^1, ,
杨丽君 ^2, ,
王戈明 ^{3,
,} ,
胡朴 ^{3,
,}

1.
国网山西省电力公司电力科学研究院, 山西太原 030001
2.
重庆大学电气工程学院, 输变电装备技术全国重点实验室, 重庆 400044
3.
武汉工程大学等离子体化学与新材料湖北省重点实验室, 湖北武汉 430073

通讯作者: Email: wanggemingwit@163.com (王戈明); puhu@wit.edu.cn (胡朴)

摘要: 锂离子电池中碳酸酯类电解液的可燃性存在安全隐患，亟需开发先进阻燃体系。本文提出一种新型电解质添加剂策略，将含磷/氮离子液体(P/N-ILs)封装于金属有机框架(MOF)中。所得的P/N-ILs@MOF复合材料具有高孔隙率和结构稳定性，在有效防止P/N-ILs聚集的同时，保持了磷元素捕获自由基与氮气稀释的协同阻燃功能。添加5 wt% P/N-ILs@MOF(MIE-5)的电解液实现自熄时间缩短90%，极限氧指数提升32%。电化学测试表明，MIE-5在Li|MIE-5|LiFePPO₄电池中展现出优异的循环稳定性，300次循环后容量保持率达84.5%。此外，采用MIE-5电解液的10 Ah石墨|MIE-5|LiFePPO₄软包电池在1C倍率下循环280次后仍保留了97.7%的容量，在2C倍率下保持0.2C容量的94.9%。本研究通过MOF封装技术开创了阻燃性与电化学性能协同提升的新范式，为下一代安全耐用锂离子电池的开发提供了重要思路。

关键词:

English

MOF-encapsulated phosphorus/nitrogen ionic liquid as a multifunctional flame-retardant additive for high-safety lithium-ion batteries

Hua Yu ^{1, 2, †,} ,
Dingdu Chen ^{3, †,} ,
Xuan Wang ^1, ,
Lijun Yang ^2, ,
Geming Wang ^{3,
,} ,
Pu Hu ^{3,
,}

1.
Shanxi Electric Power Research Institute, Taiyuan 030001, Shanxi Province, China
2.
School of Electrical Engineering, State Key Laboratory of Power Transmission Equipment Technology, Chongqing University, Chongqing 400044, China
3.
Provincial Key Laboratory of Plasma Chemistry and Advanced Materials, Wuhan Institute of Technology, Wuhan 430073, Hubei Province, China

Corresponding author: Email: wanggemingwit@163.com (Geming Wang); puhu@wit.edu.cn (Pu Hu)

Received Date: 08 September 2025
Accepted Date: 16 October 2025
Revised Date: 16 October 2025
Available Online: 15 July 2026

Abstract: Safety concerns arising from the flammability of alkyl carbonate-based electrolytes in lithium-ion batteries highlight the urgent need for advanced flame-retardant systems. Herein, we propose a novel electrolyte additive strategy by encapsulating phosphorus/nitrogen-containing ionic liquids (P/N-ILs) within a metal-organic framework (MOF). The resulting P/N-ILs@MOF composite exhibits high porosity and structural stability, effectively preventing P/N-ILs aggregation while maintaining synergistic flame-retardant functions of phosphorus for radical scavenging and nitrogen for gas dilution. Electrolytes containing 5 wt% P/N-ILs@MOF (MIE-5) achieve a 90% reduction in self-extinguishing time and an increased limiting oxygen index of 32%. Electrochemical testing demonstrates that MIE-5 delivers excellent cycling stability, retaining 84.5% capacity after 300 cycles in Li|MIE-5|LiFePPO₄ cells. Moreover, a 10 Ah graphite|MIE-5|LiFePPO₄ pouch cell with MIE-5 maintains 97.7% capacity after 280 cycles at 1C and retains 94.9% of its 0.2C capacity at 2C. This study introduces a new paradigm for integrating flame retardancy with electrochemical performance via MOF-encapsulation, offering significant potential for next-generation safe and durable lithium-ion batteries.

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1.
沈阳化工大学材料科学与工程学院沈阳 110142

MOF封装磷/氮离子液体作为高安全性锂离子电池的多功能阻燃添加剂

通讯作者: Email: wanggemingwit@163.com (王戈明); puhu@wit.edu.cn (胡朴)

English

MOF-encapsulated phosphorus/nitrogen ionic liquid as a multifunctional flame-retardant additive for high-safety lithium-ion batteries

Corresponding author: Email: wanggemingwit@163.com (Geming Wang); puhu@wit.edu.cn (Pu Hu)

CCS Chemistry：嵌段共聚物自组装成 “三明治”二维有机材料，实现纳米级压力传感功能

CCS Chemistry：颜徐州、鲍哲南：你的皮肤可能是一片SPMs

CCS Chemistry：工作高效不疲劳，只须让催化剂动起来

CCS Chemistry：静电组装导向聚合- 聚电解质纳米凝胶量化制备新策略

CCS Chemistry：金黄色葡萄球菌醛基脱氢酶是如何识别特异性底物的？

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通讯作者: 陈斌, bchen63@163.com

中国化学会秘书处

MOF封装磷/氮离子液体作为高安全性锂离子电池的多功能阻燃添加剂

通讯作者: Email: wanggemingwit@163.com (王戈明); puhu@wit.edu.cn (胡朴)

English

MOF-encapsulated phosphorus/nitrogen ionic liquid as a multifunctional flame-retardant additive for high-safety lithium-ion batteries

Corresponding author: Email: wanggemingwit@163.com (Geming Wang); puhu@wit.edu.cn (Pu Hu)

CCS Chemistry：嵌段共聚物自组装成 “三明治”二维有机材料，实现纳米级压力传感功能

CCS Chemistry：颜徐州、鲍哲南： 你的皮肤可能是一片SPMs

CCS Chemistry：工作高效不疲劳，只须让催化剂动起来

CCS Chemistry：静电组装导向聚合- 聚电解质纳米凝胶量化制备新策略

CCS Chemistry：金黄色葡萄球菌醛基脱氢酶是如何识别特异性底物的？

计量

文章相关

通讯作者: 陈斌, bchen63@163.com

中国化学会秘书处

CCS Chemistry：颜徐州、鲍哲南：你的皮肤可能是一片SPMs